Magnetostriction-polarization coupling in multiferroic Mn2MnWO6

Li, Man-Rong; McCabe, Emma E.; Stephens, Peter W.; Croft, Mark; Collins, Liam; Kalinin, Sergei V.; Deng, Zheng; Retuerto, Maria; Sen Gupta, Arnab; Padmanabhan, Haricharan; Gopalan, Venkatraman; Grams, Christoph P.; Hemberger, Joachim; Orlandi, Fabio; Manuel, Pascal; Li, Wen-Min; Jin, Chang-Qing; Walker, David; Greenblatt, Martha

doi:10.1038/s41467-017-02003-3

Title: Magnetostriction-polarization coupling in multiferroic Mn₂MnWO₆

Journal Article · Mon Dec 11 00:00:00 EST 2017 · Nature Communications

DOI:https://doi.org/10.1038/s41467-017-02003-3· OSTI ID:1422535

^[1];

^[2]; Stephens, Peter W. ^[3]; Croft, Mark ^[4];

^[5];

^[5]; Deng, Zheng ^[6];

^[6]; Sen Gupta, Arnab ^[7]; Padmanabhan, Haricharan ^[7]; Gopalan, Venkatraman ^[7];

^[8]; Hemberger, Joachim ^[8];

^[9]; Manuel, Pascal ^[9]; Li, Wen-Min ^[10]; Jin, Chang-Qing ^[10]; Walker, David ^[11]; Greenblatt, Martha ^[6]

Sun Yat-Sen Univ., Guangzhou, (China). Key Lab. of Bioinorganic and Synthetic Chemistry of Ministry of Education, School of Chemistry; Rutgers Univ., Piscataway, NJ (United States). Dept. of Chemistry and Chemical Biology
Univ. of Kent, Canterbury (United Kingdom). School of Physical Sciences
Stony Brook Univ., NY (United States). Dept. of Physics and Astronomy
Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics and Astronomy
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science (CNMS), Inst. for Functional Imaging of Materials
Rutgers Univ., Piscataway, NJ (United States). Dept. of Chemistry and Chemical Biology
Pennsylvania State Univ., University Park, PA (United States). Dept. of Material Sciences and Engineering
Univ. zu Koln (Germany). II Physikalisches Institut
Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Lab., ISIS Neutron Source
Chinese Academy of Sciences (CAS), Beijing (China). Inst. of Physics
Columbia Univ., Palisades, NY (United States). Lamont Doherty Earth Observatory

Double corundum-related polar magnets are promising materials for multiferroic and magnetoelectric applications in spintronics. However, their design and synthesis is a challenge, and magnetoelectric coupling has only been observed in Ni₃TeO₆ among the known double corundum compounds to date. Here in this paper we address the high-pressure synthesis of a new polar and antiferromagnetic corundum derivative Mn₂MnWO₆, which adopts the Ni₃TeO₆-type structure with low temperature first-order field-induced metamagnetic phase transitions (T_N = 58 K) and high spontaneous polarization (~ 63.3 μC·cm^-2). The magnetostriction-polarization coupling in Mn₂MnWO₆ is evidenced by second harmonic generation effect, and corroborated by magnetic-field-dependent pyroresponse behavior, which together with the magnetic-field-dependent polarization and dielectric measurements, qualitatively indicate magnetoelectric coupling. Finally, piezoresponse force microscopy imaging and spectroscopy studies on Mn₂MnWO₆ show switchable polarization, which motivates further exploration on magnetoelectric effect in single crystal/thin film specimens.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725; AC02-98CH10886; DMR-1507252; DMR-1420620

OSTI ID:: 1422535

Journal Information:: Nature Communications, Vol. 8, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 32 works

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Title: Magnetostriction-polarization coupling in multiferroic Mn2MnWO6

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Title: Magnetostriction-polarization coupling in multiferroic Mn₂MnWO₆