Resonant inelastic X-ray scattering study of spin-wave excitations in the cuprate parent compound Ca2CuO2Cl2

Lebert, B. W.; Dean, M.; Nicolaou, A.; Pelliciari, J.; Dantz, M.; Schmitt, T.; Yu, R.; Azuma, M.; Castellan, J. -P.; Miao, H.; Gauzzi, A.; Baptiste, B.; d'Astuto, Matteo

doi:10.1103/PhysRevB.95.155110

Title: Resonant inelastic X-ray scattering study of spin-wave excitations in the cuprate parent compound Ca₂CuO₂Cl₂

Journal Article · Fri Apr 07 00:00:00 EDT 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.95.155110· OSTI ID:1348292

Lebert, B. W. ^[1]; Dean, M. ^[2]; Nicolaou, A. ^[3]; Pelliciari, J. ^[4]; Dantz, M. ^[4]; Schmitt, T. ^[4]; Yu, R. ^[5]; Azuma, M. ^[5]; Castellan, J. -P. ^[6]; Miao, H. ^[2]; Gauzzi, A. ^[7]; Baptiste, B. ^[7]; d'Astuto, Matteo ^[7]

Univ. Pierre et Marie Curie, Paris (France); Synchrotron SOLEIL, Gif-sur-Yvette Cedex (France)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Synchrotron SOLEIL, Gif-sur-Yvette Cedex (France)
Paul Scherrer Inst. (PSI), Villigen (Switzerland)
Tokyo Institute of Technology, Yokohama (Japan)
CEA-Saclay, Gif-sur-Yvette (France); Karlsruhe Institute of Technology, Karlsruhe (Germany)
Univ. Pierre et Marie Curie, Paris (France)

By means of resonant inelastic x-ray scattering at the Cu L₃ edge, we measured the spin wave dispersion along <100> and <110> in the undoped cuprate Ca₂CuO₂Cl₂. The data yields a reliable estimate of the superexchange parameter J = 135 ± 4 meV using a classical spin-1/2 2D Heisenberg model with nearest-neighbor interactions and including quantum fluctuations. Including further exchange interactions increases the estimate to J = 141 meV. The 40 meV dispersion between the magnetic Brillouin zone boundary points (1/2, 0) and (1/4, 1/4) indicates that next-nearest neighbor interactions in this compound are intermediate between the values found in La₂CuO₄ and Sr₂CuO₂Cl₂. Here by owing to the low-Z elements composing Ca₂CuOCl₂, the present results may enable a reliable comparison with the predictions of quantum many-body calculations, which would improve our understanding of the role of magnetic excitations and of electronic correlations in cuprates.

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Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC00112704; 1047478

OSTI ID:: 1348292

Alternate ID(s):: OSTI ID: 1350791

Report Number(s):: BNL-113677-2017-JA; R&D Project: PO011; KC0201060; TRN: US1700546

Journal Information:: Physical Review B, Vol. 95, Issue 15; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 3 works

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Cited By (2)

Influence of apical oxygen on the extent of in-plane exchange interaction in cuprate superconductors Peng, Y. Y.; Dellea, G.; Minola, M. Nature Physics, Vol. 13, Issue 12 https://doi.org/10.1038/nphys4248	journal	August 2017
Influence of apical oxygen on the extent of in-plane exchange interaction in cuprate superconductors Peng, Y. Y.; Dellea, G.; Minola, M. arXiv https://doi.org/10.48550/arxiv.1609.05405	text	January 2016

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Title: Resonant inelastic X-ray scattering study of spin-wave excitations in the cuprate parent compound Ca₂CuO₂Cl₂