Dual-comb spectroscopy of laser-induced plasmas

Bergevin, Jenna; Wu, Tsung-Han; Yeak, Jeremy; Brumfield, Brian E.; Harilal, Sivanandan S.; Phillips, Mark C.; Jones, R. Jason

doi:10.1038/s41467-018-03703-0

Title: Dual-comb spectroscopy of laser-induced plasmas

Journal Article · Wed Mar 28 00:00:00 EDT 2018 · Nature Communications

DOI:https://doi.org/10.1038/s41467-018-03703-0· OSTI ID:1438977

Bergevin, Jenna; Wu, Tsung-Han; Yeak, Jeremy; Brumfield, Brian E.; Harilal, Sivanandan S.; Phillips, Mark C.; Jones, R. Jason

Dual-comb spectroscopy has become a powerful spectroscopic technique in applications that rely on its broad spectral coverage combined with high frequency resolution capabilities. Experiments to date have primarily focused on detection and analysis of multiple gas species under semi-static conditions, with applications ranging from environmental monitoring of greenhouse gases to high resolution molecular spectroscopy. Here, we utilize dual-comb spectroscopy to demonstrate broadband, high-resolution, and time-resolved measurements in a laser induced plasma for the first time. As a first demonstration, we simultaneously detect trace amounts of Rb and K in solid samples with a single laser ablation shot, with transitions separated by over 6 THz (13 nm) and spectral resolution sufficient to resolve isotopic and ground state hyperfine splittings of the Rb D2 line. This new spectroscopic approach offers the broad spectral coverage found in the powerful techniques of laser-induced breakdown spectroscopy (LIBS) while providing the high-resolution and accuracy of cw laser-based spectroscopies.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE

DOE Contract Number:: AC05-76RL01830

OSTI ID:: 1438977

Report Number(s):: PNNL-SA-132479; DN2001000

Journal Information:: Nature Communications, Vol. 9, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

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Time-resolved mid-infrared dual-comb spectroscopy Abbas, Muhammad A.; Pan, Qing; Mandon, Julien Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-53825-8	journal	November 2019
Laser induced breakdown in pulsed helium atmospheric pressure plasma jet Popović, Dean; Bišćan, Marijan; Milošević, Slobodan Plasma Sources Science and Technology, Vol. 28, Issue 5 https://doi.org/10.1088/1361-6595/ab1d10	journal	May 2019
Frequency comb spectroscopy Picqué, Nathalie; Hänsch, Theodor W. Nature Photonics, Vol. 13, Issue 3 https://doi.org/10.1038/s41566-018-0347-5	journal	February 2019
Frequency comb spectroscopy Picqué, Nathalie; Hänsch, Theodor W. arXiv https://doi.org/10.48550/arxiv.1902.11249	text	January 2019
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Broadband Time-Resolved Absorption and Dispersion Spectroscopy of Methane and Ethane in a Plasma Using a Mid-Infrared Dual-Comb Spectrometer Abbas, Muhammad Ali; Dijk, Luuk van; Jahromi, Khalil Eslami Sensors, Vol. 20, Issue 23 https://doi.org/10.3390/s20236831	journal	November 2020
11-μs time-resolved, continuous dual-comb spectroscopy with spectrally filtered mode-locked frequency combs Hoghooghi, Nazanin; Cole, Ryan K.; Rieker, Gregory B. Applied Physics B, Vol. 127, Issue 2 https://doi.org/10.1007/s00340-020-07552-y	journal	January 2021

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