Anisotropic high-harmonic generation in bulk crystals

You, Yong Sing; Reis, David A.; Ghimire, Shambhu

doi:10.1038/NPHYS3955

Title: Anisotropic high-harmonic generation in bulk crystals

Journal Article · Mon Nov 21 00:00:00 EST 2016 · Nature Physics

DOI:https://doi.org/10.1038/NPHYS3955· OSTI ID:1352542

You, Yong Sing ^[1]; Reis, David A. ^[2]; Ghimire, Shambhu ^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)

The microscopic valence electron density determines the optical, electronic, structural and thermal properties of materials. However, current techniques for measuring this electron charge density are limited: for example, scanning tunnelling microscopy is confined to investigations at the surface, and electron diffraction requires very thin samples to avoid multiple scattering. Therefore, an optical method is desirable for measuring the valence charge density of bulk materials. Since the discovery of high-harmonic generation (HHG) in solids, there has been growing interest in using HHG to probe the electronic structure of solids. Here, using single-crystal MgO, we demonstrate that high-harmonic generation in solids is sensitive to interatomic bonding. We find that harmonic efficiency is enhanced (diminished) for semi-classical electron trajectories that connect (avoid) neighbouring atomic sites in the crystal. Finally, these results indicate the possibility of using materials’ own electrons for retrieving the interatomic potential and thus the valence electron density, and perhaps even wavefunctions, in an all-optical setting.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1352542

Journal Information:: Nature Physics, Vol. 13, Issue 4; ISSN 1745-2473

Publisher:: Nature Publishing Group (NPG)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 300 works

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Journal Article · Tue May 17 00:00:00 EDT 2011 · Accounts of Chemical Research, 44(5):360-368 · OSTI ID:1352542

Feng, Min; Zhao, Jin; Huang, Tian; +2 more

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