Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu2-xFexSi2

Kung, H.-H.; Ran, S.; Kanchanavatee, N.; Krapivin, V.; Lee, A.; Mydosh, J. A.; Haule, K.; Maple, M. B.; Blumberg, G.

doi:10.1103/PhysRevLett.117.227601

Title: Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in ${URu}_{2 - x} {Fe}_{x} {Si}_{2}$

Journal Article · Tue Nov 22 00:00:00 EST 2016 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.117.227601· OSTI ID:1418620

Kung, H.-H. ^[1]; Ran, S. ^[2]; Kanchanavatee, N. ^[2]; Krapivin, V. ^[1]; Lee, A. ^[1]; Mydosh, J. A. ^[3]; Haule, K. ^[1]; Maple, M. B. ^[2]; Blumberg, G. ^[4]

Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics & Astronomy
Univ. of California, San Diego, CA (United States). Dept. of Physics; Univ. of California, San Diego, CA (United States). Center for Advanced Nanoscience
Leiden Univ. (Netherlands). Kamerlingh Onnes Lab.
Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics & Astronomy; National Inst. of Chemical Physics and Biophysics,Tallinn (Estonia)

We study URu_2-xFe_xSi₂, in which two types of staggered phases compete at low temperature as the iron concentration x is varied: the nonmagnetic \hidden order" (HO) phase below the critical concentration x_c, and unconventional antiferromagnetic (AF) phase above x_c. By using polarization resolved Raman spectroscopy, we detect a collective mode of pseudovector-like A_{2_g} symmetry whose energy continuously evolves with increasing x; it monotonically decreases in the HO phase until it vanishes at x = x_c, and then reappears with increasing energy in the AF phase. The mode's evolution provides direct evidence for unified order parameter for both nonmagnetic and magnetic phases arising from the orbital degrees-of-freedom of the uranium-5f electrons.

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Research Organization:: Rutgers Univ., New Brunswick, NJ (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0005463; DMR-1104884; DMR-1405303; FG02-04ER46105; DMR-1206553

OSTI ID:: 1418620

Alternate ID(s):: OSTI ID: 1333315

Journal Information:: Physical Review Letters, Vol. 117, Issue 22; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 22 works

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Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂ Mydosh, J. A.; Oppeneer, P. M.; Riseborough, P. S. Journal of Physics: Condensed Matter, Vol. 32, Issue 14 https://doi.org/10.1088/1361-648x/ab5eba	journal	January 2020
Octupolar order in d-orbital Mott insulators Paramekanti, Arun; Maharaj, Dalini D.; Gaulin, Bruce D. arXiv https://doi.org/10.48550/arxiv.1909.03089	text	January 2019