Ultrafast Independent N–H and N–C Bond Deformation Investigated with Resonant Inelastic X-Ray Scattering

Eckert, Sebastian; Norell, Jesper; Miedema, Piter S.; Beye, Martin; Fondell, Mattis; Quevedo, Wilson; Kennedy, Brian; Hantschmann, Markus; Pietzsch, Annette; Van?Kuiken, Benjamin E.; Ross, Matthew; Minitti, Michael P.; Moeller, Stefan P.; Schlotter, William F.; Khalil, Munira; Odelius, Michael; F?hlisch, Alexander

doi:10.1002/anie.201700239

Ultrafast Independent N–H and N–C Bond Deformation Investigated with Resonant Inelastic X-Ray Scattering

Journal Article · Tue Apr 04 00:00:00 EDT 2017 · Angewandte Chemie (International Edition)

DOI:https://doi.org/10.1002/anie.201700239· OSTI ID:1352452

^[1]; Norell, Jesper ^[2]; ^[3]; ^[3]; Fondell, Mattis ^[3]; Quevedo, Wilson ^[3]; Kennedy, Brian ^[3]; Hantschmann, Markus ^[3]; ^[3]; ^[4]; ^[4]; Minitti, Michael P. ^[5]; Moeller, Stefan P. ^[5]; Schlotter, William F. ^[5]; ^[4]; ^[2]; ^[1]

Institut f?r Physik und Astronomie, Universit?t Potsdam, Karl-Liebknecht-Strasse 24/25 14476 Potsdam Germany, Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin f?r Materialien und Energie GmbH, Albert-Einstein-Strasse 15 12489 Berlin Germany
Department of Physics, Stockholm University, AlbaNova University Center 10691 Stockholm Sweden
Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin f?r Materialien und Energie GmbH, Albert-Einstein-Strasse 15 12489 Berlin Germany
Department of Chemistry, University of Washington, Seattle WA 98195 USA
LCLS, SLAC National Accelerator Laboratory, 2575 Sand Hill Road Menlo Park CA 94025 USA

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Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0002190; AC02-76SF00515; AC02-76SF00515

OSTI ID:: 1352452

Alternate ID(s):: OSTI ID: 1352454
OSTI ID: 1368690

Journal Information:: Angewandte Chemie (International Edition), Journal Name: Angewandte Chemie (International Edition) Journal Issue: 22 Vol. 56; ISSN 1433-7851

Publisher:: WileyCopyright Statement

Country of Publication:: Germany

Language:: English

References (25)

