Rotating lattice single crystal architecture on the surface of glass

Savytskii, D.; Jain, H.; Tamura, N.; Dierolf, V.

doi:10.1038/srep36449

Title: Rotating lattice single crystal architecture on the surface of glass

Journal Article · Thu Nov 03 00:00:00 EDT 2016 · Scientific Reports

DOI:https://doi.org/10.1038/srep36449· OSTI ID:1377570

Savytskii, D. ^[1]; Jain, H. ^[1]; Tamura, N. ^[2]; Dierolf, V. ^[3]

Lehigh Univ., Bethlehem, PA (United States). Materials Science and Engineering Dept.
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Lehigh Univ., Bethlehem, PA (United States). Physics Dept.

Defying the requirements of translational periodicity in 3D, rotation of the lattice orientation within an otherwise single crystal provides a new form of solid. Such rotating lattice single (RLS) crystals are found, but only as spherulitic grains too small for systematic characterization or practical application. Here we report a novel approach to fabricate RLS crystal lines and 2D layers of unlimited dimensions via a recently discovered solid-to-solid conversion process using a laser to heat a glass to its crystallization temperature but keeping it below the melting temperature. The proof-of-concept including key characteristics of RLS crystals is demonstrated using the example of Sb₂S₃ crystals within the Sb-S-I model glass system for which the rotation rate depends on the direction of laser scanning relative to the orientation of initially formed seed. Lattice rotation in this new mode of crystal growth occurs upon crystallization through a well-organized dislocation/disclination structure introduced at the glass/ crystal interface. Implications of RLS growth on biomineralization and spherulitic crystal growth are noted.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-05CH11231; SC0005010

OSTI ID:: 1377570

Journal Information:: Scientific Reports, Vol. 6, Issue 1; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 22 works

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