Anion exchange membrane fuel cells: Current status and remaining challenges

Gottesfeld, Shimshon; Dekel, Dario R.; Page, Miles; Bae, Chulsung; Yan, Yushan; Zelenay, Piotr; Kim, Yu Seung

doi:10.1016/j.jpowsour.2017.08.010

Title: Anion exchange membrane fuel cells: Current status and remaining challenges

Journal Article · Fri Sep 01 00:00:00 EDT 2017 · Journal of Power Sources

DOI:https://doi.org/10.1016/j.jpowsour.2017.08.010· OSTI ID:1400127

Gottesfeld, Shimshon ^[1]; Dekel, Dario R. ^[2]; Page, Miles ^[3]; Bae, Chulsung ^[4]; Yan, Yushan ^[5]; Zelenay, Piotr ^[6];

^[6]

Univ. of Delaware, Newark, DE (United States). Fuel Cell Consulting Ltd., Dept. of Chemical & Biomolecular Engineering
Israel Inst. of Technology, Haifa (Israel). The Wolfson Dept. of Chemical Engineering, Nancy & Stephan Grand Technion Energy Program (GTEP)
PO-Cell Tech Ltd., Caesarea (Israel)
Rensselaer Polytechnic Inst., Troy, NY (United States). Dept. of Chemistry & Chemical Biology
Univ. of Delaware, Newark, DE (United States). Dept. of Chemical & Biomolecular Engineering
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

The anion exchange membrane fuel cell (AEMFC) is an attractive alternative to acidic proton exchange membrane fuel cells, which to date have required platinum-based catalysts, as well as acid-tolerant stack hardware. The AEMFC could use non-platinum-group metal catalysts and less expensive metal hardware thanks to the high pH of the electrolyte. Over the last decade, substantial progress has been made in improving the performance and durability of the AEMFC through the development of new materials and the optimization of system design and operation conditions. Here in this perspective article, we describe the current status of AEMFCs as having reached beginning of life performance very close to that of PEMFCs when using ultra-low loadings of Pt, while advancing towards operation on non-platinum-group metal catalysts alone. In the latter sections, we identify the remaining technical challenges, which require further research and development, focusing on the materials and operational factors that critically impact AEMFC performance and/or durability. Finally, these perspectives may provide useful insights for the development of next-generation of AEMFCs.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: AC52-06NA25396; 284522

