Compression of a multiphase mantle assemblage: Effects of undesirable stress and stress annealing on the iron spin state crossover in ferropericlase: Stresses and HS-LS Crossover in (Mg,Fe)O

Glazyrin, Konstantin; Miyajima, Nobuyoshi; Smith, Jesse S.; Lee, Kanani K.  M.

doi:10.1002/2015JB012321

Title: Compression of a multiphase mantle assemblage: Effects of undesirable stress and stress annealing on the iron spin state crossover in ferropericlase: Stresses and HS-LS Crossover in (Mg,Fe)O

Journal Article · Mon May 30 00:00:00 EDT 2016 · Journal of Geophysical Research. Solid Earth

DOI:https://doi.org/10.1002/2015JB012321· OSTI ID:1379196

Glazyrin, Konstantin ^[1]; Miyajima, Nobuyoshi ^[2]; Smith, Jesse S. ^[3]; Lee, Kanani K. M. ^[4]

Yale Univ., New Haven, CT (United States). Dept. of Geology and Geophysics; Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). German Electron Synchrotron DESY in the Helmholtz Association
Univ. of Bayreuth (Germany). Geo Inst.
Carnegie Inst. of Washington, Argonne, IL (United States). Geophysical Lab.
Yale Univ., New Haven, CT (United States). Dept. of Geology and Geophysics

Using synchrotron-based X-ray diffraction, we explore characteristic signatures for nonhydrostaticstresses and their effect on the spin state crossover of ferrous iron in (Mg, Fe)O ferropericlase (Fp) uponcompression in a two-phase mixture which includes an Al- and Fe-bearing bridgmanite (Bm). Here, we observe aninfluence of nonhydrostatic stresses on the spin state crossover starting pressure and width. The undesirablestresses discussed here include uniaxial deviatoric stress evolving in the diamond anvil cell and effects ofintergrain interaction. And while the former leads to a pressure overestimation, the latter one lowers the pressure ofthe onset for the high-spin to low-spin electronic transition in Fe²⁺ in ferropericlase (Mg, Fe)O with respect tohydrostatic conditions.

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Research Organization:: Carnegie Inst. of Science, Washington, DC (United States). Geophysical Lab.

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: NA0002006; NA0001974; FG02-99ER45775; AC02-06CH11357; FG02-94ER14466; EAR-0955824

OSTI ID:: 1379196

Journal Information:: Journal of Geophysical Research. Solid Earth, Vol. 121, Issue 5; ISSN 2169-9313

Publisher:: American Geophysical UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 15 works

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Title: Compression of a multiphase mantle assemblage: Effects of undesirable stress and stress annealing on the iron spin state crossover in ferropericlase: Stresses and HS-LS Crossover in (Mg,Fe)O

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