Interphases in Sodium‐Ion Batteries

Song, Junhua; Xiao, Biwei; Lin, Yuehe; Xu, Kang; Li, Xiaolin

doi:10.1002/aenm.201703082

Interphases in Sodium‐Ion Batteries

Journal Article · Wed Mar 14 00:00:00 EDT 2018 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201703082· OSTI ID:1426322

Song, Junhua ^[1]; Xiao, Biwei ^[2]; Lin, Yuehe ^[3]; Xu, Kang ^[4]; Li, Xiaolin ^[2]

Pacific Northwest National Laboratory Richland WA 99354 USA, School of Mechanical and Materials Engineering Washington State University Pullman WA 99164 USA
Pacific Northwest National Laboratory Richland WA 99354 USA
School of Mechanical and Materials Engineering Washington State University Pullman WA 99164 USA
Electrochemistry Branch Energy and Power Division Sensor and Electronics Directorate U.S. Army Research Laboratory 2800 Powder Mill Road Adelphi MD 20783‐1197 USA

Abstract

Sodium‐ion batteries (SIBs) as economical, high energy alternatives to lithium‐ion batteries (LIBs) have received significant attention for large‐scale energy storage in the last few years. While the efforts of developing SIBs have benefited from the knowledge learned in LIBs, thanks to the apparent proximity between Na‐ions and Li‐ions, the unique physical and chemical properties of Na‐ions also distinctly differ themselves from Li‐ions. It is expected that SIBs have drastically different electrode material structure, solvation–desolvation behavior, electrode–electrolyte interphase stabilities, ion transfer properties, and hence electrochemical performance of batteries. In this review, the authors comprehensively summarize the current understanding of the anode solid electrolyte interphase and cathode electrolyte interphase in SIBs, with an emphasis on how the tuning of the stability and ion transfer properties of interphases fundamentally determines the reversibility and efficiency of electrochemical reactions. Through these carefully screened references, the authors intend to reveal the intrinsic correlation between the properties/functionalities of the interphases and the electrochemical performance of batteries.

View Accepted Manuscript (Publisher)

Sponsoring Organization:: USDOE

OSTI ID:: 1426322

Alternate ID(s):: OSTI ID: 1572521

Journal Information:: Advanced Energy Materials, Journal Name: Advanced Energy Materials Journal Issue: 17 Vol. 8; ISSN 1614-6832

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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