Review—Practical Challenges Hindering the Development of Solid State Li Ion Batteries

Kerman, Kian; Luntz, Alan; Viswanathan, Venkatasubramanian; Chiang, Yet-Ming; Chen, Zhebo

doi:10.1149/2.1571707jes

Review—Practical Challenges Hindering the Development of Solid State Li Ion Batteries

Journal Article · Fri Jun 09 00:00:00 EDT 2017 · Journal of the Electrochemical Society

DOI:https://doi.org/10.1149/2.1571707jes· OSTI ID:1425964

Kerman, Kian ^[1]; Luntz, Alan ^[2]; ^[3]; Chiang, Yet-Ming ^[4]; Chen, Zhebo ^[2]

Stanford Univ., CA (United States); Harvard University
Stanford Univ., CA (United States)
Carnegie Mellon Univ., Pittsburgh, PA (United States)
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Solid state electrolyte systems boasting Li+ conductivity of >10 mS cm^-1 at room temperature have opened the potential for developing a solid state battery with power and energy densities that are competitive with conventional liquid electrolyte systems. The primary focus of this review is twofold. First, differences in Li penetration resistance in solid state systems are discussed, and kinetic limitations of the solid state interface are highlighted. Second, technological challenges associated with processing such systems in relevant form factors are elucidated, and architectures needed for cell level devices in the context of product development are reviewed. Specific research vectors that provide high value to advancing solid state batteries are outlined and discussed.

View Accepted Manuscript (DOE)

Research Organization:: Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V)

Grant/Contract Number:: EE0007810

OSTI ID:: 1425964

Journal Information:: Journal of the Electrochemical Society, Journal Name: Journal of the Electrochemical Society Journal Issue: 7 Vol. 164; ISSN 0013-4651

Publisher:: The Electrochemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Tape Casting as a Multi Purpose Shaping Technology for Different Applications in Energy Issues Schafbauer, Wolfgang; Schulze-Küppers, Falk; Baumann, Stefan Materials Science Forum, Vol. 706-709 https://doi.org/10.4028/www.scientific.net/MSF.706-709.1035	journal	January 2012
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Thermal Stability of Various Cathode Materials against Li_6.25Al_0.25La₃Zr₂O₁₂ Electrolyte Wakasugi, Jungo; Munakata, Hirokazu; Kanamura, Kiyoshi Electrochemistry, Vol. 85, Issue 2 https://doi.org/10.5796/electrochemistry.85.77	journal	January 2017
The Mysterious Story of the Battery Startup That Promised GM a 200-Mile Electric Car LeVine, Steve The Best Business Writing 2014 https://doi.org/10.7312/star17015-024	book	December 2014