OSTI ID:: 1400127

Alternate ID(s):: OSTI ID: 1549219

Report Number(s):: LA-UR-17-21918; TRN: US1703100

Journal Information:: Journal of Power Sources, Vol. 375; ISSN 0378-7753

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 578 works

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In-depth understanding of the CO ₂ limitation of air fed anion exchange membrane fuel cells Divekar, Ashutosh G.; Yang-Neyerlin, Ami C.; Antunes, Christopher M. Sustainable Energy & Fuels, Vol. 4, Issue 4 https://doi.org/10.1039/c9se01212e	journal	January 2020
Highly Conductive and Water-Swelling Resistant Anion Exchange Membrane for Alkaline Fuel Cells Ge, Qianqian; Zhu, Xiang; Yang, Zhengjin International Journal of Molecular Sciences, Vol. 20, Issue 14 https://doi.org/10.3390/ijms20143470	journal	July 2019
Enhancement of Palladium HOR Activity in Alkaline Conditions through Ceria Surface Doping Yarmiayev, Valeria; Alesker, Maria; Muzikansky, Anya Journal of The Electrochemical Society, Vol. 166, Issue 7 https://doi.org/10.1149/2.0291907jes	journal	January 2019
Transition Metal–Nitrogen–Carbon (M–N–C) Catalysts for Oxygen Reduction Reaction. Insights on Synthesis and Performance in Polymer Electrolyte Fuel Cells Osmieri, Luigi ChemEngineering, Vol. 3, Issue 1 https://doi.org/10.3390/chemengineering3010016	journal	February 2019
Nanocellulose-based materials as components of polymer electrolyte fuel cells Vilela, Carla; Silvestre, Armando J. D.; Figueiredo, Filipe M. L. Journal of Materials Chemistry A, Vol. 7, Issue 35 https://doi.org/10.1039/c9ta07466j	journal	January 2019
Highly conductive and chemically stable alkaline anion exchange membranes via ROMP of trans -cyclooctene derivatives You, Wei; Padgett, Elliot; MacMillan, Samantha N. Proceedings of the National Academy of Sciences, Vol. 116, Issue 20 https://doi.org/10.1073/pnas.1900988116	journal	April 2019
Platinum and Platinum Group Metal-Free Catalysts for Anion Exchange Membrane Fuel Cells Men Truong, Van; Richard Tolchard, Julian; Svendby, Jørgen Energies, Vol. 13, Issue 3 https://doi.org/10.3390/en13030582	journal	January 2020
Poly(vinyl benzyl methylpyrrolidinium) hydroxide derived anion exchange membranes for water electrolysis Li, Huanhuan; Kraglund, Mikkel Rykær; Reumert, Alexander Kappel Journal of Materials Chemistry A, Vol. 7, Issue 30 https://doi.org/10.1039/c9ta04868e	journal	January 2019
The Comparability of Pt to Pt-Ru in Catalyzing the Hydrogen Oxidation Reaction for Alkaline Polymer Electrolyte Fuel Cells Operated at 80 °C Li, Qihao; Peng, Hanqing; Wang, Yingming Angewandte Chemie International Edition, Vol. 58, Issue 5 https://doi.org/10.1002/anie.201812662	journal	January 2019
Imidazolium‐Functionalized Fluorene‐Based Anion Exchange Membrane (AEM) for Fuel Cell Applications Salma, Umme; Zhang, Dishen; Nagao, Yuki ChemistrySelect, Vol. 5, Issue 4 https://doi.org/10.1002/slct.201903246	journal	January 2020
Prospects for Anion-Exchange Membranes in Alkali Metal–Air Batteries Tsehaye, Misgina Tilahun; Alloin, Fannie; Iojoiu, Cristina Energies, Vol. 12, Issue 24 https://doi.org/10.3390/en12244702	journal	December 2019
Electrospun Ionomeric Fibers with Anion Conducting Properties Mann‐Lahav, Meirav; Halabi, Manar; Shter, Gennady E. Advanced Functional Materials, Vol. 30, Issue 18 https://doi.org/10.1002/adfm.201901733	journal	April 2019
Intermediate temperature fuel cells via an ion-pair coordinated polymer electrolyte Lee, Kwan-Soo; Maurya, Sandip; Kim, Yu Seung Energy & Environmental Science, Vol. 11, Issue 4 https://doi.org/10.1039/c7ee03595k	journal	January 2018
Quantifying and elucidating the effect of CO ₂ on the thermodynamics, kinetics and charge transport of AEMFCs Zheng, Yiwei; Omasta, Travis J.; Peng, Xiong Energy & Environmental Science, Vol. 12, Issue 9 https://doi.org/10.1039/c9ee01334b	journal	January 2019
Ni ₃ N as an Active Hydrogen Oxidation Reaction Catalyst in Alkaline Medium Ni, Weiyan; Krammer, Anna; Hsu, Chia‐Shuo Angewandte Chemie International Edition, Vol. 58, Issue 22 https://doi.org/10.1002/anie.201902751	journal	May 2019
The Effect of Ambient Carbon Dioxide on Anion-Exchange Membrane Fuel Cells Ziv, Noga; Mustain, William E.; Dekel, Dario R. ChemSusChem, Vol. 11, Issue 7 https://doi.org/10.1002/cssc.201702330	journal	March 2018
Alkali-stable partially fluorinated poly(arylene ether) anion exchange membranes with a claw-type head for fuel cells Wang, Xiu Qin; Lin, Chen Xiao; Liu, Fang Hua Journal of Materials Chemistry A, Vol. 6, Issue 26 https://doi.org/10.1039/c8ta03437k	journal	January 2018
Chemical stability of poly(phenylene oxide)-based ionomers in an anion exchange-membrane fuel cell environment Willdorf-Cohen, Sapir; Mondal, Abhishek N.; Dekel, Dario R. Journal of Materials Chemistry A, Vol. 6, Issue 44 https://doi.org/10.1039/c8ta05785k	journal	January 2018
