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Title: Charge Berezinskii-Kosterlitz-Thouless transition in superconducting NbTiN films

Abstract

Three decades after the prediction of charge-vortex duality in the critical vicinity of the two-dimensional superconductor-insulator transition (SIT), one of the fundamental implications of this duality-the charge Berezinskii-Kosterlitz-Thouless (BKT) transition that should occur on the insulating side of the SIT-has remained unobserved. The dual picture of the process points to the existence of a superinsulating state endowed with zero conductance at finite temperature. Here, we report the observation of the charge BKT transition on the insulating side of the SIT in 10 nm thick NbTiN films, identified by the BKT critical behavior of the temperature and magnetic field dependent resistance, and map out the magnetic-field dependence of the critical temperature of the charge BKT transition. Lastly, we ascertain the effects of the finite electrostatic screening length and its divergence at the magnetic field-tuned approach to the superconductor-insulator transition.

Authors:
ORCiD logo [1];  [2]; ORCiD logo [3];  [1];  [1];  [1];  [2]; ORCiD logo [4];  [5]
  1. A. V. Rzhanov Institute of Semiconductor Physics SB RAS, Novosibirsk (Russia); Novosibirsk State Univ., Novosibirsk (Russia)
  2. California Inst. of Technology (CalTech), Pasadena, CA (United States)
  3. Institut de recherches sur les lois fundamentales de l’univers, Gif-sur-Yvette (France)
  4. Argonne National Lab. (ANL), Argonne, IL (United States); Univ. of Chicago, Chicago, IL (United States)
  5. A. V. Rzhanov Institute of Semiconductor Physics SB RAS, Novosibirsk (Russia); Novosibirsk State Univ., Novosibirsk (Russia); The Univ. of Chicago, Chicago, IL (United States); Univ. Autonoma de Madrid, Madrid (Spain)
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; Ministry of Education and Science of the Russian Federation; Alexander von Humboldt Foundation
OSTI Identifier:
1431229
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 8; Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Mironov, Alexey Yu., Silevitch, Daniel M., Proslier, Thomas, Postolova, Svetlana V., Burdastyh, Maria V., Gutakovskii, Anton K., Rosenbaum, Thomas F., Vinokur, Valerii V., and Baturina, Tatyana I. Charge Berezinskii-Kosterlitz-Thouless transition in superconducting NbTiN films. United States: N. p., 2018. Web. doi:10.1038/s41598-018-22451-1.
Mironov, Alexey Yu., Silevitch, Daniel M., Proslier, Thomas, Postolova, Svetlana V., Burdastyh, Maria V., Gutakovskii, Anton K., Rosenbaum, Thomas F., Vinokur, Valerii V., & Baturina, Tatyana I. Charge Berezinskii-Kosterlitz-Thouless transition in superconducting NbTiN films. United States. doi:10.1038/s41598-018-22451-1.
Mironov, Alexey Yu., Silevitch, Daniel M., Proslier, Thomas, Postolova, Svetlana V., Burdastyh, Maria V., Gutakovskii, Anton K., Rosenbaum, Thomas F., Vinokur, Valerii V., and Baturina, Tatyana I. Tue . "Charge Berezinskii-Kosterlitz-Thouless transition in superconducting NbTiN films". United States. doi:10.1038/s41598-018-22451-1. https://www.osti.gov/servlets/purl/1431229.
@article{osti_1431229,
title = {Charge Berezinskii-Kosterlitz-Thouless transition in superconducting NbTiN films},
author = {Mironov, Alexey Yu. and Silevitch, Daniel M. and Proslier, Thomas and Postolova, Svetlana V. and Burdastyh, Maria V. and Gutakovskii, Anton K. and Rosenbaum, Thomas F. and Vinokur, Valerii V. and Baturina, Tatyana I.},
abstractNote = {Three decades after the prediction of charge-vortex duality in the critical vicinity of the two-dimensional superconductor-insulator transition (SIT), one of the fundamental implications of this duality-the charge Berezinskii-Kosterlitz-Thouless (BKT) transition that should occur on the insulating side of the SIT-has remained unobserved. The dual picture of the process points to the existence of a superinsulating state endowed with zero conductance at finite temperature. Here, we report the observation of the charge BKT transition on the insulating side of the SIT in 10 nm thick NbTiN films, identified by the BKT critical behavior of the temperature and magnetic field dependent resistance, and map out the magnetic-field dependence of the critical temperature of the charge BKT transition. Lastly, we ascertain the effects of the finite electrostatic screening length and its divergence at the magnetic field-tuned approach to the superconductor-insulator transition.},
doi = {10.1038/s41598-018-22451-1},
journal = {Scientific Reports},
issn = {2045-2322},
number = 1,
volume = 8,
place = {United States},
year = {2018},
month = {3}
}