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Investigation on the interface between Li10GeP2S12 electrolyte and carbon conductive agents in all-solid-state lithium battery Yoon, Kyungho; Kim, Jung-Joon; Seong, Won Mo Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-26101-4	journal	May 2018
Building Better Batteries in the Solid State: A Review Mauger, Alain; Julien, Christian M.; Paolella, Andrea Materials, Vol. 12, Issue 23, p. 3892 https://doi.org/10.3390/ma12233892	journal	November 2019
Spark Plasma Sintering of Lithium Aluminum Germanium Phosphate Solid Electrolyte and its Electrochemical Properties Zhu, Hongzheng; Prasad, Anil; Doja, Somi Nanomaterials, Vol. 9, Issue 8 https://doi.org/10.3390/nano9081086	journal	July 2019
Correlative electrochemical strain and scanning electron microscopy for local characterization of the solid state electrolyte Li _1.3 Al _0.3 Ti _1.7 (PO ₄ ) ₃ Schön, Nino; Gunduz, Deniz Cihan; Yu, Shicheng Beilstein Journal of Nanotechnology, Vol. 9 https://doi.org/10.3762/bjnano.9.148	journal	January 2018
A Brief Review of Current Lithium Ion Battery Technology and Potential Solid State Battery Technologies Ulvestad, Andrew arXiv https://doi.org/10.48550/arxiv.1803.04317	preprint	January 2018
Progress of the Interface Design in All-Solid-State Li-S Batteries Yue, Junpei; Yan, Min; Yin, Ya-Xia Advanced Functional Materials, Vol. 28, Issue 38 https://doi.org/10.1002/adfm.201707533	journal	March 2018
Enhanced Interfacial Stability of Hybrid-Electrolyte Lithium-Sulfur Batteries with a Layer of Multifunctional Polymer with Intrinsic Nanoporosity Yu, Xingwen; Manthiram, Arumugam Advanced Functional Materials, Vol. 29, Issue 3 https://doi.org/10.1002/adfm.201805996	journal	November 2018
Mixed Electronic and Ionic Conduction Properties of Lithium Lanthanum Titanate Wang, Michael J.; Wolfenstine, Jeffrey B.; Sakamoto, Jeff Advanced Functional Materials, Vol. 30, Issue 10 https://doi.org/10.1002/adfm.201909140	journal	January 2020
In Situ Transmission Electron Microscopy for Energy Materials and Devices Fan, Zheng; Zhang, Liqiang; Baumann, Daniel Advanced Materials, Vol. 31, Issue 33 https://doi.org/10.1002/adma.201900608	journal	June 2019
Electrochemical and Structural Analysis in All‐Solid‐State Lithium Batteries by Analytical Electron Microscopy: Progress and Perspectives Zhang, Chunchen; Feng, Yuzhang; Han, Zhen Advanced Materials https://doi.org/10.1002/adma.201903747	journal	October 2019
High Capacity All-Solid-State Lithium Batteries Enabled by Pyrite-Sulfur Composites Ulissi, Ulderico; Ito, Seitaro; Hosseini, Seyed Milad Advanced Energy Materials, Vol. 8, Issue 26 https://doi.org/10.1002/aenm.201801462	journal	July 2018
Ameliorating the Interfacial Problems of Cathode and Solid‐State Electrolytes by Interface Modification of Functional Polymers Wang, Li‐Ping; Zhang, Xu‐Dong; Wang, Tai‐Shan Advanced Energy Materials, Vol. 8, Issue 24 https://doi.org/10.1002/aenm.201801528	journal	July 2018
Slurry‐Fabricable Li ⁺ ‐Conductive Polymeric Binders for Practical All‐Solid‐State Lithium‐Ion Batteries Enabled by Solvate Ionic Liquids Oh, Dae Yang; Nam, Young Jin; Park, Kern Ho Advanced Energy Materials, Vol. 9, Issue 16 https://doi.org/10.1002/aenm.201802927	journal	February 2019
Diffusion Limitation of Lithium Metal and Li–Mg Alloy Anodes on LLZO Type Solid Electrolytes as a Function of Temperature and Pressure Krauskopf, Thorben; Mogwitz, Boris; Rosenbach, Carolin Advanced Energy Materials, Vol. 9, Issue 44 https://doi.org/10.1002/aenm.201902568	journal	October 2019
Understanding Li‐Ion Dynamics in Lithium Hydroxychloride (Li ₂ OHCl) Solid State Electrolyte via Addressing the Role of Protons Song, Ah‐Young; Turcheniuk, Kostiantyn; Leisen, Johannes Advanced Energy Materials, Vol. 10, Issue 8 https://doi.org/10.1002/aenm.201903480	journal	January 2020
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Ice as Solid Electrolyte To Conduct Various Kinds of Ions Guo, Zeliang; Wang, Tianshuai; Wei, Hehe Angewandte Chemie, Vol. 131, Issue 36 https://doi.org/10.1002/ange.201907832	journal	July 2019