Molcas 8: New capabilities for multiconfigurational quantum chemical calculations across the periodic table : Molcas 8 Aquilante, Francesco; Autschbach, Jochen; Carlson, Rebecca K. Journal of Computational Chemistry, Vol. 37, Issue 5 https://doi.org/10.1002/jcc.24221	journal	November 2015
Molecular structures and protonation state of 2-Mercaptopyridine in aqueous solution Eckert, S.; Miedema, P. S.; Quevedo, W. Chemical Physics Letters, Vol. 647 https://doi.org/10.1016/j.cplett.2016.01.050	journal	March 2016
Intersystem Crossing Pathways in the Noncanonical Nucleobase 2-Thiouracil: A Time-Dependent Picture Mai, Sebastian; Marquetand, Philipp; González, Leticia The Journal of Physical Chemistry Letters, Vol. 7, Issue 11 https://doi.org/10.1021/acs.jpclett.6b00616	journal	May 2016
Energies and alkylations of tautomeric heterocyclic compounds: old problems - new answers Beak, Peter Accounts of Chemical Research, Vol. 10, Issue 5 https://doi.org/10.1021/ar50113a006	journal	May 1977
The restricted active space self-consistent-field method, implemented with a split graph unitary group approach Malmqvist, Per Aake.; Rendell, Alistair.; Roos, Bjoern O. The Journal of Physical Chemistry, Vol. 94, Issue 14 https://doi.org/10.1021/j100377a011	journal	July 1990
Solvent effects on protomeric equilibriums: quantitative correlation with an electrostatic hydrogen-bonding model Beak, Peter; Covington, Johnny B. Journal of the American Chemical Society, Vol. 100, Issue 12 https://doi.org/10.1021/ja00480a069	journal	June 1978
Convergent Proton-Transfer Photocycles Violate Mirror-Image Symmetry in a Key Melanin Monomer Olsen, Seth; Riesz, Jennifer; Mahadevan, Indu Journal of the American Chemical Society, Vol. 129, Issue 21 https://doi.org/10.1021/ja069280u	journal	May 2007
Superior Photoprotective Motifs and Mechanisms in Eumelanins Uncovered Corani, Alice; Huijser, Annemarie; Gustavsson, Thomas Journal of the American Chemical Society, Vol. 136, Issue 33 https://doi.org/10.1021/ja501499q	journal	August 2014
2,4-Dithiothymine as a Potent UVA Chemotherapeutic Agent Pollum, Marvin; Jockusch, Steffen; Crespo-Hernández, Carlos E. Journal of the American Chemical Society, Vol. 136, Issue 52 https://doi.org/10.1021/ja510611j	journal	December 2014
UV-Induced Proton Transfer between DNA Strands Zhang, Yuyuan; de La Harpe, Kimberly; Beckstead, Ashley A. Journal of the American Chemical Society, Vol. 137, Issue 22 https://doi.org/10.1021/jacs.5b03914	journal	June 2015
Displacement of protomeric equilibriums by self-association: hydroxypyridine-pyridone and mercaptopyridine-thiopyridone isomer pairs Beak, Peter; Covington, Johnny B.; Smith, Stanley G. The Journal of Organic Chemistry, Vol. 45, Issue 8 https://doi.org/10.1021/jo01296a002	journal	April 1980
Excited-State Dynamics in 6-Thioguanosine from the Femtosecond to Microsecond Time Scale Reichardt, Christian; Guo, Cao; Crespo-Hernández, Carlos E. The Journal of Physical Chemistry B, Vol. 115, Issue 12 https://doi.org/10.1021/jp112018u	journal	March 2011
Resonance Raman Spectroscopic and Theoretical Investigation of the Excited State Proton Transfer Reaction Dynamics of 2-Thiopyridone Du, Rui; Liu, Chong; Zhao, Yanying The Journal of Physical Chemistry B, Vol. 115, Issue 25 https://doi.org/10.1021/jp203185a	journal	June 2011
Ultrafast Proton Dynamics in Aqueous Amino Acid Solutions Studied by Resonant Inelastic Soft X-ray Scattering Blum, M.; Odelius, M.; Weinhardt, L. The Journal of Physical Chemistry B, Vol. 116, Issue 46 https://doi.org/10.1021/jp302958j	journal	November 2012
Information Content in O[1s] K-edge X-ray Emission Spectroscopy of Liquid Water Odelius, Michael The Journal of Physical Chemistry A, Vol. 113, Issue 29 https://doi.org/10.1021/jp903096k	journal	July 2009
Photochemistry of Pheomelanin Building Blocks and Model Chromophores: Excited-State Intra- and Intermolecular Proton Transfer El Nahhas, Amal; Pascher, Torbjörn; Leone, Loredana The Journal of Physical Chemistry Letters, Vol. 5, Issue 12 https://doi.org/10.1021/jz500720g	journal	June 2014
Orbital-specific mapping of the ligand exchange dynamics of Fe(CO)5 in solution Wernet, Ph.; Kunnus, K.; Josefsson, I. Nature, Vol. 520, Issue 7545 https://doi.org/10.1038/nature14296	journal	April 2015
Increase in the photoreactivity of uracil derivatives by doubling thionation Pollum, M.; Jockusch, S.; Crespo-Hernández, C. E. Phys. Chem. Chem. Phys., Vol. 17, Issue 41 https://doi.org/10.1039/C5CP04822B	journal	January 2015
Probing hydrogen bonding orbitals: resonant inelastic soft X-ray scattering of aqueous NH ₃ Weinhardt, L.; Ertan, E.; Iannuzzi, M. Physical Chemistry Chemical Physics, Vol. 17, Issue 40 https://doi.org/10.1039/C5CP04898B	journal	January 2015
The restricted active space followed by second-order perturbation theory method: Theory and application to the study of CuO2 and Cu2O2 systems Malmqvist, Per Åke; Pierloot, Kristine; Shahi, Abdul Rehaman Moughal The Journal of Chemical Physics, Vol. 128, Issue 20 https://doi.org/10.1063/1.2920188	journal	May 2008
Communication: The dark singlet state as a doorway state in the ultrafast and efficient intersystem crossing dynamics in 2-thiothymine and 2-thiouracil Pollum, Marvin; Crespo-Hernández, Carlos E. The Journal of Chemical Physics, Vol. 140, Issue 7 https://doi.org/10.1063/1.4866447	journal	February 2014
Dynamics of the OH group and the electronic structure of liquid alcohols Schreck, Simon; Pietzsch, Annette; Kunnus, Kristjan Structural Dynamics, Vol. 1, Issue 5 https://doi.org/10.1063/1.4897981	journal	September 2014
X-ray resonant scattering involving dissociative states Gelmukhanov, Faris; Ågren, Hans Physical Review A, Vol. 54, Issue 1 https://doi.org/10.1103/PhysRevA.54.379	journal	July 1996
Spatial Quantum Beats in Vibrational Resonant Inelastic Soft X-Ray Scattering at Dissociating States in Oxygen Pietzsch, A.; Sun, Y. -P.; Hennies, F. Physical Review Letters, Vol. 106, Issue 15 https://doi.org/10.1103/PhysRevLett.106.153004	journal	April 2011
Resonant inelastic x-ray scattering studies of elementary excitations Ament, Luuk J. P.; van Veenendaal, Michel; Devereaux, Thomas P. Reviews of Modern Physics, Vol. 83, Issue 2 https://doi.org/10.1103/RevModPhys.83.705	journal	June 2011

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