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Works referenced in this record:

Superinsulator and quantum synchronization
journal, April 2008

  • Vinokur, Valerii M.; Baturina, Tatyana I.; Fistul, Mikhail V.
  • Nature, Vol. 452, Issue 7187
  • DOI: 10.1038/nature06837

Disordered Berezinskii-Kosterlitz-Thouless transition and superinsulation
journal, January 2018


From quantum corrections to magnetic-field-tuned superconductor–insulator quantum phase transition in TiN films
journal, April 2005


Superconductivity in the insulating phase above the field-tuned superconductor–insulator transition in disordered indium oxide films
journal, May 2005


Presence of quantum diffusion in two dimensions: Universal resistance at the superconductor-insulator transition
journal, January 1990


Charge Kosterlitz-Thouless Transition in Two-Dimensional Arrays of Small Tunnel Junctions
journal, August 1995

  • Kobayashi, Shun-ichi; Kanda, Akinobu; Yamada, Ren-ichi
  • Japanese Journal of Applied Physics, Vol. 34, Issue Part 1, No. 8B
  • DOI: 10.1143/JJAP.34.4548

Gauge theories of Josephson junction arrays
journal, September 1996


The superconducting transition of 2-D Josephson-junction arrays in a small perpendicular magnetic field
journal, June 1990

  • van der Zant, H. S. J.; Rijken, H. A.; Mooij, J. E.
  • Journal of Low Temperature Physics, Vol. 79, Issue 5-6
  • DOI: 10.1007/BF00682288

The critical properties of the two-dimensional xy model
journal, March 1974


Superinsulator–superconductor duality in two dimensions
journal, April 2013


Charge and vortex dynamics in arrays of tunnel junctions
journal, March 1991


Quantum Metallicity on the High-Field Side of the Superconductor-Insulator Transition
journal, March 2007


Disorder induced granularity in an amorphous superconductor
journal, June 1994


Effect of self-capicitance on charge Kosterlitz-Thouless transition in two-dimensional arrays of small tunnel junctions
journal, September 1996


Quantum Superinductor with Tunable Nonlinearity
journal, September 2012


Hyperactivated resistance in TiN films on the insulating side of the disorder-driven superconductor-insulator transition
journal, February 2008


Disorder-Induced Inhomogeneities of the Superconducting State Close to the Superconductor-Insulator Transition
journal, October 2008


(Invited) Atomic Layer Deposition of Superconductors
conference, January 2011

  • Proslier, Thomas; Klug, J.; Becker, Nicholas C.
  • 220th ECS Meeting, ECS Transactions
  • DOI: 10.1149/1.3633673

Long range order and metastability in two dimensional solids and superfluids. (Application of dislocation theory)
journal, June 1972


Observation of Giant Positive Magnetoresistance in a Cooper Pair Insulator
journal, October 2009


Improvement of the critical temperature of superconducting NbTiN and NbN thin films using the AlN buffer layer
journal, March 2010


Precursor of Charge KTB Transition in Normal and Superconducting Tunnel Junction Array
journal, January 1995

  • Kanda, Akinobu; Kobayashi, Shun-ichi
  • Journal of the Physical Society of Japan, Vol. 64, Issue 1
  • DOI: 10.1143/JPSJ.64.19

Quantum phase transitions in disordered two-dimensional superconductors
journal, August 1990


Emergence of nanoscale inhomogeneity in the superconducting state of a homogeneously disordered conventional superconductor
journal, October 2013

  • Kamlapure, Anand; Das, Tanmay; Ganguli, Somesh Chandra
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep02979

Unbinding of charge-anticharge pairs in two-dimensional arrays of small tunnel junctions
journal, July 1990


Collective Cooper-Pair Transport in the Insulating State of Josephson-Junction Arrays
journal, February 2008


