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Report on the Synchrotron Characterization of U-Mo and U-Zr Alloys and the Modeling Results

Technical Report ·
DOI:https://doi.org/10.2172/1364512· OSTI ID:1364512
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  1. Purdue Univ., West Lafayette, IN (United States)
  2. Illinois Inst. of Technology, Chicago, IL (United States)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States)
ABSTRACT Uranium-molybdenum (U-Mo) and uranium-zirconium (U-Zr) are two promising fuel candidates for nuclear transmutation reactors which burn long-lived minor actinides and fission products within fast spectrum reactors. The objectives of this research are centered on understanding the early stages of fuel performance through the examination of the irradiation induced microstructural changes in U-Zr and U-Mo alloys subjected to low neutron fluences. Specimens that were analyzed include those that were previously irradiated in the Advanced Test Reactor at INL. This most recent work has focused on a sub-set of the irradiated specimens, specifically U-Zr and U-Mo alloys that were irradiated to 0.01 dpa at temperatures ranging from (150-800oC). These specimens were analyzed with two types of synchrotron techniques, including X-ray absorption fine structure and X-ray diffraction. These techniques provide non-destructive microstructural analysis, including phase identification and quantitation, lattice parameters, crystallite sizes, as well as bonding, structure, and chemistry. Preliminary research has shown changes in the phase fractions, crystallite sizes, and lattice parameters as a function of irradiation and temperature. Future data analyses will continue to explore these microstructural changes.
Research Organization:
Idaho National Laboratory (INL), Idaho Falls, ID (United States)
Sponsoring Organization:
USDOE Office of Nuclear Energy (NE)
DOE Contract Number:
AC07-05ID14517;
OSTI ID:
1364512
Report Number(s):
INL/EXT--16-40130
Country of Publication:
United States
Language:
English

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