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Title: Temperature and polarization dependence of low-energy magnetic fluctuations in nearly optimally doped NaFe 0.9785 Co 0.0215 As

Journal Article · · Physical Review B
 [1];  [1];  [1];  [2];  [3];  [3];  [4];  [5]; ORCiD logo [6];  [7];  [8]
  1. Rice Univ., Houston, TX (United States)
  2. Chinese Academy of Sciences (CAS), Beijing (China); Univ. of Chinese Academy of Sciences, Beijing (China)
  3. Beijing Normal Univ., Beijing (China)
  4. Forschungszentrum Julich GmbH, Garching (Germany)
  5. Univ. Grenoble Alpes, Grenoble (France)
  6. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  7. Chinese Academy of Sciences (CAS), Beijing (China); Univ. of Chinese Academy of Sciences, Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
  8. Rice Univ., Houston, TX (United States); Beijing Normal Univ., Beijing (China)

We use unpolarized and polarized neutron scattering to study the temperature and polarization dependence of low-energy magnetic fluctuations in nearly optimally doped NaFe0.9785Co0.0215As, with coexisting superconductivity (Tc ≈ 19 K) and weak antiferromagnetic order (TN ≈ 30 K, ordered moment ≈ 0.02μB/Fe). A single spin resonance mode with intensity tracking the superconducting order parameter is observed, although energy of the mode only softens slightly upon approaching Tc. Polarized neutron scattering reveals that the single resonance is mostly isotropic in spin space, similar to overdoped NaFe0.935Co0.045As but different from optimal electron-, hole-, and isovalently doped BaFe2As2 compounds, all featuring an additional prominent anisotropic component. Spin anisotropy in NaFe0.9785Co0.0215As is instead present at energies below the resonance, which becomes partially gapped below Tc, similar to the situation in optimally doped YBa2Cu3O6.9. Here, our results indicate that anisotropic spin fluctuations in NaFe1–xCoxAs appear in the form of a resonance in the underdoped regime, become partially gapped below Tc near optimal doping, and disappear in overdoped compounds.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
1409258
Journal Information:
Physical Review B, Vol. 96, Issue 18; ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English

References (58)

