Charge density wave order in 1D mirror twin boundaries of single-layer MoSe2

Barja, Sara; Wickenburg, Sebastian; Liu, Zhen-Fei; Zhang, Yi; Ryu, Hyejin; Ugeda, Miguel M.; Hussain, Zahid; Shen, Zhi-Xun; Mo, Sung-Kwan; Wong, Ed; Salmeron, Miquel B.; Wang, Feng; Crommie, Michael F.; Ogletree, D. Frank; Neaton, Jeffrey B.; Weber-Bargioni, Alexander

doi:10.1038/nphys3730

Title: Charge density wave order in 1D mirror twin boundaries of single-layer MoSe₂

Journal Article · Mon Apr 18 00:00:00 EDT 2016 · Nature Physics

DOI:https://doi.org/10.1038/nphys3730· OSTI ID:1379553

Barja, Sara ^[1]; Wickenburg, Sebastian ^[1]; Liu, Zhen-Fei ^[1];

^[2]; Ryu, Hyejin ^[3]; Ugeda, Miguel M. ^[4]; Hussain, Zahid ^[3]; Shen, Zhi-Xun ^[5];

^[3]; Wong, Ed ^[1]; Salmeron, Miquel B. ^[6]; Wang, Feng ^[7]; Crommie, Michael F. ^[7]; Ogletree, D. Frank ^[1]; Neaton, Jeffrey B. ^[8]; Weber-Bargioni, Alexander ^[1]

Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Foundry, Materials Division
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source; Nanjing Univ. (China). Collaborative Innovation Center of Advanced Microstructures
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source
Univ. of California, Berkeley, CA (United States). Dept. of Physics; CIC nanoGUNE, Donostia-San Sebastian (Spain); Ikerbasque, Bilbao (Spain). Basque Foundation for Science
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Univ. of California, Berkeley, CA (United States). Dept. of Physics, Dept. of Materials Science and Engineering
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Division, Kavli Energy NanoSciences Inst.; Univ. of California, Berkeley, CA (United States). Dept. of Physics
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Foundry, Materials Division, Kavli Energy NanoSciences Inst.; Univ. of California, Berkeley, CA (United States). Dept. of Physics

Here, We provide direct evidence for the existence of isolated, one-dimensional charge density waves at mirror twin boundaries (MTBs) of single-layer semiconducting MoSe ₂. Such MTBs have been previously observed by transmission electron microscopy and have been predicted to be metallic in MoSe ₂ and MoS₂. Our low-temperature scanning tunnelling microscopy/spectroscopy measurements revealed a substantial bandgap of 100 meV opening at the Fermi energy in the otherwise metallic one-dimensional structures. We found a periodic modulation in the density of states along the MTB, with a wavelength of approximately three lattice constants. In addition to mapping the energy-dependent density of states, we determined the atomic structure and bonding of the MTB through simultaneous high-resolution non-contact atomic force microscopy. Density functional theory calculations based on the observed structure reproduced both the gap opening and the spatially resolved density of states.

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Research Organization:: Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-05CH11231; AC02-76SF00515

OSTI ID:: 1379553

Journal Information:: Nature Physics, Vol. 12, Issue 8; ISSN 1745-2473

Publisher:: Nature Publishing Group (NPG)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 156 works

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Title: Charge density wave order in 1D mirror twin boundaries of single-layer MoSe₂