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Investigation of High-temperature Oxidation Kinetics and Residual Ductility of Oxidized Samples of Sponge-based E110 Alloy Cladding Tubes

Conference · · MRS Advances
DOI:https://doi.org/10.1557/adv.2016.641· OSTI ID:1362233

Two-sided oxidation experiments were recently conducted at 1000-1200°C in flowing steam with samples of sponge-based Zr-1Nb alloy E110. Although the old electrolytic E110 tubing exhibited a high degree of susceptibility to nodular corrosion and experienced breakaway oxidation rates in relatively short time, the new sponge-based E110 has demonstrated steam oxidation behavior comparable to Zircaloy-4. The sponge-based E110 followed the parabolic law, and the derived oxidation rate constant is in good agreement with the Cathcart-Pawel (CP) correlation at 1100-1200°C. For 1000°C oxidation, the weight-gain of sponge-based E110 is much lower than Zircaloy-4. No breakaway oxidation was observed at 1000°C up to 8000 s. Ring compression tests were conducted to evaluate the residual ductility of oxidized samples at room temperature and at 135°C. All sponge-based E110 specimens were still ductile at 135°C after being oxidized up to 20% equivalent cladding reacted at 1000-1200°C. Metallographic examinations were performed on oxidized E110 specimens to correlate material performance with microstructure.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
1362233
Journal Information:
MRS Advances, Journal Name: MRS Advances Journal Issue: 21-22 Vol. 2; ISSN 2059-8521
Publisher:
Springer Nature
Country of Publication:
United States
Language:
English

References (5)

Advanced Zirconium Alloy for PWR Application journal January 2010
Cladding embrittlement during postulated loss-of-coolant accidents report July 2008
Ultra Low Tin Quaternary Alloys PWR Performance—Impact of Tin Content on Corrosion Resistance, Irradiation Growth, and Mechanical Properties journal January 2011
Zirconium metal-water oxidation kinetics. IV. Reaction rate studies. [BWR:PWR] report July 1977
High-temperature steam-oxidation behavior of Zr-1Nb cladding alloy E110 journal September 2009

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