Impact of biogenic very short-lived bromine on the Antarctic ozone hole during the 21st century

Fernandez, Rafael P.; Kinnison, Douglas E.; Lamarque, Jean -Francois; Tilmes, Simone; Saiz-Lopez, Alfonso

doi:10.5194/acp-17-1673-2017

Title: Impact of biogenic very short-lived bromine on the Antarctic ozone hole during the 21st century

Journal Article · Fri Feb 03 00:00:00 EST 2017 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-17-1673-2017· OSTI ID:1358422

^[1]; Kinnison, Douglas E. ^[2]; Lamarque, Jean -Francois ^[2]; Tilmes, Simone ^[2]; Saiz-Lopez, Alfonso ^[3]

Institute of Physical Chemistry Rocasolano, Madrid (Spain); National Research Council (CONICET); Mendoza (Argentina)
National Center for Atmospheric Research, Boulder, CO (United States)
Institute of Physical Chemistry Rocasolano, Madrid (Spain)

Active bromine released from the photochemical decomposition of biogenic very short-lived bromocarbons (VSL^Br) enhances stratospheric ozone depletion. Based on a dual set of 1960–2100 coupled chemistry–climate simulations (i.e. with and without VSL^Br), we show that the maximum Antarctic ozone hole depletion increases by up to 14 % when natural VSL^Br are considered, which is in better agreement with ozone observations. The impact of the additional 5 pptv VSL^Br on Antarctic ozone is most evident in the periphery of the ozone hole, producing an expansion of the ozone hole area of ~5 million km², which is equivalent in magnitude to the recently estimated Antarctic ozone healing due to the implementation of the Montreal Protocol. We find that the inclusion of VSL^Br in CAM-Chem (Community Atmosphere Model with Chemistry, version 4.0) does not introduce a significant delay of the modelled ozone return date to 1980 October levels, but instead affects the depth and duration of the simulated ozone hole. Our analysis further shows that total bromine-catalysed ozone destruction in the lower stratosphere surpasses that of chlorine by the year 2070 and indicates that natural VSL^Br chemistry would dominate Antarctic ozone seasonality before the end of the 21st century. As a result, this work suggests a large influence of biogenic bromine on the future Antarctic ozone layer.

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Research Organization:: Institute for Advanced Study, Princeton, NJ (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER)

Grant/Contract Number:: SC0009988

OSTI ID:: 1358422

Journal Information:: Atmospheric Chemistry and Physics (Online), Vol. 17, Issue 3; ISSN 1680-7324

Publisher:: European Geosciences UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 35 works

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09 BIOMASS FUELS
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Title: Impact of biogenic very short-lived bromine on the Antarctic ozone hole during the 21st century

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