Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals

Hachtel, Jordan A.; Davidson, II, Roderick B.; Kovalik, Elena R.; Retterer, Scott T.; Lupini, Andrew R.; Haglund, Jr., Richard F.; Lawrie, Benjamin J.; Pantelides, Sokrates T.

doi:10.1364/OL.43.000927

Title: Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals

Journal Article · Thu Feb 15 00:00:00 EST 2018 · Optics Letters

DOI:https://doi.org/10.1364/OL.43.000927· OSTI ID:1435311

^[1]; Davidson, II, Roderick B. ^[2];

^[3];

^[1];

^[1]; Haglund, Jr., Richard F. ^[4];

^[1]; Pantelides, Sokrates T. ^[2]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Vanderbilt Univ., Nashville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of North Carolina, Chapel Hill, NC (United States)
Vanderbilt Univ., Nashville, TN (United States)

Asymmetric nanophotonic structures enable a wide range of opportunities in optical nanotechnology because they support efficient optical nonlinearities mediated by multiple plasmon resonances over a broad spectral range. The Archimedean nanospiral is a canonical example of a chiral plasmonic structure because it supports even-order nonlinearities that are not generally accessible in locally symmetric geometries. However, the complex spiral response makes nanoscale experimental characterization of the plasmonic near-field structure highly desirable. Here we employ high-efficiency, high-spatial-resolution cathodoluminescence imaging in a scanning transmission electron microscope to describe the spatial, spectral, and polarization response of plasmon modes in the nanospiral geometry.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Vanderbilt Univ., Nashville, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725; FG02-01ER45916; FG02-09ER4655; FG02-09ER46554

OSTI ID:: 1435311

Alternate ID(s):: OSTI ID: 1420366; OSTI ID: 1597874

Journal Information:: Optics Letters, Vol. 43, Issue 4; ISSN 0146-9592

Publisher:: Optical Society of America (OSA)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 11 works

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References (20)

