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Effects of excess Fe on upper critical field and magnetotransport in Fe1+y ( Te1-x Sx ) z

Journal Article · · Physical Review. B, Condensed Matter and Materials Physics
We have investigated the upper critical field anisotropy and magnetotransport properties of Fe 1.14 ( 1 ) Te 0.91 ( 2 ) S 0.09 ( 2 ) single crystals in stable magnetic fields up to 35 T. The results show that μ 0 H c 2 ( T ) along the c axis and in the a b plane exhibit saturation at low temperatures. The anisotropy of μ 0 H c 2 ( T ) decreases with decreasing temperature, becoming nearly isotropic for T → 0 . Our analysis indicates that the spin-paramagnetic pair breaking with spin-orbital scattering is responsible for the behavior of μ 0 H c 2 ( T ) . Furthermore, from analysis of the normal-state properties, we show evidence that the excess Fe is a key factor determining the normal- and superconducting-state physical properties.
Research Organization:
Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)
Sponsoring Organization:
USDOE SC Office of Basic Energy Sciences (SC-22)
DOE Contract Number:
AC02-98CH10886
OSTI ID:
1385911
Journal Information:
Physical Review. B, Condensed Matter and Materials Physics, Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Issue: 18 Vol. 81; ISSN 1098-0121; ISSN PRBMDO
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English

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