0D-2D and 1D-2D Semiconductor Hybrids Composed of All Inorganic Perovskite Nanocrystals and Single-Layer Graphene with Improved Light Harvesting

Chen, Jia-Shiang; Doane, Tennyson L.; Li, Mingxing; Zang, Huidong; Maye, Mathew M.; Cotlet, Mircea

doi:10.1002/ppsc.201700310

Title: 0D-2D and 1D-2D Semiconductor Hybrids Composed of All Inorganic Perovskite Nanocrystals and Single-Layer Graphene with Improved Light Harvesting

Journal Article · Wed Dec 27 00:00:00 EST 2017 · Particle & Particle Systems Characterization

DOI:https://doi.org/10.1002/ppsc.201700310· OSTI ID:1414964

Chen, Jia-Shiang ^[1]; Doane, Tennyson L. ^[2]; Li, Mingxing ^[3]; Zang, Huidong ^[3]; Maye, Mathew M. ^[2];

^[3]

Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN); Stony Brook Univ., NY (United States). Dept. of Materials Science and Chemical Engineering
Syracuse Univ., NY (United States). Dept. of Chemistry
Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)

In this study, inorganic cesium lead iodide (CsPbI₃) perovskite nanoparticles (PNPs) and perovskite nanowires (PNWs) with single-layer graphene (SLG) are combined to obtain 0D–2D PNP–SLG and 1D–2D PNW–SLG hybrids with improved light harvesting. Time-resolved single-nanostructure photoluminescence studies of PNPs, PNWs, and related hybrids reveal (i) quasi-two-state photoluminescence blinking in PNPs, (ii) highly polarized photoluminescence emitted by PNWs and (iii) efficient interfacial electron transfer between perovskite nanostructures and SLG in both PNP–SLG and PNW–SLG hybrids. Thus, doping of poorly absorbing, highly conductive SLG with perovskite nanocrystals and nanowires provides a simple, yet efficient path to obtain hybrids with increased light-harvesting properties for potential utilization in the next-generation photodetectors and photovoltaic devices, including polarization sensitive photodetectors.

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Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704

OSTI ID:: 1414964

Journal Information:: Particle & Particle Systems Characterization, Journal Name: Particle & Particle Systems Characterization Vol. 35 Journal Issue: 2; ISSN 0934-0866

Publisher:: WileyCopyright Statement

Country of Publication:: Germany

Language:: English

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Cited by: 17 works

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