Quasi-two-dimensional Bose-Einstein condensation of spin triplets in the dimerized quantum magnet
- Tokyo Institute of Technology, Tokyo (Japan)
- Univ. of Tokyo, Chiba (Japan)
- IFW Dresden, Dresden (Germany); Technical Univ. Dresden, Dresden (Germany)
- Ehime Univ., Ehime (Japan)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sorbonne Univ., Univ. Pierre et Marie Curie - Paris 6, Paris (France)
- Aix-Marseille Univ., Marseille Cedex 9 (France)
We synthesized single crystals of composition Ba2CuSi2O6Cl2 and investigated their quantum magnetic properties. The crystal structure is closely related to that of the quasi-two-dimensional (2D) dimerized magnet BaCuSi2O6 also known as Han purple. Ba2CuSi2O6Cl2 has a singlet ground state with an excitation gap of Δ/kB = 20.8 K. The magnetization curves for two different field directions almost perfectly coincide when normalized by the g factor except for a small jump anomaly for a magnetic field perpendicular to the c axis. The magnetization curve with a nonlinear slope above the critical field is in excellent agreement with exact-diagonalization calculations based on a 2D coupled spin-dimer model. Individual exchange constants are also evaluated using density functional theory (DFT). The DFT results demonstrate a 2D exchange network and weak frustration between interdimer exchange interactions, supported by weak spin-lattice coupling implied from our magnetostriction data. Lastly, the magnetic-field-induced spin ordering in Ba2CuSi2O6Cl2 is described as the quasi-2D Bose-Einstein condensation of triplets.
- Research Organization:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Organization:
- USDOE
- Grant/Contract Number:
- AC52-06NA25396
- OSTI ID:
- 1343717
- Alternate ID(s):
- OSTI ID: 1325607
- Report Number(s):
- LA-UR-16-28415; PRBMDO; TRN: US1701625
- Journal Information:
- Physical Review B, Vol. 94, Issue 9; ISSN 2469-9950
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
Web of Science
Triplon band splitting and topologically protected edge states in the dimerized antiferromagnet
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journal | May 2019 |
Magnetic dimerization in the frustrated spin ladder
|
journal | November 2017 |
Fiber Bragg Grating Dilatometry in Extreme Magnetic Field and Cryogenic Conditions
|
journal | November 2017 |
Triplon band splitting and topologically protected edge states in the dimerized antiferromagnet | text | January 2018 |
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