Salt-Based Organic-Inorganic Nanocomposites: Towards A Stable Lithium Metal/Li ₁₀ GeP ₂ S ₁₂ Solid Electrolyte Interface Gao, Yue; Wang, Daiwei; Li, Yuguang C. Angewandte Chemie International Edition, Vol. 57, Issue 41 https://doi.org/10.1002/anie.201807304	journal	September 2018
Kinetics‐Controlled Degradation Reactions at Crystalline LiPON/Li _x CoO ₂ and Crystalline LiPON/Li‐Metal Interfaces Leung, Kevin; Pearse, Alexander J.; Talin, A. Alec ChemSusChem, Vol. 11, Issue 12 https://doi.org/10.1002/cssc.201800027	journal	March 2018
Synthesis and Properties of NaSICON‐type LATP and LAGP Solid Electrolytes DeWees, Rachel; Wang, Hui ChemSusChem, Vol. 12, Issue 16 https://doi.org/10.1002/cssc.201900725	journal	July 2019
Direct Solution‐Based Synthesis of Na ₄ (B ₁₂ H ₁₂ )(B ₁₀ H ₁₀ ) Solid Electrolyte Gigante, Angelina; Duchêne, Léo; Moury, Romain ChemSusChem, Vol. 12, Issue 21 https://doi.org/10.1002/cssc.201902152	journal	October 2019
Sustainable Battery Materials from Biomass Liedel, Clemens ChemSusChem, Vol. 13, Issue 9 https://doi.org/10.1002/cssc.201903577	journal	April 2020
Sulfide‐Compatible Conductive and Adhesive Glue‐Like Interphase Engineering for Sheet‐Type All‐Solid‐State Battery Cho, Woosuk; Park, Jesik; Kim, Kyungsu Small https://doi.org/10.1002/smll.201902138	journal	August 2019
Data‐Driven Materials Exploration for Li‐Ion Conductive Ceramics by Exhaustive and Informatics‐Aided Computations Nakayama, Masanobu; Kanamori, Kenta; Nakano, Koki The Chemical Record, Vol. 19, Issue 4 https://doi.org/10.1002/tcr.201800129	journal	November 2018
Towards Synergistic Electrode–Electrolyte Design Principles for Nonaqueous Li–O $$_2$$ 2 batteries Khetan, Abhishek; Krishnamurthy, Dilip; Viswanathan, Venkatasubramanian Topics in Current Chemistry, Vol. 376, Issue 2 https://doi.org/10.1007/s41061-018-0188-1	journal	March 2018
Batteries and fuel cells for emerging electric vehicle markets Cano, Zachary P.; Banham, Dustin; Ye, Siyu Nature Energy, Vol. 3, Issue 4 https://doi.org/10.1038/s41560-018-0108-1	journal	April 2018
Characterization and performance evaluation of lithium-ion battery separators Lagadec, Marie Francine; Zahn, Raphael; Wood, Vanessa Nature Energy, Vol. 4, Issue 1 https://doi.org/10.1038/s41560-018-0295-9	journal	December 2018
High electronic conductivity as the origin of lithium dendrite formation within solid electrolytes Han, Fudong; Westover, Andrew S.; Yue, Jie Nature Energy, Vol. 4, Issue 3 https://doi.org/10.1038/s41560-018-0312-z	journal	January 2019
Challenges and opportunities towards fast-charging battery materials Liu, Yayuan; Zhu, Yangying; Cui, Yi Nature Energy, Vol. 4, Issue 7 https://doi.org/10.1038/s41560-019-0405-3	journal	June 2019
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Probing ion current in solid-electrolytes at the meso- and nanoscale Martinez, Joseph; Ashby, David; Zhu, Cheng Faraday Discussions, Vol. 210 https://doi.org/10.1039/c8fd00071a	journal	January 2018
Formation of self-limited, stable and conductive interfaces between garnet electrolytes and lithium anodes for reversible lithium cycling in solid-state batteries He, Minghui; Cui, Zhonghui; Chen, Cheng Journal of Materials Chemistry A, Vol. 6, Issue 24 https://doi.org/10.1039/c8ta02276c	journal	January 2018
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Influence of electronically conductive additives on the cycling performance of argyrodite-based all-solid-state batteries Strauss, Florian; Stepien, Dominik; Maibach, Julia RSC Advances, Vol. 10, Issue 2 https://doi.org/10.1039/c9ra10253a	journal	January 2020
A review on strategies addressing interface incompatibilities in inorganic all-solid-state lithium batteries Gurung, Ashim; Pokharel, Jyotshna; Baniya, Abiral Sustainable Energy & Fuels, Vol. 3, Issue 12 https://doi.org/10.1039/c9se00549h	journal	January 2019
Organic electrode materials with solid-state battery technology Heiska, Juho; Nisula, Mikko; Karppinen, Maarit Journal of Materials Chemistry A, Vol. 7, Issue 32 https://doi.org/10.1039/c9ta04328d	journal	January 2019
