Two-dimensional heterostructures for energy storage

Gogotsi, Yury G.; Pomerantseva, Ekaterina

doi:10.1038/nenergy.2017.89

Two-dimensional heterostructures for energy storage

Journal Article · Mon Jun 12 00:00:00 EDT 2017 · Nature Energy

DOI:https://doi.org/10.1038/nenergy.2017.89· OSTI ID:1399223

Gogotsi, Yury G. ^[1]; Pomerantseva, Ekaterina ^[1]

Drexel Univ., Philadelphia, PA (United States)

Two-dimensional (2D) materials provide slit-shaped ion diffusion channels that enable fast movement of lithium and other ions. However, electronic conductivity, the number of intercalation sites, and stability during extended cycling are also crucial for building high-performance energy storage devices. While individual 2D materials, such as graphene, show some of the required properties, none of them can offer all properties needed to maximize energy density, power density, and cycle life. Here we argue that stacking different 2D materials into heterostructured architectures opens an opportunity to construct electrodes that would combine the advantages of the individual building blocks while eliminating the associated shortcomings. We discuss characteristics of common 2D materials and provide examples of 2D heterostructured electrodes that showed new phenomena leading to superior electrochemical performance. As a result, we also consider electrode fabrication approaches and finally outline future steps to create 2D heterostructured electrodes that could greatly expand current energy storage technologies.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1399223

Alternate ID(s):: OSTI ID: 1388915

Journal Information:: Nature Energy, Journal Name: Nature Energy Journal Issue: 7 Vol. 2

