Far-IR magnetospectroscopy of magnons and electromagnons in TbFeO3 single crystals at low temperatures

Stanislavchuk, T. N.; Wang, Yazhong; Cheong, S. -W.; Sirenko, A. A.

doi:10.1103/PhysRevB.95.054427

Title: Far-IR magnetospectroscopy of magnons and electromagnons in $TbFe O_{3}$ single crystals at low temperatures

Journal Article · Wed Feb 01 00:00:00 EST 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.95.054427· OSTI ID:1409548

Stanislavchuk, T. N.; Wang, Yazhong; Cheong, S. -W.; Sirenko, A. A.

Transmittance spectra of TbFe O 3 single crystals have been studied in the far-infrared spectral range 15 - 120 c m - 1 in the external magnetic fields up to 9 T and at low temperatures down to 1.5 K. The temperature and magnetic-field dependencies of the antiferromagnetic resonance (AFMR) modes have been measured below and above the magnetic ordering temperature of Tb moments T Tb N = 3.3 K . Both the quasiferromagnetic and quasiantiferromagnetic modes of AFMR demonstrate hardening at T < T Tb N . The quasiantiferromagnetic mode gains electric-dipole activity along the c axis below T Tb N and thus behaves as a hybrid, i.e., both electric- and magnetic-dipole active, mode. In addition to AFMR modes, below T Tb N we observed the appearance of electromagnon excitation at about 27 c m - 1 , which is electric-dipole active along the c axis. The electromagnon is optically active only in a narrow temperature range, 2.7 K < T < T Tb N at H = 0 , and in a narrow range of magnetic fields 2.4–2.7 T applied along the b axis at T = 1.5 K . We argue that this electromagnon appears in magnetic phases, which are compatible with a spontaneous electric polarization along the b axis.

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Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

DOE Contract Number:: SC0012704

OSTI ID:: 1409548

Report Number(s):: BNL-114600-2017-JA¿¿¿; PRBMDO

Journal Information:: Physical Review B, Vol. 95, Issue 5; ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

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