Space and time-resolved probing of heterogeneous catalysis reactions using lab-on-a-chip
- Louisiana State Univ., Baton Rouge, LA (United States); Energy Frontier Research Centers (EFRC) (United States). Center for Atomic-Level Catalyst Design (CALCD)
- Louisiana State Univ., Baton Rouge, LA (United States)
Probing catalytic reactions on a catalyst surface in real time is a major challenge. In this paper, we demonstrate the utility of a continuous flow millifluidic chip reactor coated with a nanostructured gold catalyst as an effective platform for in situ investigation of the kinetics of catalytic reactions by taking 5-(hydroxymethyl)furfural (HMF) to 2,5-furandicarboxylic acid (FDCA) conversion as a model reaction. The idea conceptualized in this paper can not only dramatically change the ability to probe the time-resolved kinetics of heterogeneous catalysis reactions but also used for investigating other chemical and biological catalytic processes, thereby making this a broad platform for probing reactions as they occur within continuous flow reactors.
- Research Organization:
- Energy Frontier Research Centers (EFRC) (United States). Center for Atomic-Level Catalyst Design (CALCD)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); Board of Regents
- Grant/Contract Number:
- SC0001058; LEQSF (2009-14)-EFRC-MATCH; LEDSF-EPS(2012)-OPT-IN-15
- OSTI ID:
- 1369711
- Journal Information:
- Nanoscale, Vol. 8, Issue 10; Related Information: CALCD partners with Louisiana State University (lead); Clemson University; University of Florida; Georgia Institute of Technology; Grambling State University; Oak Ridge National Laboratory; Ohio State University; Pennsylvania State; Texas A&M University; Vienna University of Technology, Austria; University of Utrecht, Netherlands; ISSN 2040-3364
- Publisher:
- Royal Society of ChemistryCopyright Statement
- Country of Publication:
- United States
- Language:
- English
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