Evidence for strong enhancement of the magnetic ordering temperature of trivalent Nd metal under extreme pressure [Anomalous enhancement of the magnetic ordering temperature of trivalent Nd metal under extreme pressure: Possible Kondo lattice behavior]

Song, J.; Bi, W.; Haskel, D.; Schilling, J. S.

doi:10.1103/PhysRevB.95.205138

Title: Evidence for strong enhancement of the magnetic ordering temperature of trivalent Nd metal under extreme pressure [Anomalous enhancement of the magnetic ordering temperature of trivalent Nd metal under extreme pressure: Possible Kondo lattice behavior]

Journal Article · Mon May 15 00:00:00 EDT 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.95.205138· OSTI ID:1374149

Song, J. ^[1]; Bi, W. ^[2]; Haskel, D. ^[3]; Schilling, J. S. ^[1]

Washington Univ., St. Louis, MO (United States)
Argonne National Lab. (ANL), Argonne, IL (United States); Univ. of Illinois at Urbana-Champaign, Urbana, IL (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Four-point electrical resistivity measurements were carried out on Nd metal and dilute magnetic alloys containing up to 1 at.% Nd in superconducting Y for temperatures 1.5–295 K under pressures to 210 GPa. The magnetic ordering temperature T_o of Nd appears to rise steeply under pressure, increasing ninefold to 180 K at 70 GPa before falling rapidly. Y(Nd) alloys display both a resistivity minimum and superconducting pair breaking ΔT_c as large as 38 K/at.% Nd. The present results give evidence that for pressures above 30–40 GPa, the exchange coupling J between Nd ions and conduction electrons becomes negative, thus activating Kondo physics in this highly correlated electron system. Furthermore, the rise and fall of T_o and ΔT_c with pressure can be accounted for in terms of an increase in the Kondo temperature.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES); Consortium for Materials Properties Research in Earth Sciences (COMPRES)

Grant/Contract Number:: AC02-06CH11357; FC52-08NA28554

OSTI ID:: 1374149

Alternate ID(s):: OSTI ID: 1358645

Journal Information:: Physical Review B, Vol. 95, Issue 20; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 9 works

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