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Nodeless multiband superconductivity in stoichiometric single-crystalline CaKFe4As4

Journal Article · · Physical Review B
Measurements of the London penetration depth Δλ(T) and tunneling conductance in single crystals of the recently discovered stoichiometric iron-based superconductor CaKFe4As4 (CaK1144) show nodeless, two-effective-gap superconductivity with a larger gap of about 6–10 meV and a smaller gap of about 1–4 meV. Having a critical temperature Tc,onset ≈ 35.8 K, this material behaves similar to slightly overdoped (Ba1–xKx)Fe2As2 (e.g., x = 0.54,Tc ≈ 34 K), a known multigap s± superconductor. Here, we conclude that the superconducting behavior of stoichiometric CaK1144 demonstrates that two-gap s± superconductivity is an essential property of high-temperature superconductivity in iron-based superconductors, independent of the degree of substitutional disorder.
Research Organization:
Ames Laboratory (AMES), Ames, IA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
AC02-07CH11358
OSTI ID:
1350068
Alternate ID(s):
OSTI ID: 1346271
Report Number(s):
IS-J--9232
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 10 Vol. 95; ISSN 2469-9950; ISSN PRBMDO
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (47)

Magnetic Penetration Depth in Unconventional Superconductors journal January 2007
Scanning tunneling spectroscopy in MgB2 journal March 2003
Using gap symmetry and structure to reveal the pairing mechanism in Fe-based superconductors journal January 2016
STM study of multiband superconductivity in NbSe2 using a superconducting tip journal May 2004
Scanning tunneling spectroscopy with superconducting tips of Al journal April 2008
New-Structure-Type Fe-Based Superconductors: Ca A Fe 4 As 4 ( A = K, Rb, Cs) and Sr A Fe 4 As 4 ( A = Rb, Cs) journal March 2016
Superconductivity gets an iron boost journal March 2010
High-temperature superconductivity in iron-based materials journal August 2010
Observation of ordered vortices with Andreev bound states in Ba0.6K0.4Fe2As2 journal February 2011
Measurements of the absolute value of the penetration depth in high-Tc superconductors using a low-Tc superconductive coating journal December 2000
Compact very low temperature scanning tunneling microscope with mechanically driven horizontal linear positioning stage journal March 2011
The puzzle of high temperature superconductivity in layered iron pnictides and chalcogenides journal October 2010
London penetration depth in iron-based superconductors journal September 2011
Spectroscopic scanning tunneling microscopy insights into Fe-based superconductors journal November 2011
Magnetic penetration depth in unconventional superconductors journal June 2006
Imaging superconducting vortex cores and lattices with a scanning tunneling microscope journal May 2014
Observation of unreconstructed square atomic square lattice in Ca(Fe 0.965 Co 0.035 ) 2 As 2 cleaved at very low temperatures journal December 2014
Effect of strong scattering on the low-temperature penetration depth of a d -wave superconductor journal August 1993
Geometric barrier and current string in type-II superconductors obtained from continuum electrodynamics journal February 1999
Meissner-London state in superconductors of rectangular cross section in a perpendicular magnetic field journal July 2000
Nanoscale superconducting-gap variations and lack of phase separation in optimally doped BaFe 1.86 Co 0.14 As 2 journal June 2009
Superfluid density and specific heat within a self-consistent scheme for a two-band superconductor journal July 2009
Pair breaking in iron pnictides journal December 2009
Disorder-induced transition between s ± and s + + states in two-band superconductors journal November 2011
Rutgers relation for the analysis of superfluid density in superconductors journal June 2013
London penetration depth and pair breaking journal December 2013
Comprehensive scenario for single-crystal growth and doping dependence of resistivity and anisotropic upper critical fields in (Ba 1 − x K x )Fe 2 As 2 ( 0.22 ≤ x ≤ 1 ) journal April 2014
Competition between superconductivity and magnetic/nematic order as a source of anisotropic superconducting gap in underdoped Ba 1 − x K x Fe 2 As 2 journal July 2014
Interband coupling and nonmagnetic interband scattering in ± s superconductors journal June 2016
Anisotropic thermodynamic and transport properties of single-crystalline CaKFe 4 As 4 journal August 2016
Superconducting Density of States and Vortex Cores of 2H- NbS 2 journal October 2008
Tunneling Spectroscopy in Small Grains of Superconducting MgB 2 journal June 2001
Scanning tunneling spectroscopy of high-temperature superconductors journal March 2007
Superconductivity in iron compounds journal December 2011
Energy gap evolution across the superconductivity dome in single crystals of (Ba 1− x K x )Fe 2 As 2 journal September 2016
A Sharp Peak of the Zero-Temperature Penetration Depth at Optimal Composition in BaFe2(As1-xPx)2 journal June 2012
Pairing Mechanism in Fe-Based Superconductors journal March 2012
FeAs-Based Superconductivity: A Case Study of the Effects of Transition Metal Doping on BaFe 2 As 2 journal August 2010
Superfluid density and specific heat within self-consistent scheme for two-band superconductor text January 2009
FeAs-based superconductivity: a case study of the effects of transition metal doping on BaFe2As2 text January 2010
High-temperature superconductivity in iron-based materials text January 2010
Disorder induced transition between s_+- and s_++ states in two-band superconductors text January 2011
Superconductivity in Iron Compounds text January 2011
Spectroscopic scanning tunneling microscopy insights into Fe-based superconductors text January 2012
Using Gap Symmetry and Structure to Reveal the Pairing Mechanism in Fe-based Superconductors text January 2015
Energy Gap Evolution Across the Superconductivity Dome in Single Crystals of (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ text January 2016
Magnetic Penetration Depth in Unconventional Superconductors text January 2006

