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Stripes developed at the strong limit of nematicity in FeSe film

Journal Article · · Nature Physics
DOI:https://doi.org/10.1038/nphys4186· OSTI ID:1425888
 [1];  [2];  [3];  [3];  [4];  [5];  [3];  [6];  [5];  [6];  [7];  [8];  [7]
  1. Tsinghua Univ., Beijing (China). State Key Lab. of Low-Dimensional Quantum Physics. Dept. of Physics; Collaborative Innovation Center of Quantum Matter, Beijing (China); SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences
  2. Collaborative Innovation Center of Quantum Matter, Beijing (China); SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source; Peking Univ., Beijing (China). International Center for Quantum Materials. School of Physics
  3. Tsinghua Univ., Beijing (China). State Key Lab. of Low-Dimensional Quantum Physics. Dept. of Physics
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source
  5. SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences
  6. SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource
  7. Tsinghua Univ., Beijing (China). State Key Lab. of Low-Dimensional Quantum Physics. Dept. of Physics; Collaborative Innovation Center of Quantum Matter, Beijing (China)
  8. SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences. Dept. of Physics and Applied Physics. Geballe Lab. for Advanced Materials
A single monolayer of iron selenide grown on strontium titanate shows an impressive enhancement of superconductivity compared with the bulk, as well as a novel Fermi surface topology, extreme two-dimensionality, and the possibility of phonon-enhanced electron pairing. For films thicker than one unit cell, however, the electronic structure is markedly different, with a drastically suppressed superconductivity and strong nematicity appearing. The physics driving this extraordinary dichotomy of superconducting behaviour is far from clear. In this paper, we use low-temperature scanning tunnelling microscopy to study multilayers of iron selenide grown by molecular beam epitaxy, and find a stripe-type charge ordering instability that develops beneath the nematic state. The charge ordering is visible and pinned in the vicinity of impurities. And as it emerges in the strong limit of nematicity, it suggests that a magnetic fluctuation with a rather small wavevector may be competing with the ordinary collinear antiferromagnetic ordering in multilayer films. Finally, the existence of stripes in iron-based superconductors, which resemble the stripe order in cuprates, not only suggests that electronic anisotropy and correlation are playing an important role, but also provides a platform for probing the complex interactions between nematicity, charge ordering, magnetism and superconductivity in high-temperature superconductors.
Research Organization:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States); Tsinghua Univ., Beijing (China)
Sponsoring Organization:
Ministry of Science and Technology of China; National Science Foundation (NSF) (United States); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
AC02-05CH11231; AC02-76SF00515
OSTI ID:
1425888
Alternate ID(s):
OSTI ID: 1437971
Journal Information:
Nature Physics, Journal Name: Nature Physics Journal Issue: 10 Vol. 13; ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)Copyright Statement
Country of Publication:
United States
Language:
English

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Cited By (12)

Discovery of a strain-stabilised smectic electronic order in LiFeAs text January 2018
Discovery of a strain-stabilised smectic electronic order in LiFeAs journal July 2018
Nematicity, magnetism and superconductivity in FeSe journal December 2017
Superconducting selenides intercalated with organic molecules: synthesis, crystal structure, electric and magnetic properties, superconducting properties, and phase separation in iron based-chalcogenides and hybrid organic-inorganic superconductors journal May 2018
Charge ordering in high-temperature superconductors visualized by scanning tunneling microscopy journal October 2019
Spectroscopic evidence of nematic fluctuations in LiFeAs journal July 2019
Study of intrinsic defect states of FeSe with scanning tunneling microscopy journal October 2019
Theoretical study of impurity-induced magnetism in FeSe journal January 2019
Antiferromagnetic Order in Epitaxial FeSe Films on SrTiO 3 journal February 2018
Orbital Origin of Extremely Anisotropic Superconducting Gap in Nematic Phase of FeSe Superconductor journal August 2018
Charge Density Wave and Spin Density Wave in Two-Orbital Model for Iron-Based Superconductors journal June 2018
Theoretical study of impurity-induced magnetism in FeSe text January 2018

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