Studies on Thermoelectric Properties of n-type Polycrystalline SnSe 1-x S x by Iodine Doping

Zhang, Qian; Chere, Eyob Kebede; Sun, Jingying; Cao, Feng; Dahal, Keshab; Chen, Shuo; Chen, Gang; Ren, Zhifeng

doi:10.1002/aenm.201500360

Title: Studies on Thermoelectric Properties of n-type Polycrystalline SnSe _1-x S _x by Iodine Doping

Journal Article · Wed Apr 22 00:00:00 EDT 2015 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201500360· OSTI ID:1387039

Zhang, Qian ^[1]; Chere, Eyob Kebede ^[1]; Sun, Jingying ^[1]; Cao, Feng ^[1]; Dahal, Keshab ^[1]; Chen, Shuo ^[1]; Chen, Gang ^[2]; Ren, Zhifeng ^[1]

Department of Physics and TcSUH, University of Houston, Houston TX 77204 USA
Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge MA 02139 USA

Iodine-doped n-type SnSe polycrystalline by melting and hot pressing is prepared. The prepared material is anisotropic with a peak ZT of ≈0.8 at about 773 K measured along the hot pressing direction. This is the first report on thermoelectric properties of n-type Sn chalcogenide alloys. With increasing content of iodine, the carrier concentration changed from 2.3 × 1017 cm-3 (p-type) to 5.0 × 1015 cm-3 (n-type) then to 2.0 × 1017 cm-3 (n-type). The decent ZT is mainly attributed to the intrinsically low thermal conductivity due to the high anharmonicity of the chemical bonds like those in p-type SnSe. By alloying with 10 at% SnS, even lower thermal conductivity and an enhanced Seebeck coefficient were achieved, leading to an increased ZT of ≈1.0 at about 773 K measured also along the hot pressing direction.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Solid-State Solar-Thermal Energy Conversion Center (S3TEC)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

DOE Contract Number:: SC0001299; FG02-09ER46577

OSTI ID:: 1387039

Journal Information:: Advanced Energy Materials, Vol. 5, Issue 12; Related Information: S3TEC partners with Massachusetts Institute of Technology (lead); Boston College; Oak Ridge National Laboratory; Rensselaer Polytechnic Institute; ISSN 1614-6832

Publisher:: Wiley

Country of Publication:: United States

Language:: English

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solar (photovoltaic)
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materials and chemistry by design
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Title: Studies on Thermoelectric Properties of n-type Polycrystalline SnSe 1-x S x by Iodine Doping

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Title: Studies on Thermoelectric Properties of n-type Polycrystalline SnSe _1-x S _x by Iodine Doping