Vacuum ultraviolet photoionization and photodissociation of polyatomic molecules and radicals
Conference
·
OSTI ID:139916
- Iowa State Univ., Ames (United States)
In the past decade, tremendous progress has been made in understanding the photodissociation (PD) dynamics of triatomic molecules. However, the PD study of radicals, especially polyatomic radicals, has remained essentially an unexplored research area. Detailed state-to-state PD cross sections for radicals in the UV and VUV provide challenges not only for dynamical calculations, but also for ab initio quantum chemical studies. The authors have developed a laser based pump-probe apparatus for the measurement of absolute PD cross sections for CH{sub 3}S and HS is summarized.
- Research Organization:
- Brookhaven National Lab., Upton, NY (United States)
- OSTI ID:
- 139916
- Report Number(s):
- BNL--48923; CONF-9306172--; ON: DE93015758
- Country of Publication:
- United States
- Language:
- English
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