skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Anomalous ultrafast dynamics of hot plasmonic electrons in nanostructures with hot spots

Journal Article · · Nature Nanotechnology

Research Organization:
Energy Frontier Research Centers (EFRC) (United States). Argonne-Northwestern Solar Energy Research Center (ANSER)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
DOE Contract Number:
SC0001059
OSTI ID:
1386272
Journal Information:
Nature Nanotechnology, Vol. 10, Issue 9; Related Information: ANSER partners with Northwestern University (lead); Argonne National Laboratory; University of Chicago; University of Illinois, Urbana-Champaign; Yale University; ISSN 1748-3387
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English

References (33)

Controlling Subnanometer Gaps in Plasmonic Dimers Using Graphene journal October 2013
Kinetic Density Functional Theory for Plasmonic Nanostructures: Breaking of the Plasmon Peak in the Quantum Regime and Generation of Hot Electrons journal March 2015
Antennas for light journal February 2011
Subpicosecond Optical Switching with a Negative Index Metamaterial journal October 2009
Plasmon-induced hot-electron generation at nanoparticle/metal-oxide interfaces for photovoltaic and photocatalytic devices journal January 2014
Mechanisms and Applications of Plasmon-Induced Charge Separation at TiO 2 Films Loaded with Gold Nanoparticles journal May 2005
Nanoantenna-enhanced ultrafast nonlinear spectroscopy of a single gold nanoparticle journal May 2011
Ultrafast resonant optical scattering from single gold nanorods: Large nonlinearities and plasmon saturation journal April 2006
Hot Electrons Do the Impossible: Plasmon-Induced Dissociation of H 2 on Au journal December 2012
Optical Generation of Hot Plasmonic Carriers in Metal Nanocrystals: The Effects of Shape and Field Enhancement journal March 2014
Theoretical Studies of Plasmonics using Electronic Structure Methods journal June 2011
Photocatalytic Activity Enhanced by Plasmonic Resonant Energy Transfer from Metal to Semiconductor journal August 2012
Ultrafast Resonant Dynamics of Surface Plasmons in Gold Nanorods journal January 2007
Ultrafast Electron Dynamics and Optical Nonlinearities in Metal Nanoparticles journal March 2001
Resonant Optical Antennas journal June 2005
Probing the Ultimate Limits of Plasmonic Enhancement journal August 2012
Ultrafast Nonlinear Optical Response of a Single Gold Nanorod near Its Surface Plasmon Resonance journal July 2011
Optical nanoantenna arrays loaded with nonlinear materials journal December 2010
Optical Studies of Dynamics in Noble Metal Nanostructures journal June 2011
Photogeneration of hot plasmonic electrons with metal nanocrystals: Quantum description and potential applications journal February 2014
Plasmon-Induced Hot Carriers in Metallic Nanoparticles journal July 2014
Hotspot-mediated ultrafast nonlinear control of multifrequency plasmonic nanoantennas journal September 2014
Near-Infrared Plasmon-Assisted Water Oxidation journal April 2012
Control of Radiative Processes Using Tunable Plasmonic Nanopatch Antennas journal July 2014
Transient Optical Response of a Single Gold Nanoantenna: The Role of Plasmon Detuning journal March 2015
Ultrafast Plasmon-Induced Electron Transfer from Gold Nanodots into TiO 2 Nanoparticles journal December 2007
Drude Relaxation Rate in Grained Gold Nanoantennas journal March 2010
Ultrafast dynamics of nonequilibrium electrons in a gold nanoparticle system journal May 1998
Ultrafast Phase Transition via Catastrophic Phonon Collapse Driven by Plasmonic Hot-Electron Injection journal January 2014
Photodetection with Active Optical Antennas journal May 2011
Resonant optical antennas conference April 2014
Nanoantenna-enhanced ultrafast nonlinear spectroscopy of a single gold nanoparticle text January 2011
Ultrafast resonant optical scattering from single gold nanorods: Large nonlinearities and plasmon saturation text January 2005

Cited By (58)