Country of Publication:: United States

Language:: English

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2D Titania–Carbon Superlattices Vertically Encapsulated in 3D Hollow Carbon Nanospheres Embedded with 0D TiO ₂ Quantum Dots for Exceptional Sodium‐Ion Storage Xia, Qingbing; Lin, Zeheng; Lai, Weihong Angewandte Chemie International Edition, Vol. 58, Issue 40 https://doi.org/10.1002/anie.201907189	journal	August 2019
Functional MXene Materials: Progress of Their Applications Li, Xiuqin; Wang, Chengyin; Cao, Yu Chemistry - An Asian Journal, Vol. 13, Issue 19 https://doi.org/10.1002/asia.201800543	journal	August 2018
2D Titanium Carbide/Reduced Graphene Oxide Heterostructures for Supercapacitor Applications Navarro-Suárez, Adriana M.; Maleski, Kathleen; Makaryan, Taron Batteries & Supercaps, Vol. 1, Issue 1 https://doi.org/10.1002/batt.201800014	journal	April 2018
Enhanced Lithium Storage Performance of Liquid-Phase Exfoliated Graphene Supported WS ₂ Heterojunctions Li, Jianhui; Yan, Haiting; Wei, Wei ChemElectroChem, Vol. 5, Issue 21 https://doi.org/10.1002/celc.201800926	journal	August 2018
Chemical Mass Production of MoS 2 /Graphene van der Waals Heterostructure as a High‐Performance Li‐ion Intercalation Host Gong, Shan; Zhao, Guangyu; Zhang, Naiqing ChemElectroChem, Vol. 6, Issue 13 https://doi.org/10.1002/celc.201900783	journal	July 2019
“All‐In‐One” integrated ultrathin SnS ₂ @3D multichannel carbon matrix power high‐areal–capacity lithium battery anode Xu, Hongyi; Peng, Chengxin; Yan, Yuhua Carbon Energy, Vol. 1, Issue 2 https://doi.org/10.1002/cey2.22	journal	October 2019
Thermally Reduced Graphene/MXene Film for Enhanced Li‐ion Storage Xu, Shuaikai; Dall'Agnese, Yohan; Li, Junzhi Chemistry – A European Journal, Vol. 24, Issue 69 https://doi.org/10.1002/chem.201805162	journal	June 2018
Few‐Layer MoS ₂ Nanosheets Encapsulated in N‐Doped Carbon Hollow Spheres as Long‐Life Anode Materials for Lithium‐Ion Batteries Wang, Faze; Li, Fanggang; Ma, Li Chemistry – A European Journal, Vol. 25, Issue 64 https://doi.org/10.1002/chem.201902624	journal	October 2019
Hierarchical Porous NiO/β-NiMoO ₄ Heterostructure as Superior Anode Material for Lithium Storage Wang, Zhijian; Zhang, Shilin; Zeng, Hai ChemPlusChem, Vol. 83, Issue 10 https://doi.org/10.1002/cplu.201800220	journal	July 2018
Niobium carbide/reduced graphene oxide hybrid porous aerogel as high capacity and long‐life anode material for Li‐ion batteries Butt, Rehman; Siddique, Ahmad Hassan; Bokhari, Syeda Wishal International Journal of Energy Research, Vol. 43, Issue 9 https://doi.org/10.1002/er.4598	journal	May 2019
Recent Advances in Layered Ti ₃ C ₂ T _x MXene for Electrochemical Energy Storage Xiong, Dongbin; Li, Xifei; Bai, Zhimin Small, Vol. 14, Issue 17 https://doi.org/10.1002/smll.201703419	journal	February 2018
Fabrication of a 3D Hierarchical Sandwich Co ₉ S ₈ /α-MnS@N-C@MoS ₂ Nanowire Architectures as Advanced Electrode Material for High Performance Hybrid Supercapacitors Kandula, Syam; Shrestha, Khem Raj; Kim, Nam Hoon Small, Vol. 14, Issue 23 https://doi.org/10.1002/smll.201800291	journal	May 2018
Charge Transfer Salt and Graphene Heterostructure‐Based Micro‐Supercapacitors with Alternating Current Line‐Filtering Performance Zhao, Doudou; Chang, Wei; Lu, Chenbao Small, Vol. 15, Issue 48 https://doi.org/10.1002/smll.201901494	journal	May 2019
Interplay between Short- and Long-Ranged Forces Leading to the Formation of Ag Nanoparticle Superlattice Lee, Jaewon; Nakouzi, Elias; Xiao, Dongdong Small, Vol. 15, Issue 33 https://doi.org/10.1002/smll.201901966	journal	June 2019
Functional 2D Germanene Fluorescent Coating of Microrobots for Micromachines Multiplexing Maric, Tijana; Beladi‐Mousavi, Seyyed Mohsen; Khezri, Bahareh Small, Vol. 16, Issue 27 https://doi.org/10.1002/smll.201902365	journal	August 2019
N‐Doped Carbon Nanofibers with Interweaved Nanochannels for High‐Performance Sodium‐Ion Storage Zhao, Wenxiang; Hu, Xiang; Ci, Suqin Small, Vol. 15, Issue 46 https://doi.org/10.1002/smll.201904054	journal	September 2019