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How Metallic Protection Layers Extend the Lifetime of NASICON-Based Solid-State Lithium Batteries Cortes, Francisco Javier Quintero; Lewis, John A.; Tippens, Jared Journal of The Electrochemical Society, Vol. 167, Issue 5 https://doi.org/10.1149/2.0032005jes	journal	October 2019
Modeling and Simulation of Pore Morphology Modifications using Laser-Structured Graphite Anodes in Lithium-Ion Batteries Kraft, Ludwig; Habedank, Jan B.; Frank, Alexander Journal of The Electrochemical Society, Vol. 167, Issue 1 https://doi.org/10.1149/2.0062001jes	journal	September 2019
Defect Detection in Solid-State Battery Electrolytes Using Lock-In Thermal Imaging Sulas, Dana B.; Johnston, Steve; Seitzman, Natalie Journal of The Electrochemical Society, Vol. 165, Issue 13 https://doi.org/10.1149/2.0131814jes	journal	January 2018
Lithium Dendrite Growth Suppression and Ionic Conductivity of Li ₂ S-P ₂ S ₅ -P ₂ O ₅ Glass Solid Electrolytes Prepared by Mechanical Milling Cengiz, Mazlum; Oh, Hyukkeun; Lee, Se-Hee Journal of The Electrochemical Society, Vol. 166, Issue 16 https://doi.org/10.1149/2.0311916jes	journal	January 2019
Hot Formation for Improved Low Temperature Cycling of Anode-Free Lithium Metal Batteries Genovese, Matthew; Louli, A. J.; Weber, Rochelle Journal of The Electrochemical Society, Vol. 166, Issue 14 https://doi.org/10.1149/2.0661914jes	journal	January 2019
Higher Energy Barrier for Interfacial Li-Ion Transfer from EC/LiPF ₆ Electrolyte into (010) LiFePO ₄ Cathode Surface than Bulk Li-Ion Diffusion within Both Cathode and Electrolyte Bhandari, Arihant; Gupta, Prashant Kumar; Bhattacharya, Jishnu Journal of The Electrochemical Society, Vol. 166, Issue 13 https://doi.org/10.1149/2.0851913jes	journal	January 2019
Role of Stress Concentrations on the Electrochemical Response of a Li-Ion Battery Anode Particle Ansari, Mohammad Ayub; Kumbhar, Pramod Yallappa; Swaminathan, Narasimhan Journal of The Electrochemical Society, Vol. 166, Issue 12 https://doi.org/10.1149/2.0881912jes	journal	January 2019
Slurry-Based Processing of Solid Electrolytes: A Comparative Binder Study Riphaus, Nathalie; Strobl, Philipp; Stiaszny, Barbara Journal of The Electrochemical Society, Vol. 165, Issue 16 https://doi.org/10.1149/2.0961816jes	journal	January 2018
Synthesis and Electrochemical Characterization of a Glass-Ceramic Li ₇ P ₂ S ₈ I Solid Electrolyte for All-Solid-State Li-Ion Batteries Choi, Seon-Joo; Lee, Sang-Hun; Ha, Yoon-Cheol Journal of The Electrochemical Society, Vol. 165, Issue 5 https://doi.org/10.1149/2.0981805jes	journal	January 2018
Free-Standing PEO/LiTFSI/LAGP Composite Electrolyte Membranes for Applications to Flexible Solid-State Lithium-Based Batteries Lee, Jeremy; Howell, Thomas; Rottmayer, Michael Journal of The Electrochemical Society, Vol. 166, Issue 2 https://doi.org/10.1149/2.1321902jes	journal	January 2019
Lithium Metal Penetration Induced by Electrodeposition through Solid Electrolytes: Example in Single-Crystal Li ₆ La ₃ ZrTaO ₁₂ Garnet Swamy, Tushar; Park, Richard; Sheldon, Brian W. Journal of The Electrochemical Society, Vol. 165, Issue 16 https://doi.org/10.1149/2.1391814jes	journal	January 2018
Spark Plasma Sintering of Lithium Aluminum Germanium Phosphate Solid Electrolyte and its Electrochemical Properties Zhu, Hongzheng; Prasad, Anil; Doja, Somi Multidisciplinary Digital Publishing Institute https://doi.org/10.14288/1.0380661	text	January 2019
Correlative electrochemical strain and scanning electron microscopy for local characterization of the solid state electrolyte Li1.3Al0.3Ti1.7(PO4)3 Schön, Nino Philippe; Gunduz, Deniz Cihan; Yu, Shicheng RWTH Aachen University https://doi.org/10.18154/rwth-2018-224903	text	January 2018
Slurry-Based Processing of Solid Electrolytes: A Comparative Binder Study Riphaus, Nathalie; Strobl, Philipp; Stiaszny, Barbara Karlsruhe https://doi.org/10.5445/ir/1000089322	text	January 2018
Influence of electronically conductive additives on the cycling performance of argyrodite-based all-solid-state batteries Strauss, Florian; Stepien, Dominik; Maibach, Julia Karlsruhe https://doi.org/10.5445/ir/1000105409	text	January 2020

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