Multigaps Embedded Nanoassemblies Enhance In Situ Raman Spectroscopy for Intracellular Telomerase Activity Sensing journal February 2016
Tailorable Dynamics in Nonlinear Optical Metasurfaces journal June 2019
Efficiency and Bond Selectivity in Plasmon-Induced Photochemistry journal June 2017
Broadband Metamaterial Absorbers journal October 2018
“Hot” in Plasmonics: Temperature‐Related Concepts and Applications of Metal Nanostructures journal November 2019
Interface-Engineered Plasmonics in Metal/Semiconductor Heterostructures journal June 2016
Light-Induced Tuning and Reconfiguration of Nanophotonic Structures: Light-Induced Tuning and Reconfiguration of Nanophotonic Structures journal August 2017
Insight into plasmonic hot-electron transfer and plasmon molecular drive: new dimensions in energy conversion and nanofabrication journal December 2017
Nonlinear photonic metasurfaces journal March 2017
Evolution from the plasmon to exciton state in ligand-protected atomically precise gold nanoparticles journal October 2016
Plasmonic hot electron transport drives nano-localized chemistry journal March 2017
Ultrafast switching of tunable infrared plasmons in indium tin oxide nanorod arrays with large absolute amplitude journal February 2016
Direct observation of ultrafast plasmonic hot electron transfer in the strong coupling regime journal January 2019
“Hot” electrons in metallic nanostructures—non-thermal carriers or heating? journal October 2019
Enhanced generation and anisotropic Coulomb scattering of hot electrons in an ultra-broadband plasmonic nanopatch metasurface journal October 2017
Electron heating and thermal relaxation of gold nanorods revealed by two-dimensional electronic spectroscopy journal March 2018
Determination of hot carrier energy distributions from inversion of ultrafast pump-probe reflectivity measurements journal May 2018
Disentangling charge carrier from photothermal effects in plasmonic metal nanostructures journal June 2019
Designer photonic dynamics by using non-uniform electron temperature distribution for on-demand all-optical switching times journal July 2019
From plasmon-enhanced molecular spectroscopy to plasmon-mediated chemical reactions journal August 2018
Plasmon-induced hot electron transfer in AgNW@TiO2@AuNPs nanostructures journal September 2018
Ultrafast and nonlinear surface-enhanced Raman spectroscopy journal January 2016
Hybrid nanostructures of metal/two-dimensional nanomaterials for plasmon-enhanced applications journal January 2016
Plasmonic nanoparticle-semiconductor composites for efficient solar water splitting journal January 2016
Generation of hot electrons in nanostructures incorporating conventional and unconventional plasmonic materials journal January 2019
Direct optical excitation of dark plasmons for hot electron generation journal January 2019
Nanoscale tracking plasmon-driven photocatalysis in individual nanojunctions by vibrational spectroscopy journal January 2018
Highly efficient plasmon-mediated electron injection into cerium oxide from embedded silver nanoparticles journal January 2019
Tunable surface plasmon polaritons and ultrafast dynamics in 2D nanohole arrays journal January 2019
Electrocatalytic glycerol oxidation enabled by surface plasmon polariton-induced hot carriers in Kretschmann configuration journal January 2019
Recent advances in cancer bioimaging using a rationally designed Raman reporter in combination with plasmonic gold journal January 2020
Ultrafast light-induced softening of chalcogenide thin films above the rigidity percolation transition journal September 2018
In situ detection of hot-electron-induced photocatalytic reduction using Au@Ag, Au@Ag 2 S, and Au@SiO 2 core-shell nanoparticles journal May 2019
40 GHz-rate all-optical cross-modulation of core-guided near infrared light in single mode fiber by surface plasmons on gold-coated tilted fiber Bragg gratings journal December 2019
Hot carrier dynamics in a dispersionless plasmonic system journal December 2019
Plasmon charge transfer dynamics in layered Au–ZnO nanocomposites journal February 2020
Vibrational coupling in plasmonic molecules journal October 2017
Dual-plasmonic Au/graphene/Au-enhanced ultrafast, broadband, self-driven silicon Schottky photodetector journal October 2018
Coherent control of the noninstantaneous nonlinear power-law response in resonant nanostructures journal January 2020
Ab initio phonon coupling and optical response of hot electrons in plasmonic metals journal August 2016
Enhancement of electron hot spot relaxation in photoexcited plasmonic structures by thermal diffusion journal November 2016
Experimental and Ab Initio Ultrafast Carrier Dynamics in Plasmonic Nanoparticles journal February 2017
Transport of hot carriers in plasmonic nanostructures journal July 2019
Nonlinear optics in all-dielectric nanoantennas and metasurfaces: a review journal March 2019
Optical plasmon nanostrip probe as an effective ultrashort pulse delivery system journal January 2019
Plasmonic hot carrier dynamics in solid-state and chemical systems for energy conversion journal January 2016
Exciton-plasmon polariton coupling and hot carrier generation in two-dimensional SiB semiconductors: a first-principles study journal February 2020
Nanoplasmon–Semiconductor Hybrid for Interface Catalysis journal September 2018
The UV Plasmonic Behavior of Distorted Rhodium Nanocubes journal December 2017
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation journal January 2019
Direct optical excitation of dark plasmons for hot electron generation text January 2019
Multigaps Embedded Nanoassemblies Enhance In Situ Raman Spectroscopy for Intracellular Telomerase Activity Sensing journal October 2020
Ab initio phonon coupling and optical response of hot electrons in plasmonic metals text January 2016
Enhancement of electron hot spot relaxation in photoexcited plasmonic structures by thermal diffusion text January 2016
Experimental and ab initio ultrafast carrier dynamics in plasmonic nanoparticles text January 2016
Ultrafast light-induced softening of chalcogenide thin films above the rigidity percolation transition text January 2018
Hot carrier dynamics in a dispersionless plasmonic system text January 2019
Coherent Control of the Non-instantaneous Nonlinear Power-law Response in Resonant Nanostructures text January 2019