Large n- and p-type thermoelectric power factors from doped semiconducting single-walled carbon nanotube thin films

MacLeod, Bradley A.; Stanton, Noah J.; Gould, Isaac E.; Wesenberg, Devin; Ihly, Rachelle; Owczarczyk, Zbyslaw R.; Hurst, Katherine E.; Fewox, Christopher S.; Folmar, Christopher N.; Holman Hughes, Katherine; Zink, Barry L.; Blackburn, Jeffrey L.; Ferguson, Andrew J.

doi:10.1039/C7EE01130J

Title: Large n- and p-type thermoelectric power factors from doped semiconducting single-walled carbon nanotube thin films

Journal Article · Fri Sep 08 00:00:00 EDT 2017 · Energy & Environmental Science

DOI:https://doi.org/10.1039/C7EE01130J· OSTI ID:1395100

^[1]; Stanton, Noah J. ^[2];

^[2]; Wesenberg, Devin ^[3];

^[2]; Owczarczyk, Zbyslaw R. ^[2];

^[2]; Fewox, Christopher S. ^[4]; Folmar, Christopher N. ^[4];

^[4];

^[3];

^[2];

^[2]

National Renewable Energy Lab. (NREL), Golden, CO (United States); International Thermodyne, Inc., Charlotte, NC (United States)
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Univ. of Denver, Denver, CO (United States)
International Thermodyne, Inc., Charlotte, NC (United States)

Lightweight, robust, and flexible single-walled carbon nanotube (SWCNT) materials can be processed inexpensively using solution-based techniques, similar to other organic semiconductors. In contrast to many semiconducting polymers, semiconducting SWCNTs (s-SWCNTs) represent unique one-dimensional organic semiconductors with chemical and physical properties that facilitate equivalent transport of electrons and holes. These factors have driven increasing attention to employing s-SWCNTs for electronic and energy harvesting applications, including thermoelectric (TE) generators. Here we demonstrate a combination of ink chemistry, solid-state polymer removal, and charge-transfer doping strategies that enable unprecedented n-type and p-type TE power factors, in the range of 700 μW m^–1 K^–2 at 298 K for the same solution-processed highly enriched thin films containing 100% s-SWCNTs. We also demonstrate that the thermal conductivity appears to decrease with decreasing s-SWCNT diameter, leading to a peak material zT ≈ 0.12 for s-SWCNTs with diameters in the range of 1.0 nm. Here, our results indicate that the TE performance of s-SWCNT-only material systems is approaching that of traditional inorganic semiconductors, paving the way for these materials to be used as the primary components for efficient, all-organic TE generators.

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Research Organization:: National Renewable Energy Lab. (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Workforce Development for Teachers and Scientists (WDTS)

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1395100

Report Number(s):: NREL/JA-5900-68583; EESNBY

Journal Information:: Energy & Environmental Science, Vol. 10, Issue 10; ISSN 1754-5692

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 133 works

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Thickness-dependent thermoelectric power factor of polymer-functionalized semiconducting carbon nanotube thin films Nonoguchi, Yoshiyuki; Takata, Ami; Goto, Chigusa Figshare https://doi.org/10.6084/m9.figshare.6824915	text	January 2018

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