Giant magnetoelectric effects achieved by tuning spin cone symmetry in Y-type hexaferrites

Zhai, Kun; Wu, Yan; Shen, Shipeng; Tian, Wei; Cao, Huibo; Chai, Yisheng; Chakoumakos, Bryan C.; Shang, Dashan; Yan, Liqin; Wang, Fangwei; Sun, Young

doi:10.1038/s41467-017-00637-x

Giant magnetoelectric effects achieved by tuning spin cone symmetry in Y-type hexaferrites

Journal Article · Tue Sep 12 00:00:00 EDT 2017 · Nature Communications

DOI:https://doi.org/10.1038/s41467-017-00637-x· OSTI ID:1394576

Zhai, Kun ^[1]; ^[2]; Shen, Shipeng ^[3]; Tian, Wei ^[2]; Cao, Huibo ^[2]; Chai, Yisheng ^[3]; Chakoumakos, Bryan C. ^[2]; ^[3]; Yan, Liqin ^[3]; Wang, Fangwei ^[3]; ^[1]

Chinese Academy of Sciences (CAS), Beijing (China). Beijing National Lab. for Condensed Matter Physics. Inst. of Physics; Univ. of Chinese Academy of Sciences, Beijing (China). School of Physical Science
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
Chinese Academy of Sciences (CAS), Beijing (China). Beijing National Lab. for Condensed Matter Physics. Inst. of Physics

Multiferroics materials, which exhibit coupled magnetic and ferroelectric properties, have attracted tremendous research interest because of their potential in constructing next-generation multifunctional devices. The application of single-phase multiferroics is currently limited by their usually small magnetoelectric effects. Here, we report the realization of giant magnetoelectric effects in a Y-type hexaferrite Ba_0.4Sr_1.6Mg₂Fe₁₂O₂₂ single crystal, which exhibits record-breaking direct and converse magnetoelectric coefficients and a large electric-field-reversed magnetization. We have uncovered the origin of the giant magnetoelectric effects by a systematic study in the Ba_2-x Sr _x Mg₂Fe₁₂O₂₂ family with magnetization, ferroelectricity and neutron diffraction measurements. With the transverse spin cone symmetry restricted to be two-fold, the one-step sharp magnetization reversal is realized and giant magnetoelectric coefficients are achieved. Our study reveals that tuning magnetic symmetry is an effective route to enhance the magnetoelectric effects also in multiferroic hexaferrites.

View Accepted Manuscript (DOE)

Research Organization:: Chinese Academy of Sciences (CAS), Beijing (China); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: Chinese Academy of Sciences (CAS); National Key Research and Development Program of China; National Natural Science Foundation of China (NSFC); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1394576

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 8; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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