Interface-induced multiferroism by design in complex oxide superlattices

Guo, Hangwen; Wang, Zhen; Dong, Shuai; Ghosh, Saurabh; Saghayezhian, Mohammad; Chen, Lina; Weng, Yakui; Herklotz, Andreas; Ward, Thomas Z.; Jin, Rongying; Pantelides, Sokrates T.; Zhu, Yimei; Zhang, Jiandi; Plummer, E. W.

doi:10.1073/pnas.1706814114

Title: Interface-induced multiferroism by design in complex oxide superlattices

Journal Article · Mon Jun 12 00:00:00 EDT 2017 · Proceedings of the National Academy of Sciences of the United States of America

DOI:https://doi.org/10.1073/pnas.1706814114· OSTI ID:1389234

Guo, Hangwen ^[1]; Wang, Zhen ^[2]; Dong, Shuai ^[3]; Ghosh, Saurabh ^[4]; Saghayezhian, Mohammad ^[1]; Chen, Lina ^[1]; Weng, Yakui ^[3]; Herklotz, Andreas ^[5]; Ward, Thomas Z. ^[5]; Jin, Rongying ^[1]; Pantelides, Sokrates T. ^[4]; Zhu, Yimei ^[6]; Zhang, Jiandi ^[1]; Plummer, E. W. ^[1]

Louisiana State Univ., Baton Rouge, LA (United States)
Louisiana State Univ., Baton Rouge, LA (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)
Southeast Univ., Nanjing (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Vanderbilt Univ., Nashville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)

Interfaces between materials present unique opportunities for the discovery of intriguing quantum phenomena. Here we explore the possibility that, in the case of superlattices, if one of the layers is made ultrathin, unexpected properties can be induced between the two bracketing interfaces. We pursue this objective by combining advanced growth and characterization techniques with theoretical calculations. Using prototype La_2/3Sr_1/3MnO₃/BaTiO₃ (LSMO/BTO) superlattices, we observe a structural evolution in the LSMO layers as a function of thickness. Atomic-resolution electron microscopy and spectroscopy reveal an unusual polar structure phase in ultrathin LSMO at a critical thickness due to interfacing with the adjacent BTO layers, which is confirmed by first-principles calculations. Most important is the fact that this polar phase is accompanied by re-emergent ferromagnetism, making this system a potential candidate for ultrathin ferroelectrics with ferromagnetic ordering. Monte-Carlo simulations illustrate the important role of spin-lattice coupling in LSMO. The present results open up a conceptually intriguing recipe for developing novel functional ultrathin materials via interface-induced spin-lattice coupling.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Oak Ridge Leadership Computing Facility (OLCF); Brookhaven National Laboratory (BNL), Upton, NY (United States); Vanderbilt Univ., Nashville, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; AC05-00OR22725; FG02-09ER46554

OSTI ID:: 1389234

Alternate ID(s):: OSTI ID: 1376517; OSTI ID: 1597823

Report Number(s):: BNL-114200-2017-JA; R&D Project: MA015MACA; KC0201010

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Vol. 114, Issue 26; ISSN 0027-8424

Publisher:: National Academy of Sciences, Washington, DC (United States)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 45 works

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Control of magnetic anisotropy by orbital hybridization with charge transfer in (La0.67Sr0.33MnO3)n/(SrTiO3)n superlattice Zhang, Bangmin; Wu, Lijun; Zheng, Jincheng NPG Asia Materials, Vol. 10, Issue 9 https://doi.org/10.1038/s41427-018-0084-8	journal	September 2018
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Atomic-scale mapping of interface reconstructions in multiferroic heterostructures Huang, Weichuan; Yin, Yuewei; Li, Xiaoguang Applied Physics Reviews, Vol. 5, Issue 4 https://doi.org/10.1063/1.5053426	journal	December 2018
Strain-driven lattice distortion and the resultant magnetic properties of La _0.7 Sr _0.3 MnO ₃ /BaTiO ₃ superlattices Chen, Liming; Zhang, Chunchen; Chen, Yequan Applied Physics Letters, Vol. 115, Issue 20 https://doi.org/10.1063/1.5119736	journal	November 2019
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