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Title: Directional Forces by Momentumless Excitation and Order-to-Order Transition in Peierls-Distorted Solids: The Case of GeTe

Journal Article · · Physical Review Letters

Sponsoring Organization:
USDOE
Grant/Contract Number:
SC0002623
OSTI ID:
1435993
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Vol. 120 Journal Issue: 18; ISSN 0031-9007
Publisher:
American Physical SocietyCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 30 works
Citation information provided by
Web of Science

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Role of Electronic Excitation in the Amorphization of Ge-Sb-Te Alloys journal June 2011
Transient Structures and Possible Limits of Data Recording in Phase-Change Materials journal June 2015
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Aqueous multiphoton lithography with multifunctional silk-centred bio-resists journal October 2015
Microscopic origin of the fast crystallization ability of Ge–Sb–Te phase-change memory materials journal March 2008
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Multivalency-Induced Band Gap Opening at MoS 2 Edges journal April 2015
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Directional Forces by Momentumless Excitation and Order-to-Order Transition in Peierls-Distorted Solids: The Case of GeTe
Journal Article · Tue May 01 00:00:00 EDT 2018 · Physical Review Letters · OSTI ID:1435993

Finite-temperature second-order many-body perturbation and Hartree–Fock theories for one-dimensional solids: An application to Peierls and charge-density-wave transitions in conjugated polymers
Journal Article · Tue Jan 14 00:00:00 EST 2014 · Journal of Chemical Physics · OSTI ID:1435993

Most theoretical approaches used in nuclear astrophysics to model the nucleosynthesis of heavy elements incorporate the so-called statistical model in order to describe the excitation and decay properties of atomic nuclei. One of the basic assumptions of this model is the validity of the Brink–Axel hypothesis and the related concept of so-called photon strength functions to describe γ-ray transition probabilities. We present a novel experimental approach that allows for the first time to experimentally determine the photon strength function simultaneously in two independent ways by a unique combination of quasi-monochromatic photon beams and a newly implemented γ–γ coincidence setup. This technique does not assume a priori the validity of the Brink–Axel hypothesis and sets a benchmark in terms of the detection sensitivity for measuring decay properties of photo-excited states below the neutron separation energy. The data for the spherical off-shell nucleus 128Te were obtained for γ-ray beam-energy settings between 3 MeV and 9 MeV in steps of 130 keV for the lower beam energies and in steps of up to 280 keV for the highest beam settings. We present a quantitative analysis on the consistency of the derived photon strength function with the Brink–Axel hypothesis. The data clearly demonstrate a discrepancy of up to a factor of two between the photon strength functions extracted from the photoabsorption and photon emission process, respectively. In addition, we observe that the photon strength functions are not independent of the excitation energy, as usually assumed. Thus, we conclude, that the Brink–Axel hypothesis is not strictly fulfilled in the excitation-energy region below the neutron separation threshold (Sn = 8.78 MeV) for the studied case of 128Te.
Journal Article · Tue Jan 01 00:00:00 EST 2019 · Physics Letters B · OSTI ID:1435993

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