Vogel-Fulcher-Tammann freezing of a thermally fluctuating artificial spin ice probed by x-ray photon correlation spectroscopy

Morley, S. A.; Alba Venero, D.; Porro, J. M.; Riley, S. T.; Stein, A.; Steadman, P.; Stamps, R. L.; Langridge, S.; Marrows, C. H.

doi:10.1103/PhysRevB.95.104422

Title: Vogel-Fulcher-Tammann freezing of a thermally fluctuating artificial spin ice probed by x-ray photon correlation spectroscopy

Journal Article · Thu Mar 16 00:00:00 EDT 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.95.104422· OSTI ID:1389248

Morley, S. A. ^[1]; Alba Venero, D. ^[2]; Porro, J. M. ^[2]; Riley, S. T. ^[1]; Stein, A. ^[3]; Steadman, P. ^[4]; Stamps, R. L. ^[5]; Langridge, S. ^[2]; Marrows, C. H. ^[1]

Univ. of Leeds (United Kingdom)
Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Lab., ISIS Neutron Source
Brookhaven National Lab. (BNL), Upton, NY (United States)
Science and Technology Facilities Council (STFC), Harwell Campus, Oxford (United Kingdom). Diamond Light Source, Ltd.
Univ. of Glasgow, Scotland (United Kingdom)

We report on the crossover from the thermal to the athermal regime of an artificial spin ice formed from a square array of magnetic islands whose lateral size, 30 nm × 70 nm, is small enough that they are dynamic at room temperature.We used resonant magnetic soft x-ray photon correlation spectroscopy as a method to observe the time-time correlations of the fluctuating magnetic configurations of spin ice during cooling, which are found to slow abruptly as a freezing temperature of T₀ = 178 ± 5 K is approached. This slowing is well described by a Vogel-Fulcher-Tammann law, implying that the frozen state is glassy, with the freezing temperature being commensurate with the strength of magnetostatic interaction energies in the array. The activation temperature, T_A = 40 ± 10 K, is much less than that expected from a Stoner-Wohlfarth coherent rotation model. Zerofield- cooled/field-cooled magnetometry reveals a freeing up of fluctuations of states within islands above this temperature, caused by variation in the local anisotropy axes at the oxidised edges. This Vogel-Fulcher-Tammann behavior implies that the system enters a glassy state upon freezing, which is unexpected for a system with a well-defined ground state.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; AC02-98CH10886

OSTI ID:: 1389248

Alternate ID(s):: OSTI ID: 1347265

Report Number(s):: BNL-114268-2017-JA; PRBMDO; KC0403020; TRN: US1702699

Journal Information:: Physical Review B, Vol. 95, Issue 10; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 32 works

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