Voltage Control of Two-Magnon Scattering and Induced Anomalous Magnetoelectric Coupling in Ni–Zn Ferrite

Xue, Xu; Dong, Guohua; Zhou, Ziyao; Xian, Dan; Hu, Zhongqiang; Ren, Wei; Ye, Zuo-Guang; Chen, Wei; Jiang, Zhuang-De; Liu, Ming

doi:10.1021/acsami.7b15433

Title: Voltage Control of Two-Magnon Scattering and Induced Anomalous Magnetoelectric Coupling in Ni–Zn Ferrite

Journal Article · Fri Dec 01 00:00:00 EST 2017 · ACS Applied Materials and Interfaces

DOI:https://doi.org/10.1021/acsami.7b15433· OSTI ID:1417022

Xue, Xu ^[1]; Dong, Guohua ^[1];

^[1]; Xian, Dan ^[2]; Hu, Zhongqiang ^[1]; Ren, Wei ^[3];

^[4];

^[5]; Jiang, Zhuang-De ^[2];

^[3]

Xi’an Jiaotong Univ., Shaanxi (China). Electronic Materials Research Lab., Key Lab. of the Ministry of Education & International Center for Dielectric Research
Xi’an Jiaotong Univ., Xi’an (China). Collaborative Innovation Center of High-End Manufacturing Equipment
Xi’an Jiaotong Univ., Shaanxi (China). Electronic Materials Research Lab., Key Lab. of the Ministry of Education & International Center for Dielectric Research; Xi’an Jiaotong Univ., Xi’an (China). Collaborative Innovation Center of High-End Manufacturing Equipment
Xi’an Jiaotong Univ., Shaanxi (China). Electronic Materials Research Lab., Key Lab. of the Ministry of Education & International Center for Dielectric Research; Simon Fraser Univ., Burnaby, BC (Canada). Dept. of Chemistry and 4D LABS
Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division

Controlling spin dynamics through modulation of spin interactions in a fast, compact, and energy-efficient way is compelling for its abundant physical phenomena and great application potential in next-generation voltage controllable spintronic devices. In this work, we report electric field manipulation of spin dynamics-the two-magnon scattering (TMS) effect in Ni_0.5Zn_0.5Fe₂O₄ (NZFO)/Pb(Mg_2/3Nb_1/3)-PbTiO₃ (PMN-PT) multiferroic heterostructures, which breaks the bottleneck of magnetostatic interaction-based magnetoelectric (ME) coupling in multiferroics. An alternative approach allowing spin-wave damping to be controlled by external electric field accompanied by a significant enhancement of the ME effect has been demonstrated. A two-way modulation of the TMS effect with a large magnetic anisotropy change up to 688 Oe has been obtained, referring to a 24 times ME effect enhancement at the TMS critical angle at room temperature. Furthermore, the anisotropic spin-freezing behaviors of NZFO were first determined via identifying the spatial magnetic anisotropy fluctuations. Finally, a large spin-freezing temperature change of 160 K induced by the external electric field was precisely determined by electron spin resonance.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: Natural Science Foundation of China (NNSFC); Fundamental Research Funds for the Central Universities; Natural Sciences and Engineering Research Council of Canada (NSERC); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division

Grant/Contract Number:: AC02-06CH11357; 51472199; 11534015; 51602244

OSTI ID:: 1417022

Journal Information:: ACS Applied Materials and Interfaces, Vol. 9, Issue 49; ISSN 1944-8244

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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Title: Voltage Control of Two-Magnon Scattering and Induced Anomalous Magnetoelectric Coupling in Ni–Zn Ferrite

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