Analysis of Recent Measurements of the Viscosity of Glasses
journal, June 1925


Phase diagram of the strongly disordered s -wave superconductor NbN close to the metal-insulator transition
journal, January 2012


Nature of the superconductor–insulator transition in disordered superconductors
journal, October 2007

  • Dubi, Yonatan; Meir, Yigal; Avishai, Yshai
  • Nature, Vol. 449, Issue 7164
  • DOI: 10.1038/nature06180

The two-dimensional Coulomb gas, vortex unbinding, and superfluid-superconducting films
journal, October 1987


Magnetic field induced emergent inhomogeneity in a superconducting film with weak and homogeneous disorder
journal, August 2017


Collapse of the Cooper pair phase coherence length at a superconductor-to-insulator transition
journal, February 2013


Evidence for a Finite-Temperature Insulator
journal, August 2015

  • Ovadia, M.; Kalok, D.; Tamir, I.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep13503

Superconductor-Insulator Transitions
journal, August 2010


Duality picture of Superconductor-insulator transitions on Superconducting nanowire
journal, June 2016

  • Makise, Kazumasa; Terai, Hirotaka; Tominari, Yukihiro
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep27001

Dielectric function near a polarization catastrophe
journal, August 1984


Localized Superconductivity in the Quantum-Critical Region of the Disorder-Driven Superconductor-Insulator Transition in TiN Thin Films
journal, December 2007


Metal–insulator transition in a weakly interacting many-electron system with localized single-particle states
journal, May 2006


Nanopattern-stimulated superconductor-insulator transition in thin TiN films
journal, February 2011


Stress Tuning of the Metal-Insulator Transition at Millikelvin Temperatures
journal, May 1982


Atomic layer deposition of transition metals
journal, October 2003

  • Lim, Booyong S.; Rahtu, Antti; Gordon, Roy G.
  • Nature Materials, Vol. 2, Issue 11
  • DOI: 10.1038/nmat1000

Ordering, metastability and phase transitions in two-dimensional systems
journal, April 1973

  • Kosterlitz, J M; Thouless, D J
  • Journal of Physics C: Solid State Physics, Vol. 6, Issue 7, p. 1181-1203
  • DOI: 10.1088/0022-3719/6/7/010

Die Abhängigkeit der Viscosität von der Temperatur bie unterkühlten Flüssigkeiten
journal, October 1926

  • Tammann, G.; Hesse, W.
  • Zeitschrift für anorganische und allgemeine Chemie, Vol. 156, Issue 1
  • DOI: 10.1002/zaac.19261560121

Existence of a Bose metal at T = 0
journal, July 1999


Dual threshold diode based on the superconductor-to-insulator transition in ultrathin TiN films
journal, January 2013

  • Baturina, Tatyana I.; Kalok, David; Bilušić, Ante
  • Applied Physics Letters, Vol. 102, Issue 4
  • DOI: 10.1063/1.4789510

Superconducting phase transitions in ultrathin TiN films
journal, January 2012


High-field termination of a Cooper-pair insulator
journal, June 2015


Electronic transport in two-dimensional high dielectric constant nanosystems
journal, April 2015

  • Ortuño, M.; Somoza, A. M.; Vinokur, V. M.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep09667

Duality symmetry and its breakdown in the vicinity of the superconductor–insulator transition
journal, June 2013

  • Ovadia, Maoz; Kalok, David; Sacépé, Benjamin
  • Nature Physics, Vol. 9, Issue 7
  • DOI: 10.1038/nphys2636

Interacting Electrons in Disordered Wires: Anderson Localization and Low- T Transport
journal, November 2005


Strongly Disordered TiN and NbTiN s -Wave Superconductors Probed by Microwave Electrodynamics
journal, September 2012


Superconductor-insulator transition and universal resistance in Josephson-junction arrays in a magnetic field
journal, September 1990


Experimental Evidence for a Collective Insulating State in Two-Dimensional Superconductors
journal, January 2005


Fluctuation conductivity in disordered superconducting films
journal, May 2012

  • Tikhonov, Konstantin S.; Schwiete, Georg; Finkel'stein, Alexander M.
  • Physical Review B, Vol. 85, Issue 17
  • DOI: 10.1103/PhysRevB.85.174527

Quantum-critical region of the disorder-driven superconductor–insulator transition
journal, February 2008