Progress in High‐Voltage Cathode Materials for Rechargeable Sodium‐Ion Batteries

You, Ya; Manthiram, Arumugam

doi:10.1002/aenm.201701785

Title: Progress in High‐Voltage Cathode Materials for Rechargeable Sodium‐Ion Batteries

Journal Article · Mon Sep 18 00:00:00 EDT 2017 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201701785· OSTI ID:1392184

You, Ya ^[1]; Manthiram, Arumugam ^[1]

Materials Science and Engineering Program and Texas Materials Institute The University of Texas at Austin Austin TX 78712 USA

Abstract Room‐temperature rechargeable sodium‐ion batteries are considered as a promising alternative technology for grid and other storage applications due to their competitive cost benefit and sustainable resource supply, triumphing other battery systems on the market. To facilitate the practical realization of the sodium‐ion technology, the energy density of sodium‐ion batteries needs to be boosted to the level of current commercial Li‐ion batteries. An effective approach would be to elevate the operating voltage of the battery, which requires the use of electrochemically stable cathode materials with high voltage versus Na ⁺ /Na. This review summarizes the recent progress with the emerging high‐voltage cathode materials for room‐temperature sodium‐ion batteries, which include layered transitional‐metal oxides, Na‐rich materials, and polyanion compounds. The key challenges and corresponding strategies for these materials are also discussed, with an emphasis placed on the intrinsic structural properties, Na storage electrochemistry, and the voltage variation tendency with respect to the redox reactions. The insights presented in this article can serve as a guide for improving the energy densities of room‐temperature Na‐ion batteries.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: DE‐SC0005397

OSTI ID:: 1392184

Journal Information:: Advanced Energy Materials, Journal Name: Advanced Energy Materials Vol. 8 Journal Issue: 2; ISSN 1614-6832

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Cited by: 303 works

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Strong Oxygen Participation in the Redox Governing the Structural and Electrochemical Properties of Na-Rich Layered Oxide Na ₂ IrO ₃ Perez, Arnaud J.; Batuk, Dmitry; Saubanère, Matthieu Chemistry of Materials, Vol. 28, Issue 22 https://doi.org/10.1021/acs.chemmater.6b03338	journal	October 2016
Na4Co3(PO4)2P2O7: A novel storage material for sodium-ion batteries Nose, Masafumi; Nakayama, Hideki; Nobuhara, Kunihiro Journal of Power Sources, Vol. 234 https://doi.org/10.1016/j.jpowsour.2013.01.162	journal	July 2013
Crystal-Chemical Guide for Understanding Redox Energy Variations of M ^2+/3+ Couples in Polyanion Cathodes for Lithium-Ion Batteries Gutierrez, Arturo; Benedek, Nicole A.; Manthiram, Arumugam Chemistry of Materials, Vol. 25, Issue 20 https://doi.org/10.1021/cm401949n	journal	October 2013
Subzero-Temperature Cathode for a Sodium-Ion Battery You, Ya; Yao, Hu-Rong; Xin, Sen Advanced Materials, Vol. 28, Issue 33 https://doi.org/10.1002/adma.201600846	journal	June 2016
A Layered P2- and O3-Type Composite as a High-Energy Cathode for Rechargeable Sodium-Ion Batteries Guo, Shaohua; Liu, Pan; Yu, Haijun Angewandte Chemie International Edition, Vol. 54, Issue 20 https://doi.org/10.1002/anie.201411788	journal	April 2015

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