Frustrated ground state in the metallic Ising antiferromagnet Nd2Ni2In

Sala, G.; Mašková, S.; Stone, M. B.

doi:10.1103/PhysRevMaterials.1.054404

Frustrated ground state in the metallic Ising antiferromagnet ${Nd}_{2} {Ni}_{2} In$

Journal Article · Sun Oct 01 04:00:00 EDT 2017 · Physical Review Materials

DOI:https://doi.org/10.1103/PhysRevMaterials.1.054404· OSTI ID:1400165

Sala, G.; Mašková, S.; Stone, M. B.

We use inelastic neutron scattering measurements to examine the inter-metallic Ising anti-ferromagnet \NNI. The dynamical structure factor displays a spectrum with multiple crystal field excitations. These crystal field excitations consist of a set of four transitions covering a range of energies between $$4$$ and $80$ meV. The analysis of the crystalline electric field scheme confirms the Ising nature of the spins and their orientation as proposed by previous studies. We characterize \NNI~as a large moment intermetallic antiferromagnet with the potential to support a geometrically frustrated Shastry-Sutherland lattice.

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

DOE Contract Number:: AC05-00OR22725

OSTI ID:: 1400165

Journal Information:: Physical Review Materials, Journal Name: Physical Review Materials Journal Issue: 5 Vol. 1; ISSN PRMHAR; ISSN 2475-9953

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

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Frustrated ground state in the metallic Ising antiferromagnet ${Nd}_{2} {Ni}_{2} In$