Distinguishing s ± and s + + electron pairing symmetries by neutron spin resonance in superconducting NaFe 0.935 Co 0.045 As journal August 2013
Weak-coupling superconductivity in a strongly correlated iron pnictide journal January 2016
Spin anisotropy due to spin-orbit coupling in optimally hole-doped Ba 0.67 K 0.33 Fe 2 As 2 journal December 2016
Resonance in the electron-doped high-transition-temperature superconductor Pr0.88LaCe0.12CuO4-δ journal July 2006
Itinerant Magnetic Excitations in Antiferromagnetic CaFe 2 As 2 journal May 2009
Prominent Role of Spin-Orbit Coupling in FeSe Revealed by Inelastic Neutron Scattering journal May 2017
Persistent high-energy spin excitations in iron-pnictide superconductors journal February 2013
Measurement of a Double Neutron-Spin Resonance and an Anisotropic Energy Gap for Underdoped Superconducting NaFe 0.985 Co 0.015 As Using Inelastic Neutron Scattering journal November 2013
Spin waves and magnetic exchange interactions in CaFe2As2 journal July 2009
Nature of magnetic excitations in superconducting BaFe1.9Ni0.1As2 journal March 2012
Electron doping evolution of structural and antiferromagnetic phase transitions in NaFe 1 x Co x As iron pnictides journal July 2016
Longitudinal Spin Excitations and Magnetic Anisotropy in Antiferromagnetically Ordered Ba Fe 2 As 2 journal December 2013
Splitting of Resonance Excitations in Nearly Optimally Doped Ba ( Fe 0.94 Co 0.06 ) 2 As 2 : An Inelastic Neutron Scattering Study with Polarization Analysis journal March 2013
Anisotropy of incommensurate magnetic excitations in slightly overdoped Ba 0.5 K 0.5 Fe 2 As 2 probed by polarized inelastic neutron scattering experiments journal September 2014
Doping dependence of spin excitations and its correlations with high-temperature superconductivity in iron pnictides journal December 2013
Transition from Three-Dimensional Anisotropic Spin Excitations to Two-Dimensional Spin Excitations by Electron Doping the FeAs-Based BaFe 1.96 Ni 0.04 As 2 Superconductor journal August 2009
Direct observation of spin–orbit coupling in iron-based superconductors journal December 2015
Effect of Pnictogen Height on Spin Waves in Iron Pnictides journal May 2014
Spin Resonance in the d -Wave Superconductor CeCoIn 5 journal February 2008
Symmetry of spin excitation spectra in the tetragonal paramagnetic and superconducting phases of 122-ferropnictides journal October 2010
Electron doping evolution of the neutron spin resonance in NaFe 1 x Co x As journal May 2016
Divergent Nematic Susceptibility in an Iron Arsenide Superconductor journal August 2012
Strong-coupling superconductivity in NaFe 1 x Co x As: Validity of Eliashberg theory journal April 2013
Spin anisotropy of the magnetic excitations in the normal and superconducting states of optimally doped YBa 2 Cu 3 O 6.9 studied by polarized neutron spectroscopy journal September 2011
Crossover from spin waves to diffusive spin excitations in underdoped Ba ( Fe 1 x Co x ) 2 As 2 journal May 2014
Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors journal May 2016
Normal-state spin dynamics and temperature-dependent spin-resonance energy in optimally doped BaFe1.85Co0.15As2 journal December 2009
Spin Excitation Anisotropy as a Probe of Orbital Ordering in the Paramagnetic Tetragonal Phase of Superconducting BaFe 1.904 Ni 0.096 As 2 journal September 2013
Magnonlike Dispersion of Spin Resonance in Ni-doped Ba Fe 2 As 2 journal April 2013
Antiferromagnetic order and spin dynamics in iron-based superconductors journal August 2015
Neutron Scattering Studies of spin excitations in hole-doped Ba0.67K0.33Fe2As2 superconductor journal October 2011
Polarized neutron scattering studies of magnetic excitations in electron-overdoped superconducting BaFe 1.85 Ni 0.15 As 2 journal June 2012
Unified Phase Diagram for Iron-Based Superconductors journal October 2017
Experimental elucidation of the origin of the ‘double spin resonances’ in Ba ( Fe 1 x Co x ) 2 As 2 journal May 2016
Itinerant spin excitations in SrFe 2 As 2 measured by inelastic neutron scattering journal June 2011
Spin-Orbit Interactions and the Nematicity Observed in the Fe-Based Superconductors journal April 2015
Fermi surface nesting induced strong pairing in iron-based superconductors journal April 2009
Magnetic anisotropy in hole-doped superconducting Ba 0.67 K 0.33 Fe 2 As 2 probed by polarized inelastic neutron scattering journal February 2013
Environmental stability and anisotropic resistivity of Co-doped Na 1 δ Fe 1 x Co x As journal October 2012
Temperature dependence of the resonance and low-energy spin excitations in superconducting FeTe 0.6 Se 0.4 journal February 2012
In-plane spin excitation anisotropy in the paramagnetic state of NaFeAs journal October 2013
Robust upward dispersion of the neutron spin resonance in the heavy fermion superconductor Ce1−xYbxCoIn5 journal September 2016
Anisotropic resonance modes emerging in an antiferromagnetic superconducting state journal September 2017
Spin excitation anisotropy in the paramagnetic tetragonal phase of BaFe 2 As 2 journal July 2017
Structural and magnetic phase transitions in Na 1 δ FeAs journal July 2009
Electron doping evolution of the magnetic excitations in NaFe 1 x Co x As journal June 2016
Local magnetic anisotropy in BaFe 2 As 2 : A polarized inelastic neutron scattering study journal August 2012
Suppression of spin-exciton state in hole overdoped iron-based superconductors journal March 2016
Transition from Sign-Reversed to Sign-Preserved Cooper-Pairing Symmetry in Sulfur-Doped Iron Selenide Superconductors journal May 2016
Anisotropic neutron spin resonance in underdoped superconducting NaFe 1 x Co x As journal October 2014
Crossover from weak to strong pairing in unconventional superconductors journal June 2011
Nematic spin fluid in the tetragonal phase of BaFe 2 As 2 journal August 2011
A universal relationship between magnetic resonance and superconducting gap in unconventional superconductors journal October 2009
Polarized and unpolarized neutron-scattering study of the dynamical spin susceptibility of Y Ba 2 Cu 3 O 7 journal September 1996
Spin fluctuations in iron pnictides and chalcogenides: From antiferromagnetism to superconductivity journal January 2016
Nematic Quantum Critical Fluctuations in BaFe 2 x Ni x As 2 journal October 2016
Electron-doping evolution of the low-energy spin excitations in the iron arsenide superconductor BaFe 2 x Ni x As 2 journal May 2010
A common thread: The pairing interaction for unconventional superconductors journal October 2012

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