Composite Poly(norbornene) Anion Conducting Membranes for Achieving Durability, Water Management and High Power (3.4 W/cm ² ) in Hydrogen/Oxygen Alkaline Fuel Cells Huang, Garrett; Mandal, Mrinmay; Peng, Xiong Journal of The Electrochemical Society, Vol. 166, Issue 10 https://doi.org/10.1149/2.1301910jes	journal	January 2019
Relating alkaline stability to the structure of quaternary phosphonium cations Zhang, Bingzi; Long, Hai; Kaspar, Robert B. RSC Advances, Vol. 8, Issue 47 https://doi.org/10.1039/c8ra03440k	journal	January 2018
Ether-free polyfluorenes tethered with quinuclidinium cations as hydroxide exchange membranes Allushi, Andrit; Pham, Thanh Huong; Olsson, Joel S. Journal of Materials Chemistry A, Vol. 7, Issue 47 https://doi.org/10.1039/c9ta09213g	journal	January 2019
A review of the synthesis and characterization of anion exchange membranes Hagesteijn, Kimberly F. L.; Jiang, Shanxue; Ladewig, Bradley P. Journal of Materials Science, Vol. 53, Issue 16 https://doi.org/10.1007/s10853-018-2409-y	journal	May 2018
How does a small structural change of anode ionomer make a big difference in alkaline membrane fuel cell performance? Park, Eun Joo; Maurya, Sandip; Lee, Albert S. Journal of Materials Chemistry A, Vol. 7, Issue 43 https://doi.org/10.1039/c9ta10157h	journal	January 2019
Quaternized aryl ether-free polyaromatics for alkaline membrane fuel cells: synthesis, properties, and performance – a topical review Park, Eun Joo; Kim, Yu Seung Journal of Materials Chemistry A, Vol. 6, Issue 32 https://doi.org/10.1039/c8ta05428b	journal	January 2018
Predicting the Effects of Carbon Dioxide on the Conductivity of Electrospun Anion Exchange Membranes Wrubel, Jacob A.; Peracchio, Aldo A.; Cassenti, Brice N. Journal of The Electrochemical Society, Vol. 166, Issue 14 https://doi.org/10.1149/2.0481914jes	journal	January 2019
Poly(bis-arylimidazoliums) possessing high hydroxide ion exchange capacity and high alkaline stability Fan, Jiantao; Willdorf-Cohen, Sapir; Schibli, Eric M. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10292-z	journal	May 2019
Anion exchange membranes with branched ionic clusters for fuel cells He, Yubin; Ge, Xiaolin; Liang, Xian Journal of Materials Chemistry A, Vol. 6, Issue 14 https://doi.org/10.1039/c8ta01114a	journal	January 2018
Interfacing nickel nitride and nickel boosts both electrocatalytic hydrogen evolution and oxidation reactions Song, Fuzhan; Li, Wei; Yang, Jiaqi Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-06728-7	journal	October 2018
Electrocatalysis of oxygen reduction on heteroatom-doped nanocarbons and transition metal–nitrogen–carbon catalysts for alkaline membrane fuel cells Sarapuu, Ave; Kibena-Põldsepp, Elo; Borghei, Maryam Journal of Materials Chemistry A, Vol. 6, Issue 3 https://doi.org/10.1039/c7ta08690c	journal	January 2018
ETFE-based anion-exchange membrane ionomer powders for alkaline membrane fuel cells: a first performance comparison of head-group chemistry Gonçalves Biancolli, Ana Laura; Herranz, Daniel; Wang, Lianqin Journal of Materials Chemistry A, Vol. 6, Issue 47 https://doi.org/10.1039/c8ta08309f	journal	January 2018
Oxygen Reduction Reaction Activity of Mesostructured Cobalt‐Based Metal Oxides Studied with the Cavity‐Microelectrode Technique Behnken, Julian; Yu, Mingquan; Deng, Xiaohui ChemElectroChem, Vol. 6, Issue 13 https://doi.org/10.1002/celc.201900722	journal	July 2019
A Review on Fuel Cell-Based Locomotive Powering Options for Sustainable Transportation Siddiqui, Osamah; Dincer, Ibrahim Arabian Journal for Science and Engineering, Vol. 44, Issue 2 https://doi.org/10.1007/s13369-018-3607-2	journal	October 2018
Strategies for Reducing the PGM Loading in High Power AEMFC Anodes Omasta, Travis J.; Zhang, Yufeng; Park, Andrew Michael ECS Transactions, Vol. 85, Issue 13 https://doi.org/10.1149/08513.0873ecst	journal	June 2018
Structurally Well-Defined Anion-Exchange Membranes Containing Perfluoroalkyl and Ammonium-Functionalized Fluorenyl Groups Ozawa, Mizuki; Kimura, Taro; Otsuji, Kanji ACS Omega, Vol. 3, Issue 11 https://doi.org/10.1021/acsomega.8b02742	journal	November 2018
Quaternized cellulose and graphene oxide crosslinked polyphenylene oxide based anion exchange membrane Das, Gautam; Park, Bang Ju; Kim, Jihyeon Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-45947-w	journal	July 2019
Novel Heteroatom-Doped Fe/N/C Electrocatalysts With Superior Activities for Oxygen Reduction Reaction in Both Acid and Alkaline Solutions Rauf, Muhammad; Wang, Jingwen; Iqbal, Waheed Frontiers in Chemistry, Vol. 8 https://doi.org/10.3389/fchem.2020.00078	journal	February 2020
Ionizing Radiation for Preparation and Functionalization of Membranes and Their Biomedical and Environmental Applications Membranes, Vol. 9, Issue 12 https://doi.org/10.3390/membranes9120163	journal	December 2019

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