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Title: Quantifying black carbon deposition over the Greenland ice sheet from forest fires in Canada

Journal Article · · Geophysical Research Letters
DOI:https://doi.org/10.1002/2017GL073701· OSTI ID:1390441
ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [4]; ORCiD logo [5]; ORCiD logo [3]; ORCiD logo [1]; ORCiD logo [6]; ORCiD logo [6]; ORCiD logo [7]; ORCiD logo [1];  [1]; ORCiD logo [8]; ORCiD logo [9]
  1. Inst. Pierre Simon Laplace (IPSL), Paris (France). Lab. Atmosphères, Milieux, Observations Spatiales (LATMOS); Sorbonne Univ., Pierre and Marie Curie Campus (UPMC), Paris (France); Univ. of Versailles Saint-Quentin-en-Yvelines (UVSQ) (France); Centre National de la Recherche Scientifique (CNRS), Paris (France)
  2. US Army Corps of Engineers (ACE), Fort Wainwright, AK (United States). Cold Regions Research and Engineering Lab. (CRREL); Dartmouth College, Hanover, NH (United States)
  3. NASA Langley Research Center, Hampton, VA (United States)
  4. Center for International Climate and Environmental Research-Oslo (CICERO) (Norway)
  5. Dartmouth College, Hanover, NH (United States); NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States)
  6. National Center for Atmospheric Research, Boulder, CO (United States)
  7. Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
  8. Univ. of Michigan, Ann Arbor, MI (United States)
  9. Univ. of New Hampshire, Durham, NH (United States)

We identify an important Black Carbon (BC) aerosol deposition event that was observed in snow stratigraphy and dated to between 27 July 2013 – 2 August 2013. This event comprises a significant portion (~60%) of total deposition over a 10 month period (July 2013 – April 2014). Here we link this event to forest fires burning in Canada during summer 2013 using modeling and remote sensing tools. Aerosols were detected by both the CALIOP and MODIS instruments during transport between Canada and Greenland, confirming that this event involved emissions from forest fires in Canada. We use high-resolution regional chemical transport mod-eling (WRF-Chem) combined with high-resolution fire emissions (FINNv1.5) to study aerosol emissions, transport, and deposition during this event. The model accurately captures the timing of the BC deposition event and shows that the major contribution to deposition during this event is emissions originating from fires in Canada. However, the model under-predicts aerosol deposition compared to measurements at all sites by a factor of 2–100. Under-prediction of modeled BC deposition originates from uncertainties in fire emissions combined with uncertainties in aerosol scavenging by clouds. This study suggests that it is possible to describe the transport of an exceptional smoke event on regional and continental scales. Improvements in model descriptions of precipitation scavenging and emissions from wildfires are needed to correctly predict deposition, which is critical for determining the climate impacts of aerosols that originate from fires.

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE; National Science Foundation (NSF); National Aeronautics and Space Administration (NASA); GENCI (France)
Grant/Contract Number:
AC05-76RL01830; ARC1203876; ARC1204145; NNX14AE72G; NNH15AZ74I; 2016-017141
OSTI ID:
1390441
Report Number(s):
PNNL-SA-125266; KP1701000
Journal Information:
Geophysical Research Letters, Vol. 44, Issue 15; ISSN 0094-8276
Publisher:
American Geophysical UnionCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 37 works
Citation information provided by
Web of Science

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Cited By (11)

Modeled Response of Greenland Snowmelt to the Presence of Biomass Burning-Based Absorbing Aerosols in the Atmosphere and Snow journal June 2018
Radiative Forcing by Dust and Black Carbon on the Juneau Icefield, Alaska journal April 2019
Progress and Challenges in Quantifying Wildfire Smoke Emissions, Their Properties, Transport, and Atmospheric Impacts journal December 2019
Space‐Based Observations for Understanding Changes in the Arctic‐Boreal Zone journal January 2020
Palynological insights into global change impacts on Arctic vegetation, fire, and pollution recorded in Central Greenland ice journal March 2019
Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol journal April 2019
Recognizing Women Leaders in Fire Science journal August 2018
Investigating the impact of aerosol deposition on snowmelt over the Greenland Ice Sheet using a large-ensemble kernel journal January 2018
Impact of MODIS sensor calibration updates on Greenland Ice Sheet surface reflectance and albedo trends journal January 2017
Palynological insights into global change impacts on Arctic vegetation, fire, and pollution recorded in Central Greenland ice text January 2019
Impact of MODIS sensor calibration updates on Greenland Ice Sheet surface reflectance and albedo trends text January 2017

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