skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Measurement of scintillation and ionization yield with high-pressure gaseous mixtures of Xe and TMA for improved neutrinoless double beta decay and dark matter searches

Journal Article · · Journal of Instrumentation
 [1];  [1];  [1];  [1];  [2];  [1];  [1]
  1. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of Texas, Arlington, TX (United States)

The gaseous Xenon(Xe) time projection chamber (TPC) is an attractive detector technique for neutrinoless double beta decay and WIMP dark matter searches. While it is less dense compared to Liquid Xe detectors, it has intrinsic advantages in tracking capability and better energy resolution. The performance of gaseous Xe can be further improved by molecular additives such as trimethylamine(TMA), which is expected to (1) cool down the ionization electrons, (2) convert Xe excitation energy to TMA ionizations through Penning transfer, and (3) produce scintillation and electroluminescence light in a more easily detectable wavelength (300 nm). In order to test the feasibility of the performance improvements with TMA, in this paper we made the first direct measurement of Penning and fluorescence transfer efficiency with gaseous mixtures of Xe and TMA. While we observed a Penning transfer efficiency up to ~35%, we found strong suppression of primary scintillation light with TMA. We also found that the primary scintillation light with Xe and TMA mixture can be well characterized by ~3% fluorescence transfer from Xe to TMA, with further suppression due to TMA self-quenching. No evidence of the scintillation light produced by recombination of TMA ions was found. This strong suppression of scintillation light makes dark matter searches quite challenging, while the possibility of improved neutrinoless double beta decay searches remains open. Finally, this work has been carried out within the context of the NEXT collaboration.

Research Organization:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC02-05CH11231; FC52-08NA28752
OSTI ID:
1379237
Journal Information:
Journal of Instrumentation, Vol. 11, Issue 3; ISSN 1748-0221
Publisher:
Institute of Physics (IOP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 6 works
Citation information provided by
Web of Science

References (8)

Columnar recombination: a tool for nuclear recoil directional sensitivity in a xenon-based direct detection WIMP search journal October 2013
Micro-physics simulations of columnar recombination along nuclear recoil tracks in high-pressure Xe gas for directional dark matter searches journal November 2015
Accurate γ and MeV-electron track reconstruction with an ultra-low diffusion Xenon/TMA TPC at 10 atm
  • González-Díaz, Diego; Álvarez, V.; Borges, F. I. G.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 804 https://doi.org/10.1016/j.nima.2015.08.033
journal December 2015
Modelling the behaviour of microbulk Micromegas in xenon/trimethylamine gas
  • Ruiz-Choliz, E.; González-Díaz, D.; Diago, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 799 https://doi.org/10.1016/j.nima.2015.07.062
journal November 2015
Ionization fluctuations and resolution of ionization chambers and semiconductor detectors journal February 1967
Measurements of Charge and Light in Pure High Pressure Xe towards the Study of Xe+TMA Mixtures with Dark Matter Directionality Sensitivity and Supra-intrinsic Energy Resolution for 0νββ Decay Searches journal January 2015
Ionization and scintillation of nuclear recoils in gaseous xenon
  • Renner, J.; Gehman, V. M.; Goldschmidt, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 793 https://doi.org/10.1016/j.nima.2015.04.057
journal September 2015
The photophysics of tertiary aliphatic amines journal December 1981

Cited By (1)