Pressure-induced elastic anomaly in a polyamorphous metallic glass

Zeng, Qiaoshi; Zeng, Zhidan; Lou, Hongbo; Kono, Yoshio; Zhang, Bo; Kenney-Benson, Curtis; Park, Changyong; Mao, Wendy L.

doi:10.1063/1.4984746

Pressure-induced elastic anomaly in a polyamorphous metallic glass

Journal Article · Wed May 31 00:00:00 EDT 2017 · Applied Physics Letters

DOI:https://doi.org/10.1063/1.4984746· OSTI ID:1368293

^[1]; Zeng, Zhidan ^[1]; Lou, Hongbo ^[1]; Kono, Yoshio ^[2]; ^[3]; Kenney-Benson, Curtis ^[2]; ^[2]; Mao, Wendy L. ^[4]

Center for High Pressure Science and Technology Advanced Research (HPSTAR), Shanghai (People's Republic of China)
Carnegie Inst. of Washington, Argonne, IL (United States). Geophysical Lab., HPCAT
Hefei Univ. of Technology (China)
Stanford Univ., CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)

The pressure-induced transitions discovered in metallic glasses (MGs) have attracted considerable research interest offering an exciting opportunity to study polyamorphism in densely packed systems. Despite the large body of work on these systems, the elastic properties of the MGs during polyamorphic transitions remain unclear. Here, using an in situ high-pressure ultrasonic sound velocity technique integrated with x-ray radiography and x-ray diffraction in a Paris-Edinburgh cell, we accurately determined both the compressional and shear wave velocities of a polyamorphous Ce₆₈Al₁₀Cu₂₀Co₂ MG up to 5.8 GPa. We observed elastic anomalies of a MG with minima (at ~1.5 GPa) in the sound velocities, bulk modulus, and Poisson’s ratio during its polyamorphic transition. Finally, this behavior was discussed in comparison to the elastic anomalies of silica glass and crystalline Ce.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Laboratory. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Organization:: National Natural Science Foundation of China (NSFC); National Science Foundation (NSF); National Thousand Youth Talents Program in China; USDOE; USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-06CH11357; FG02-99ER45775; NA0001974

OSTI ID:: 1368293

Alternate ID(s):: OSTI ID: 1985542

Journal Information:: Applied Physics Letters, Journal Name: Applied Physics Letters Journal Issue: 22 Vol. 110; ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: ENGLISH

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