Electronic structure of the chiral helimagnet and 3d-intercalated transition metal dichalcogenide Cr1/3NbS2

Sirca, N.; Mo, S. -K.; Bondino, F.; Pis, I.; Nappini, S.; Vilmercati, P.; Yi, Jieyu; Gai, Zheng; Snijders, Paul C.; Das, P. K.; Vobornik, I.; Ghimire, N. J.; Koehler, Michael R.; Sopkota, D.; Parker, David S.; Mandrus, D. G.; Mannella, Norman

doi:10.1103/PhysRevB.94.075141

Title: Electronic structure of the chiral helimagnet and 3d-intercalated transition metal dichalcogenide Cr_1/3NbS₂

Journal Article · Thu Aug 18 00:00:00 EDT 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.94.075141· OSTI ID:1311264

Sirca, N. ^[1]; Mo, S. -K. ^[2]; Bondino, F. ^[3]; Pis, I. ^[4]; Nappini, S. ^[3]; Vilmercati, P. ^[1]; Yi, Jieyu ^[1]; Gai, Zheng ^[5]; Snijders, Paul C. ^[6]; Das, P. K. ^[7]; Vobornik, I. ^[3]; Ghimire, N. J. ^[1]; Koehler, Michael R. ^[1]; Sopkota, D. ^[1]; Parker, David S. ^[8]; Mandrus, D. G. ^[9]; Mannella, Norman ^[1]

Univ. of Tennessee, Knoxville, TN (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
Institute of Materials Workshop (IOM), CNR Laboratory, Trieste (Italy)
Institute of Materials Workshop (IOM), CNR Laboratory, Trieste (Italy); Elettra Sincrotrone Trieste, Basovizza (Italy)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science (CNMS)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
Institute of Materials Workshop (IOM), CNR Laboratory, Trieste (Italy); International Centre for Theoretical Physics, Strada Costiera, Trieste (Italy)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

©2016 American Physical Society. The electronic structure of the chiral helimagnet Cr1/3NbS2 has been studied with core level and angle-resolved photoemission spectroscopy (ARPES). Intercalated Cr atoms are found to be effective in donating electrons to the NbS2 layers but also cause significant modifications of the electronic structure of the host NbS2 material. In particular, the data provide evidence that a description of the electronic structure of Cr1/3NbS2 on the basis of a simple rigid band picture is untenable. The data also reveal substantial inconsistencies with the predictions of standard density functional theory. The relevance of these results to the attainment of a correct description of the electronic structure of chiral helimagnets, magnetic thin films/multilayers, and transition metal dichalcogenides intercalated with 3d magnetic elements is discussed.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: AC05-00OR22725; AC02-05CH1123; DMR-1151687; DMR-1410428; AC02-05CH11231

OSTI ID:: 1311264

Alternate ID(s):: OSTI ID: 1298342; OSTI ID: 1393070

Journal Information:: Physical Review B, Vol. 94, Issue 7; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 34 works

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