Confined Pyrolysis of ZIF‐8 Polyhedrons Wrapped with Graphene Oxide Nanosheets to Prepare 3D Porous Carbon Heterostructures Ding, Bing; Fan, Zengjie; Lin, Qingyang Small Methods, Vol. 3, Issue 11 https://doi.org/10.1002/smtd.201900277	journal	May 2019
Review of MXenes as new nanomaterials for energy storage/delivery and selected environmental applications Jun, Byung-Moon; Kim, Sewoon; Heo, Jiyong Nano Research, Vol. 12, Issue 3 https://doi.org/10.1007/s12274-018-2225-3	journal	October 2018
Two-dimensional SnO2/graphene heterostructures for highly reversible electrochemical lithium storage Zhu, Youqi; Cao, Tai; Li, Zhi Science China Materials, Vol. 61, Issue 12 https://doi.org/10.1007/s40843-018-9324-0	journal	August 2018
Layer-by-layer self-assembly of pillared two-dimensional multilayers Tian, Weiqian; VahidMohammadi, Armin; Wang, Zhen Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10631-0	journal	June 2019
Heterointerface effects in the electrointercalation of van der Waals heterostructures Bediako, D. Kwabena; Rezaee, Mehdi; Yoo, Hyobin Nature, Vol. 558, Issue 7710 https://doi.org/10.1038/s41586-018-0205-0	journal	June 2018
Emerging nanofabrication and quantum confinement techniques for 2D materials beyond graphene Stanford, Michael G.; Rack, Philip D.; Jariwala, Deep npj 2D Materials and Applications, Vol. 2, Issue 1 https://doi.org/10.1038/s41699-018-0065-3	journal	July 2018
One-step synthesis of 2D-layered carbon wrapped transition metal nitrides from transition metal carbides (MXenes) for supercapacitors with ultrahigh cycling stability Yuan, Wenyu; Cheng, Laifei; Wu, Heng Chemical Communications, Vol. 54, Issue 22 https://doi.org/10.1039/c7cc09017j	journal	January 2018
Dwindling the re-stacking by simultaneous exfoliation of boron nitride and decoration of α-Fe ₂ O ₃ nanoparticles using a solvothermal route Thangasamy, Pitchai; Sathish, Marappan New Journal of Chemistry, Vol. 42, Issue 7 https://doi.org/10.1039/c7nj04325b	journal	January 2018
Recent advances in the nanoengineering of electrocatalysts for CO ₂ reduction Li, Fengwang; MacFarlane, Douglas R.; Zhang, Jie Nanoscale, Vol. 10, Issue 14 https://doi.org/10.1039/c7nr09620h	journal	January 2018
MXenes/graphene heterostructures for Li battery applications: a first principles study Aierken, Yierpan; Sevik, Cem; Gülseren, Oğuz Journal of Materials Chemistry A, Vol. 6, Issue 5 https://doi.org/10.1039/c7ta09001c	journal	January 2018
Graphene-coupled Ti ₃ C ₂ MXenes-derived TiO ₂ mesostructure: promising sodium-ion capacitor anode with fast ion storage and long-term cycling Wang, Rutao; Wang, Shijie; Zhang, Yabin Journal of Materials Chemistry A, Vol. 6, Issue 3 https://doi.org/10.1039/c7ta09153b	journal	January 2018
Two-dimensional nanostructures for sodium-ion battery anodes Mao, Jianfeng; Zhou, Tengfei; Zheng, Yang Journal of Materials Chemistry A, Vol. 6, Issue 8 https://doi.org/10.1039/c7ta10500b	journal	January 2018
Improved capacity of redox-active functional carbon cathodes by dimension reduction for hybrid supercapacitors Liu, Tianyuan; Lee, Byeongyong; Lee, Michael J. Journal of Materials Chemistry A, Vol. 6, Issue 8 https://doi.org/10.1039/c7ta10881h	journal	January 2018
Transition-metal dichalcogenides/Mg(OH) ₂ van der Waals heterostructures as promising water-splitting photocatalysts: a first-principles study Luo, Yi; Wang, Sake; Ren, Kai Physical Chemistry Chemical Physics, Vol. 21, Issue 4 https://doi.org/10.1039/c8cp06960c	journal	January 2019
Using van der Waals heterostructures based on two-dimensional blue phosphorus and XC (X = Ge, Si) for water-splitting photocatalysis: a first-principles study Ren, Kai; Ren, Chongdan; Luo, Yi Physical Chemistry Chemical Physics, Vol. 21, Issue 19 https://doi.org/10.1039/c8cp07680d	journal	January 2019
Applications of 2D MXenes in energy conversion and storage systems Pang, Jinbo; Mendes, Rafael G.; Bachmatiuk, Alicja Chemical Society Reviews, Vol. 48, Issue 1 https://doi.org/10.1039/c8cs00324f	journal	January 2019