Cited By (24)

Electronic Properties and Fermi Surface for New Layered High-Temperature Superconductors CaAFe4As4 (A = K, Rb, and Cs): FLAPW-GGA Calculations journal November 2017
A brief review on μSR studies of unconventional Fe- and Cr-based superconductors journal October 2018
Effect of pressure on the self-hole-doped superconductor RbGd 2 Fe 4 As 4 O 2 journal December 2018
Chemical stability and superconductivity in Ag-sheathed CaKFe 4 As 4 superconducting tapes journal November 2018
Evaluation of a practical level of critical current densities in pnictides and recently discovered superconductors journal July 2019
Optimization of superconducting properties of the stoichiometric CaKFe 4 As 4 journal December 2019
Measuring the Lower Critical Field of Superconductors Using Nitrogen-Vacancy Centers in Diamond Optical Magnetometry journal January 2019
Analysis of the London penetration depth in Ni-doped CaKFe 4 As 4 journal September 2019
Signature of multigap nodeless superconductivity in CaKFe 4 As 4 journal April 2017
Electronic properties, low-energy Hamiltonian, and superconducting instabilities in CaKFe 4 As 4 journal September 2017
Magnetic fluctuations and superconducting properties of CaKFe 4 As 4 studied by As 75 NMR journal September 2017
NMR study of the new magnetic superconductor CaK ( Fe 0.951 Ni 0.049 ) 4 As 4 : Microscopic coexistence of the hedgehog spin-vortex crystal and superconductivity journal December 2017
Influence of multiband sign-changing superconductivity on vortex cores and vortex pinning in stoichiometric high- T c   CaKFe 4 As 4 journal April 2018
In-plane magnetic penetration depth of superconducting CaKFe 4 As 4 journal April 2018
Robust s ± pairing in CaK ( Fe 1 − x Ni x ) 4 As 4 ( x = 0 and 0.05) from the response to electron irradiation journal April 2018
Antiferromagnetic order in CaK ( Fe 1 − x Ni x ) 4 As 4 and its interplay with superconductivity journal June 2018
Large and significantly anisotropic critical current density induced by planar defects in CaKFe 4 As 4 single crystals journal March 2019
Anisotropy induced vortex lattice rearrangement in CaKFe 4 As 4 journal April 2019
Odd and Even Modes of Neutron Spin Resonance in the Bilayer Iron-Based Superconductor CaKFe 4 As 4 journal June 2018
Hedgehog Spin-Vortex Crystal Antiferromagnetic Quantum Criticality in CaK ( Fe 1 − x Ni x ) 4 As 4 Revealed by NMR journal September 2018
Diamagnetic Response of Potassium-Adsorbed Multilayer FeSe Film journal December 2019
Ultrahigh critical current densities, the vortex phase diagram, and the effect of granularity of the stoichiometric high- T c superconductor CaKFe 4 As 4 journal July 2018
75As NMR Studies of Magnetic Properties of the Magnetic Superconductor CaK(Fe0.967Ni0.033)4As4 journal April 2019
A brief review on muSR studies of unconventional Fe and Cr-based superconductors text January 2018

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