Carbon-Nanotube-Based Thermoelectric Materials and Devices

Blackburn, Jeffrey L.; Ferguson, Andrew J.; Cho, Chungyeon; Grunlan, Jaime C.

doi:10.1002/adma.201704386

Title: Carbon-Nanotube-Based Thermoelectric Materials and Devices

Journal Article · Mon Jan 22 00:00:00 EST 2018 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201704386· OSTI ID:1419418

Blackburn, Jeffrey L. ^[1]; Ferguson, Andrew J. ^[1]; Cho, Chungyeon ^[2]; Grunlan, Jaime C. ^[2]

National Renewable Energy Lab. (NREL), Golden, CO (United States)
Texas A & M Univ., College Station, TX (United States)

Abstract Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity‐generation sectors, and manufacturing processes. Thermal energy is also an abundant low‐flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off‐grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric‐energy‐harvesting devices. Carbon‐based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source‐materials, their amenability to high‐throughput solution‐phase fabrication routes, and the high specific energy (i.e., W g ⁻¹ ) enabled by their low mass. Single‐walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric‐energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube‐based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon‐nanotube‐based materials and composites have for producing high‐performance next‐generation devices for thermoelectric‐energy harvesting.

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), NREL Laboratory Directed Research and Development (LDRD)

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1419418

Alternate ID(s):: OSTI ID: 1417708

Report Number(s):: NREL/JA-5900-70041; TRN: US1801347

Journal Information:: Advanced Materials, Vol. 30, Issue 11; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 452 works

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The synergic regulation of conductivity and Seebeck coefficient in pure polyaniline by chemically changing the ordered degree of molecular chains Yao, Qin; Wang, Qun; Wang, Liming J. Mater. Chem. A, Vol. 2, Issue 8 https://doi.org/10.1039/C3TA14008C	journal	January 2014
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Thermoelectric power of a single-walled carbon nanotubes strand Kong, W. J.; Lu, L.; Zhu, H. W. Journal of Physics: Condensed Matter, Vol. 17, Issue 12 https://doi.org/10.1088/0953-8984/17/12/015	journal	March 2005
Segregated network polymer/carbon nanotubes composites Mierczynska, A.; Friedrich, J.; Maneck, H. Open Chemistry, Vol. 2, Issue 2 https://doi.org/10.2478/BF02475579	journal	June 2004
Charge Transport in Organic Semiconductors Coropceanu, Veaceslav; Cornil, Jerome; da Silva Filho, Demetrio A. ChemInform, Vol. 38, Issue 29 https://doi.org/10.1002/chin.200729266	journal	July 2007
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Thermoelectric Behavior of Segregated-Network Polymer Nanocomposites Yu, Choongho; Kim, Yeon Seok; Kim, Dasaroyong Nano Letters, Vol. 9, Issue 3 https://doi.org/10.1021/nl900263d	journal	March 2009
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