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Voltage Control of Two-Magnon Scattering and Induced Anomalous Magnetoelectric Coupling in Ni–Zn Ferrite

Journal Article · · ACS Applied Materials and Interfaces
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  1. Xi’an Jiaotong Univ., Shaanxi (China). Electronic Materials Research Lab., Key Lab. of the Ministry of Education & International Center for Dielectric Research
  2. Xi’an Jiaotong Univ., Xi’an (China). Collaborative Innovation Center of High-End Manufacturing Equipment
  3. Xi’an Jiaotong Univ., Shaanxi (China). Electronic Materials Research Lab., Key Lab. of the Ministry of Education & International Center for Dielectric Research; Xi’an Jiaotong Univ., Xi’an (China). Collaborative Innovation Center of High-End Manufacturing Equipment
  4. Xi’an Jiaotong Univ., Shaanxi (China). Electronic Materials Research Lab., Key Lab. of the Ministry of Education & International Center for Dielectric Research; Simon Fraser Univ., Burnaby, BC (Canada). Dept. of Chemistry and 4D LABS
  5. Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
+ Show Author Affiliations
Controlling spin dynamics through modulation of spin interactions in a fast, compact, and energy-efficient way is compelling for its abundant physical phenomena and great application potential in next-generation voltage controllable spintronic devices. In this work, we report electric field manipulation of spin dynamics-the two-magnon scattering (TMS) effect in Ni0.5Zn0.5Fe2O4 (NZFO)/Pb(Mg2/3Nb1/3)-PbTiO3 (PMN-PT) multiferroic heterostructures, which breaks the bottleneck of magnetostatic interaction-based magnetoelectric (ME) coupling in multiferroics. An alternative approach allowing spin-wave damping to be controlled by external electric field accompanied by a significant enhancement of the ME effect has been demonstrated. A two-way modulation of the TMS effect with a large magnetic anisotropy change up to 688 Oe has been obtained, referring to a 24 times ME effect enhancement at the TMS critical angle at room temperature. Furthermore, the anisotropic spin-freezing behaviors of NZFO were first determined via identifying the spatial magnetic anisotropy fluctuations. Finally, a large spin-freezing temperature change of 160 K induced by the external electric field was precisely determined by electron spin resonance.
Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
Fundamental Research Funds for the Central Universities; Natural Science Foundation of China (NNSFC); Natural Sciences and Engineering Research Council of Canada (NSERC); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Scientific User Facilities Division
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1417022
Journal Information:
ACS Applied Materials and Interfaces, Journal Name: ACS Applied Materials and Interfaces Journal Issue: 49 Vol. 9; ISSN 1944-8244
Publisher:
American Chemical Society (ACS)Copyright Statement
Country of Publication:
United States
Language:
English

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Recent progress on flexible inorganic single-crystalline functional oxide films for advanced electronics journal January 2019
Voltage control of ferromagnetic resonance and spin waves journal September 2018

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Related Subjects

75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY
ferromagnetic resonance
magnetoelectric coupling
spin-lattice coupling
two-magnon scattering
voltage control of magnetism