2D-Pnictogens: alloy-based anode battery materials with ultrahigh cycling stability Beladi-Mousavi, Seyyed Mohsen; Pumera, Martin Chemical Society Reviews, Vol. 47, Issue 18 https://doi.org/10.1039/c8cs00425k	journal	January 2018
Heterostructure of two different 2D materials based on MoS ₂ nanoflowers@rGO: an electrode material for sodium-ion capacitors Ramakrishnan, Kiruthiga; Nithya, Chandrasekaran; Karvembu, Ramasamy Nanoscale Advances, Vol. 1, Issue 1 https://doi.org/10.1039/c8na00104a	journal	January 2019
Solvent mediated hybrid 2D materials: black phosphorus – graphene heterostructured building blocks assembled for sodium ion batteries Li, Mengya; Muralidharan, Nitin; Moyer, Kathleen Nanoscale, Vol. 10, Issue 22 https://doi.org/10.1039/c8nr01400k	journal	January 2018
Construction of 3D architectures with Ni(HCO ₃ ) ₂ nanocubes wrapped by reduced graphene oxide for LIBs: ultrahigh capacity, ultrafast rate capability and ultralong cycle stability Dong, Yutao; Ma, Yuhang; Li, Dan Chemical Science, Vol. 9, Issue 46 https://doi.org/10.1039/c8sc02868k	journal	January 2018
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Graphene-supported 2D transition metal oxide heterostructures Azadmanjiri, Jalal; Srivastava, Vijay K.; Kumar, Parshant Journal of Materials Chemistry A, Vol. 6, Issue 28 https://doi.org/10.1039/c8ta03404d	journal	January 2018
Recent advances in the preparation, characterization, and applications of two-dimensional heterostructures for energy storage and conversion Das, Pratteek; Fu, Qiang; Bao, Xinhe Journal of Materials Chemistry A, Vol. 6, Issue 44 https://doi.org/10.1039/c8ta04618b	journal	January 2018
Robust heterostructures of a bimetallic sodium–zinc metal–organic framework and reduced graphene oxide for high-performance supercapacitors Rajak, Richa; Saraf, Mohit; Mobin, Shaikh M. Journal of Materials Chemistry A, Vol. 7, Issue 4 https://doi.org/10.1039/c8ta09528k	journal	January 2019
Strain-engineered BlueP–MoS ₂ van der Waals heterostructure with improved lithiation/sodiation for LIBs and SIBs Barik, Gayatree; Pal, Sourav Physical Chemistry Chemical Physics, Vol. 22, Issue 3 https://doi.org/10.1039/c9cp04349g	journal	January 2020
Graphitic carbon nitride decorated with FeNi ₃ nanoparticles for flexible planar micro-supercapacitor with ultrahigh energy density and quantum storage capacity Talukdar, Meenakshi; Behera, Sushant Kumar; Deb, Pritam Dalton Transactions, Vol. 48, Issue 32 https://doi.org/10.1039/c9dt02423a	journal	January 2019
Rational design of two-dimensional nanomaterials for lithium–sulfur batteries Jana, Milan; Xu, Rui; Cheng, Xin-Bing Energy & Environmental Science, Vol. 13, Issue 4 https://doi.org/10.1039/c9ee02049g	journal	January 2020
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Energy storage: pseudocapacitance in prospect Costentin, Cyrille; Savéant, Jean-Michel Chemical Science, Vol. 10, Issue 22 https://doi.org/10.1039/c9sc01662g	journal	January 2019
Ultrafast Li-ion migration in holey-graphene-based composites constructed by a generalized ex situ method towards high capacity energy storage Zhu, Chengling; Hui, Zeyu; Pan, Hui Journal of Materials Chemistry A, Vol. 7, Issue 9 https://doi.org/10.1039/c9ta00047j	journal	January 2019
Tailored Janus silica nanosheets integrating bispecific artificial receptors for simultaneous adsorption of 2,6-dichlorophenol and Pb( ii ) Liu, Jinxin; Wang, Pan; Zhou, Mengdie Journal of Materials Chemistry A, Vol. 7, Issue 27 https://doi.org/10.1039/c9ta01116a	journal	January 2019
Multiple roles of a heterointerface in two-dimensional van der Waals heterostructures: insights into energy-related applications Zhu, Yuanzhi; Peng, Wenchao; Li, Yang Journal of Materials Chemistry A, Vol. 7, Issue 41 https://doi.org/10.1039/c9ta06395a	journal	January 2019
Fe _1−x S@S-doped carbon core–shell heterostructured hollow spheres as highly reversible anode materials for sodium ion batteries Pan, Qichang; Zheng, Fenghua; Liu, Yanzhen Journal of Materials Chemistry A, Vol. 7, Issue 35 https://doi.org/10.1039/c9ta07302g	journal	January 2019
