Optical nonlinearities of excitons in monolayer MoS2

Soh, Daniel B.  S.; Rogers, Christopher; Gray, Dodd J.; Chatterjee, Eric; Mabuchi, Hideo

doi:10.1103/PhysRevB.97.165111

Title: Optical nonlinearities of excitons in monolayer ${MoS}_{2}$

Journal Article · Fri Apr 06 00:00:00 EDT 2018 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.97.165111· OSTI ID:1431585

^[1]; Rogers, Christopher ^[2]; Gray, Dodd J. ^[2]; Chatterjee, Eric ^[2]; Mabuchi, Hideo ^[2]

Stanford Univ., CA (United States). Edward L. Ginzton Lab.; Sandia National Lab. (SNL-CA), Livermore, CA (United States)
Stanford Univ., CA (United States). Edward L. Ginzton Lab.

We calculate linear and nonlinear optical susceptibilities arising from the excitonic states of monolayer MoS₂ for in-plane light polarizations, using second-quantized bound and unbound exciton operators. Optical selection rules are critical for obtaining the susceptibilities. We derive the valley-chirality rule for the second-order harmonic generation in monolayer MoS₂ and find that the third-order harmonic process is efficient only for linearly polarized input light while the third-order two-photon process (optical Kerr effect) is efficient for circularly polarized light using a higher order exciton state. The absence of linear absorption due to the band gap and the unusually strong two-photon third-order nonlinearity make the monolayer MoS₂ excitonic structure a promising resource for coherent nonlinear photonics.

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Research Organization:: Stanford Univ., CA (United States); Sandia National Lab. (SNL-CA), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: NA0003525

OSTI ID:: 1431585

Alternate ID(s):: OSTI ID: 1432104

Journal Information:: Physical Review B, Vol. 97, Issue 16; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 18 works

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Title: Optical nonlinearities of excitons in monolayer MoS 2

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Title: Optical nonlinearities of excitons in monolayer ${MoS}_{2}$