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Simulated changes in biogenic VOC emissions and ozone formation from habitat expansion of Acer Rubrum (red maple)

Journal Article · · Environmental Research Letters
 [1];  [2];  [3];  [2];  [4]
  1. Argonne National Lab. (ANL), Argonne, IL (United States). Environmental Science Division
  2. Univ. of Minnesota, Saint Paul, MN (United States)
  3. Univ. of Michigan, Ann Arbor, MI (United States). Dept. of Atmospheric, Oceanic and Space Sciences
  4. Univ. of Illinois, Urbana-Champaign, IL (United States). Dept. of Atmospheric Sciences
+ Show Author Affiliations
A new vegetation trend is emerging in northeastern forests of the United States, characterized by an expansion of red maple at the expense of oak. This has changed emissions of biogenic volatile organic compounds (BVOCs), primarily isoprene and monoterpenes. Oaks strongly emit isoprene while red maple emits a negligible amount. This species shift may impact nearby urban centers because the interaction of isoprene with anthropogenic nitrogen oxides can lead to tropospheric ozone formation and monoterpenes can lead to the formation of particulate matter. Here in this study the Global Biosphere Emissions and Interactions System was used to estimate the spatial changes in BVOC emission fluxes resulting from a shift in forest composition between oak and maple. A 70% reduction in isoprene emissions occurred when oak was replaced with maple. Ozone simulations with a chemical box model at two rural and two urban sites showed modest reductions in ozone concentrations of up to 5–6 ppb resulting from a transition from oak to red maple, thus suggesting that the observed change in forest composition may benefit urban air quality. This study illustrates the importance of monitoring and representing changes in forest composition and the impacts to human health indirectly through changes in BVOCs.
Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE; Univ. of Minnesota, Saint Paul, MN (United States)
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1396256
Alternate ID(s):
OSTI ID: 22480150
Journal Information:
Environmental Research Letters, Journal Name: Environmental Research Letters Journal Issue: 1 Vol. 9; ISSN 1748-9326
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English

References (38)

The Atmospheric Chemist’s Companion: Numerical Data for Use in the Atmospheric Sciences book January 2012
A biogenic hydrocarbon emission inventory for the U.S.A. using a simple forest canopy model journal August 1993
Effects of biogenic emission uncertainties on regional photochemical modeling of control strategies journal June 1994
The relation between ozone, NOx and hydrocarbons in urban and polluted rural environments journal June 1999
A review and synthesis of monoterpene speciation from forests in the United States journal January 2000
Natural emissions of non-methane volatile organic compounds, carbon monoxide, and oxides of nitrogen from North America journal January 2000
Sensitivity analysis of ground-level ozone concentration to emission changes in two urban regions of southeast Texas journal June 2005
Organic aerosol formation from the oxidation of biogenic hydrocarbons journal February 1999
Isoprene emission estimates and uncertainties for the central African EXPRESSO study domain journal December 1999
Effect of Climate Change on Isoprene Emissions and Surface Ozone Levels: ISOPRENE EMISSIONS AND SURFACE OZONE LEVELS journal September 2003
Evaluating the contribution of changes in isoprene emissions to surface ozone trends over the eastern United States journal January 2005
Effects of additional nonmethane volatile organic compounds, organic nitrates, and direct emissions of oxygenated organic species on global tropospheric chemistry journal January 2007
Multimodel estimates of intercontinental source-receptor relationships for ozone pollution journal January 2009
A numerical solution for the equations of tropospheric chemistry based on an analysis of sources and sinks of odd hydrogen journal January 1991
An improved model for estimating emissions of volatile organic compounds from forests in the eastern United States journal January 1994
A global model of natural volatile organic compound emissions journal January 1995
Influence of increased isoprene emissions on regional ozone modeling journal October 1998
Prescribing Fire in Eastern Oak Forests: Is Time Running Out? journal September 2005
Energy investment in leaves of red maple and co-occurring oaks within a forested watershed journal August 2002
Human-induced changes in US biogenic volatile organic compound emissions: evidence from long-term forest inventory data journal October 2004
Formation of Secondary Organic Aerosols Through Photooxidation of Isoprene journal February 2004
Using witness trees to assess forest change in southeastern Ohio journal October 2001
Sensitivity of ozone and aerosols to precursor emissions in Europe journal January 2012
United States land use Inventory for Estimating Biogenic Ozone Precursor Emissions journal February 1997
Three Decades of Overstory and Species Change in a Mixed Mesophytic Forest in Eastern Kentucky journal June 2005
Fire and the Development of Oak Forests journal May 1992
The Red Maple Paradox journal May 1998
Dendroecological Analysis of Successional Dynamics for a Presettlement- Origin White-Pine-Mixed-Oak Forest in the Southern Appalachians, USA journal February 1995
Changes in Structure, Pattern and Diversity Associated with Climax Forest Maturation in Piedmont, North Carolina journal January 1977
Vegetational Change in Northern New Jersey from Precolonization to the Present: A Palynological Interpretation journal July 1980
A Study of an Invasion by Red Maple of an Oak Woods in Southern Wisconsin journal May 1953
Age-Structure Relationships of Trees Species in an Appalachian Oak Forest in Southwest Virginia journal July 1982
Historical (1850–2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application journal January 2010
Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature) journal January 2006
Why are estimates of global terrestrial isoprene emissions so similar (and why is this not so for monoterpenes)? journal January 2008
The influence of foreign vs. North American emissions on surface ozone in the US journal January 2009
Description and evaluation of the Model for Ozone and Related chemical Tracers, version 4 (MOZART-4) journal January 2010
The Model of Emissions of Gases and Aerosols from Nature version 2.1 (MEGAN2.1): an extended and updated framework for modeling biogenic emissions journal January 2012

Cited By (3)

Regional to Global Biogenic Isoprene Emission Responses to Changes in Vegetation From 2000 to 2015 journal April 2018
Biodiversity matters in feedbacks between climate change and air quality: a study using an individual-based model journal April 2018
Modeling emissions for three-dimensional atmospheric chemistry transport models journal May 2018

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Related Subjects

54 ENVIRONMENTAL SCIENCES
Acer Rubrum
biogenic violatile organic compounds
isoprene
northeastern US forests
oak
ozone