Carbon–metal compound composite electrodes for capacitive deionization: synthesis, development and applications Tang, Kexin; Hong, Terence Zhi Xiang; You, Liming Journal of Materials Chemistry A, Vol. 7, Issue 47 https://doi.org/10.1039/c9ta08663c	journal	January 2019
Research Update: Recent progress on 2D materials beyond graphene: From ripples, defects, intercalation, and valley dynamics to straintronics and power dissipation Lin, Zhong; Lei, Yu; Subramanian, Shruti APL Materials, Vol. 6, Issue 8 https://doi.org/10.1063/1.5042598	journal	August 2018
Structural, electronic, and electromechanical properties of MoSSe/blue phosphorene heterobilayer Li, Xiaobao; Wang, Xiaotian; Hao, Weijie AIP Advances, Vol. 9, Issue 11 https://doi.org/10.1063/1.5122755	journal	November 2019
Metallic MoN layer and its application as anode for lithium-ion batteries Zhang, Qiaoxuan; Ma, Jiachen; Lei, Ming Nanotechnology, Vol. 29, Issue 16 https://doi.org/10.1088/1361-6528/aaad48	journal	February 2018
Direct versus reverse vertical two-dimensional Mo ₂ C/graphene heterostructures for enhanced hydrogen evolution reaction electrocatalysis Chaitoglou, Stefanos; Giannakopoulou, Tatiana; Tsoutsou, Dimitra Nanotechnology, Vol. 30, Issue 41 https://doi.org/10.1088/1361-6528/ab3155	journal	July 2019
SiOC functionalization of MoS ₂ as a means to improve stability as sodium-ion battery anode Soares, Davi Marcelo; Singh, Gurpreet Nanotechnology, Vol. 31, Issue 14 https://doi.org/10.1088/1361-6528/ab6480	journal	January 2020
Synthesis of Ti ₃ C ₂ /TiO ₂ heterostructure by microwave heating with high electrochemical performance Li, Zijiong; Liu, Yanyue; Guo, Dongfang Materials Research Express, Vol. 6, Issue 6 https://doi.org/10.1088/2053-1591/ab105d	journal	March 2019
Effects of biaxial strain and functional groups on SiC/ti ₃ C ₂ heterostructure: a first principle calculation Li, Chenliang; Tian, Bingkun; Yang, Yong Materials Research Express, Vol. 6, Issue 12 https://doi.org/10.1088/2053-1591/ab49c8	journal	November 2019
Tailoring Storage Capacity and Ion Kinetics in Ti 2 CO 2 / Graphene Heterostructures by Functionalization of Graphene Sevik, Cem; Çakır, Deniz Physical Review Applied, Vol. 12, Issue 1 https://doi.org/10.1103/physrevapplied.12.014001	journal	July 2019
Electronic and hyperbolic dielectric properties of Zr S 2 / Hf S 2 heterostructures Zhang, Liwei; Yu, Weiyang; Wang, Qin Physical Review B, Vol. 100, Issue 16 https://doi.org/10.1103/physrevb.100.165304	journal	October 2019
Interfacial and electronic properties of heterostructures of MXene and graphene Li, Rui; Sun, Weiwei; Zhan, Cheng Physical Review B, Vol. 99, Issue 8 https://doi.org/10.1103/physrevb.99.085429	journal	February 2019
Energy storage: The future enabled by nanomaterials Pomerantseva, Ekaterina; Bonaccorso, Francesco; Feng, Xinliang Science, Vol. 366, Issue 6468 https://doi.org/10.1126/science.aan8285	journal	November 2019
A Facile One-Pot Stepwise Hydrothermal Method for the Synthesis of 3D MoS ₂ /RGO Composites with Improved Lithium Storage Properties Wang, Bingning; Liu, Xuehua; Xu, Binghui Nano, Vol. 14, Issue 03 https://doi.org/10.1142/s1793292019500371	journal	March 2019
Synthesis of two-dimensional Ti ₃ C ₂ T _x /Au nanosheets with SERS performance Yue, Ming; Li, Fang; Lu, Nianhang Applied Optics, Vol. 58, Issue 30 https://doi.org/10.1364/ao.58.008290	journal	January 2019
Unraveling the multiscale damping properties of two-dimensional layered MXene Loganathan, Archana; Nautiyal, Pranjal; Boesl, Benjamin Nanomaterials and Energy, Vol. 8, Issue 1 https://doi.org/10.1680/jnaen.18.00022	journal	June 2019
Hydrodynamic assembly of two-dimensional layered double hydroxide nanostructures. Jose, Nicholas; Zeng, Hua Chun; Lapkin, Alexei Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.36120	text	January 2018
Optical Patterning of Two-Dimensional Materials Kollipara, Pavana Siddhartha; Li, Jingang; Zheng, Yuebing Research, Vol. 2020 https://doi.org/10.34133/2020/6581250	journal	January 2020

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