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Observation of stable Néel skyrmions in cobalt/palladium multilayers with Lorentz transmission electron microscopy

Journal Article · · Nature Communications
DOI:https://doi.org/10.1038/ncomms14761· OSTI ID:1372428
 [1];  [2];  [1];  [3];  [4];  [1]
  1. National Univ. of Singapore (Singapore). Dept. of Electrical and Computer Engineering
  2. Stony Brook Univ., NY (United States). Dept. of Material Science and Engineering; Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
  3. Louisiana State Univ., Baton Rouge, LA (United States). Dept. of Physics and Astronomy
  4. Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
Néel skyrmions are of high interest due to their potential applications in a variety of spintronic devices, currently accessible in ultrathin heavy metal/ferromagnetic bilayers and multilayers with a strong Dzyaloshinskii–Moriya interaction. Here in this paper we report on the direct imaging of chiral spin structures including skyrmions in an exchange-coupled cobalt/palladium multilayer at room temperature with Lorentz transmission electron microscopy, a high-resolution technique previously suggested to exhibit no Néel skyrmion contrast. Phase retrieval methods allow us to map the internal spin structure of the skyrmion core, identifying a 25 nm central region of uniform magnetization followed by a larger region characterized by rotation from in- to out-of-plane. The formation and resolution of the internal spin structure of room temperature skyrmions without a stabilizing out-of-plane field in thick magnetic multilayers opens up a new set of tools and materials to study the physics and device applications associated with chiral ordering and skyrmions.
Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
SC0012704; AC02-98CH10886
OSTI ID:
1372428
Report Number(s):
BNL--113855-2017-JA; KC0201010
Journal Information:
Nature Communications, Journal Name: Nature Communications Vol. 8; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English

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Single Chiral Skyrmions in Ultrathin Magnetic Films journal November 2018
Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems text January 2018
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Anatomy of Skyrmionic Textures in Magnetic Multilayers journal February 2019
Observation of Robust Néel Skyrmions in Metallic PtMnGa journal November 2019
In Situ Synchrotron X-Ray Diffraction Analysis of Phase Transformation in Epitaxial Metastable hcp Nickel Thin Films, Prepared via Plasma-Enhanced Atomic Layer Deposition journal October 2018
Stabilizing spin spirals and isolated skyrmions at low magnetic field exploiting vanishing magnetic anisotropy journal March 2018
Ferroelectrically tunable magnetic skyrmions in ultrathin oxide heterostructures journal November 2018
Theory of isolated magnetic skyrmions: From fundamentals to room temperature applications journal March 2018
A transmission electron microscope study of Néel skyrmion magnetic textures in multilayer thin film systems with large interfacial chiral interaction journal April 2018
Observation of magnetic skyrmions in unpatterned symmetric multilayers at room temperature and zero magnetic field journal March 2019
Direct current-tunable MHz to multi-GHz skyrmion generation and control journal July 2019
Determination of chirality and density control of Néel-type skyrmions with in-plane magnetic field journal July 2018
Controlled modification of skyrmion information in a three-terminal racetrack memory journal January 2019
Direct writing of room temperature and zero field skyrmion lattices by a scanning local magnetic field journal March 2018
Magnetic coupling of ferromagnetic SrRuO 3 epitaxial layers separated by ultrathin non-magnetic SrZrO 3 /SrIrO 3 journal November 2018
Creation of a thermally assisted skyrmion lattice in Pt/Co/Ta multilayer films journal November 2018
Spin torque nano-oscillators based on antiferromagnetic skyrmions journal January 2019
Route to form skyrmions in soft magnetic films journal August 2019
Magnetic properties of isolated skyrmion under the in-plane magnetic field and anisotropy gradient journal August 2019
Ultrafast spin dynamics and spintronics for ferrimagnets close to the spin compensation point (Review) journal September 2019
Interfacial Dzyaloshinskii-Moriya interaction between ferromagnetic insulator and heavy metal journal February 2020
Size and shape of skyrmions for variable Dzyaloshinskii–Moriya interaction and uniaxial anisotropy journal June 2018
Metastable magnetic bubble in [Co/Pd] 4 /Py multilayers journal December 2018
Trochoidal antiskyrmion motion with microwave electric fields journal August 2019
Ineffectiveness of the Dzyaloshinskii–Moriya interaction in the dynamical quantum phase transition in the ITF model journal October 2018
Skyrmion-electronics: writing, deleting, reading and processing magnetic skyrmions toward spintronic applications journal January 2020
Proposal for a micromagnetic standard problem for materials with Dzyaloshinskii–Moriya interaction journal November 2018
Current-Driven Dynamics of Frustrated Skyrmions in a Synthetic Antiferromagnetic Bilayer journal April 2019
Current-induced Out-of-plane Spin Accumulation on the (001) Surface of the Ir Mn 3 Antiferromagnet journal December 2019
Quantitative imaging of hybrid chiral spin textures in magnetic multilayer systems by Lorentz microscopy journal December 2019
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Interface Dzyaloshinskii-Moriya interaction in the interlayer antiferromagnetic-exchange coupled Pt/CoFeB/Ru/CoFeB systems journal October 2017
Spin-wave propagation in the presence of inhomogeneous Dzyaloshinskii-Moriya interactions journal November 2017
Evolution of topological skyrmions across the spin reorientation transition in Pt/Co/Ta multilayers journal May 2018
Creation of localized skyrmion bubbles in Co/Pt bilayers using a spin-valve nanopillar journal May 2018
First-principles investigation of chiral magnetic properties in multilayers: Rh/Co/Pt and Pd/Co/Pt journal October 2018
Quantifying chiral exchange interaction for Néel-type skyrmions via Lorentz transmission electron microscopy journal March 2019
Element-specific soft x-ray spectroscopy, scattering, and imaging studies of the skyrmion-hosting compound Co 8 Zn 8 Mn 4 journal April 2019
Chirality in Magnetic Multilayers Probed by the Symmetry and the Amplitude of Dichroism in X-Ray Resonant Magnetic Scattering journal January 2018
Quantification of Mixed Bloch-Néel Topological Spin Textures Stabilized by the Dzyaloshinskii-Moriya Interaction in Co / Pd Multilayers journal June 2019
Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems journal September 2019
Observation of Robust Néel Skyrmions in Metallic PtMnGa text January 2019
Spin-wave propagation in the presence of inhomogeneous Dzyaloshinskii-Moriya interactions text January 2017
Proposal for a micromagnetic standard problem for materials with Dzyaloshinskii-Moriya interaction text January 2018
Size and shape of skyrmions for variable Dzyaloshinskii-Moriya interaction and uniaxial anisotropy text January 2018
First-principles investigation of chiral magnetic properties in multilayers: Rh/Co/Pt and Pd/Co/Pt text January 2018
Metastable magnetic bubble in [Co/Pd]4/Py multilayers text January 2018
Spin torque nano-oscillators based on antiferromagnetic skyrmions text January 2018
Quantitative imaging of hybrid chiral spin textures in magnetic multilayer systems by Lorentz microscopy text January 2019
Stabilizing spin spirals and isolated skyrmions at low magnetic field exploiting vanishing magnetic anisotropy text January 2018

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