Probing plasmons in three dimensions by combining complementary spectroscopies in a scanning transmission electron microscope Hachtel, J. A.; Marvinney, C.; Mouti, A. Nanotechnology, Vol. 27, Issue 15 https://doi.org/10.1088/0957-4484/27/15/155202	journal	March 2016
Periodically Varying Height in Metal Nano-pillars for Enhanced Generation of Localized Surface Plasmon Field Chamuah, Nabadweep; Nath, Pabitra Plasmonics, Vol. 10, Issue 6 https://doi.org/10.1007/s11468-015-9926-1	journal	April 2015
Multimodal plasmonics in fused colloidal networks Teulle, Alexandre; Bosman, Michel; Girard, Christian Nature Materials, Vol. 14, Issue 1 https://doi.org/10.1038/nmat4114	journal	October 2014
Plasmonics for improved photovoltaic devices Atwater, Harry A.; Polman, Albert Nature Materials, Vol. 9, Issue 3, p. 205-213 https://doi.org/10.1038/nmat2629	journal	February 2010
Signatures of Fano Interferences in the Electron Energy Loss Spectroscopy and Cathodoluminescence of Symmetry-Broken Nanorod Dimers Bigelow, Nicholas W.; Vaschillo, Alex; Camden, Jon P. ACS Nano, Vol. 7, Issue 5 https://doi.org/10.1021/nn401161n	journal	April 2013
Localized Surface Plasmon Resonances in Spatially Dispersive Nano-Objects: Phenomenological Treatise Ginzburg, Pavel; Zayats, Anatoly V. ACS Nano, Vol. 7, Issue 5 https://doi.org/10.1021/nn400842m	journal	April 2013
Plasmonic Response of Nanoscale Spirals Ziegler, Jed I.; Haglund, Richard F. Nano Letters, Vol. 10, Issue 8 https://doi.org/10.1021/nl101475n	journal	August 2010
Plasmon assisted 3D microstructuring of gold nanoparticle-doped polymers Jonušauskas, Linas; Lau, Marcus; Gruber, Peter Nanotechnology, Vol. 27, Issue 15 https://doi.org/10.1088/0957-4484/27/15/154001	journal	February 2016
Angle-Resolved Cathodoluminescence Imaging Polarimetry Osorio, Clara I.; Coenen, Toon; Brenny, Benjamin J. M. ACS Photonics, Vol. 3, Issue 1 https://doi.org/10.1021/acsphotonics.5b00596	journal	December 2015
Au/TiO ₂ /Au as a Plasmonic Coupling Photocatalyst Wang, Hua; You, Tingting; Shi, Weiwei The Journal of Physical Chemistry C, Vol. 116, Issue 10 https://doi.org/10.1021/jp212303q	journal	March 2012
Efficient forward second-harmonic generation from planar archimedean nanospirals Davidson II, Roderick B.; Ziegler, Jed I.; Vargas, Guillermo Nanophotonics, Vol. 4, Issue 1 https://doi.org/10.1515/nanoph-2015-0002	journal	January 2015
Nanoscale optical tomography with cathodoluminescence spectroscopy Atre, Ashwin C.; Brenny, Benjamin J. M.; Coenen, Toon Nature Nanotechnology, Vol. 10, Issue 5 https://doi.org/10.1038/nnano.2015.39	journal	April 2015
Direct Write Protein Patterns for Multiplexed Cytokine Detection from Live Cells Using Electron Beam Lithography Lau, Uland Y.; Saxer, Sina S.; Lee, Juneyoung ACS Nano, Vol. 10, Issue 1 https://doi.org/10.1021/acsnano.5b05781	journal	December 2015
Complex Polarization Response in Plasmonic Nanospirals Ziegler, Jed I.; Haglund, Richard F. Plasmonics, Vol. 8, Issue 2 https://doi.org/10.1007/s11468-012-9436-3	journal	September 2012
Tailoring MoS ₂ Exciton–Plasmon Interaction by Optical Spin–Orbit Coupling Li, Ziwei; Li, Yu; Han, Tianyang ACS Nano, Vol. 11, Issue 2 https://doi.org/10.1021/acsnano.6b06834	journal	December 2016
Nonlocality-driven supercontinuum white light generation in plasmonic nanostructures Krasavin, A. V.; Ginzburg, P.; Wurtz, G. A. Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms11497	journal	May 2016
Biosensing with plasmonic nanosensors Anker, Jeffrey N.; Hall, W. Paige; Lyandres, Olga Nature Materials, Vol. 7, Issue 6 https://doi.org/10.1038/nmat2162	journal	June 2008
Analysis of polarization by means of polarized cathodoluminescence spectroscopy in a TEM Ohno, Y. Journal of Electron Microscopy, Vol. 51, Issue 5 https://doi.org/10.1093/jmicro/51.5.281	journal	October 2002
Seeing and measuring in colours: Electron microscopy and spectroscopies applied to nano-optics Kociak, Mathieu; Stéphan, Odile; Gloter, Alexandre Comptes Rendus Physique, Vol. 15, Issue 2-3 https://doi.org/10.1016/j.crhy.2013.10.003	journal	February 2014
Hot Electron Generation and Cathodoluminescence Nanoscopy of Chiral Split Ring Resonators Fang, Yurui; Verre, Ruggero; Shao, Lei Nano Letters, Vol. 16, Issue 8 https://doi.org/10.1021/acs.nanolett.6b02154	journal	July 2016

Cited By (1)

Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators Hachtel, Jordan A.; Cho, Sang-Yeon; Davidson, Roderick B. Light: Science & Applications, Vol. 8, Issue 1 https://doi.org/10.1038/s41377-019-0136-z	journal	March 2019

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Related Subjects

36 MATERIALS SCIENCE
Surface plasmons
Cathodoluminescence
Subwavelength structures
nano-structures
Polarization-selective devices