Mixed cation FA x PEA 1- x PbI 3 with enhanced phase and ambient stability toward high-performance perovskite solar cells

Li, Nan; Zhu, Zonglong; Chueh, Chu -Chen; Liu, Hongbin; Peng, Bo; Petrone, Alessio; Li, Xiaosong; Wang, Liduo; Jen, Alex K. -Y.

doi:10.1002/aenm.201601307

Mixed cation FA _x PEA _1- _x PbI ₃ with enhanced phase and ambient stability toward high-performance perovskite solar cells

Journal Article · Mon Sep 26 00:00:00 EDT 2016 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201601307· OSTI ID:1343600

Li, Nan ^[1]; Zhu, Zonglong ^[2]; Chueh, Chu -Chen ^[2]; Liu, Hongbin ^[2]; Peng, Bo ^[2]; Petrone, Alessio ^[2]; Li, Xiaosong ^[2]; Wang, Liduo ^[3]; Jen, Alex K. -Y. ^[2]

Univ. of Washington, Seattle, WA (United States); Tsinghua Univ., Beijing (China); University of Washington
Univ. of Washington, Seattle, WA (United States)
Tsinghua Univ., Beijing (China)

In this study, different from the commonly explored strategy of incorporating a smaller cation, MA⁺ and Cs⁺ into FAPbI₃ lattice to improve efficiency and stability, it is revealed that the introduction of phenylethylammonium iodide (PEAI) into FAPbI₃ perovksite to form mixed cation FA_xPEA_1–xPbI₃ can effectively enhance both phase and ambient stability of FAPbI₃ as well as the resulting performance of the derived devices. From our experimental and theoretical calculation results, it is proposed that the larger PEA cation is capable of assembling on both the lattice surface and grain boundaries to form quais-3D perovskite structures. The surrounding of PEA⁺ ions at the crystal grain boundaries not only can serve as molecular locks to tighten FAPbI₃ domains but also passivate the surface defects to improve both phase and moisture stablity. Consequently, a high-performance (PCE:17.7%) and ambient stable FAPbI₃ solar cell could be developed

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Washington, Seattle, WA (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Contributing Organization:: This work was supported by the Office of Naval Research (N00014- 14-1-0246), the Asian Office of Aerospace R&D (FA2386-15-1-4106), the Department of Energy SunShot (DE-EE0006710 ) and the National Natural Science Foundation of China under Grant No. 51273104 and 91433205. A.K.-Y.J. thanks the Boeing-Johnson Foundation for financial support. Computations were conducted through the use of advanced computational, storage, and networking infrastructure provided by the Hyak supercomputer system at the University of Washington, funded by the Student Technology Fee. N.L. thanks China Scholarship Council (201506210171) for financial support. Theoretical research is supported by the National Science Foundation (CHE-1464497 and CHE-1565520 to X.L.).

Grant/Contract Number:: EE0006710

OSTI ID:: 1343600

Report Number(s):: DOE-UW-Jen--29

Journal Information:: Advanced Energy Materials, Journal Name: Advanced Energy Materials Journal Issue: 1 Vol. 7; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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High-Performance Planar Perovskite Solar Cells Using Low Temperature, Solution-Combustion-Based Nickel Oxide Hole Transporting Layer with Efficiency Exceeding 20% Liu, Ziye; Chang, Jingjing; Lin, Zhenhua Advanced Energy Materials, Vol. 8, Issue 19 https://doi.org/10.1002/aenm.201703432	journal	March 2018
Stable Formamidinium-Based Perovskite Solar Cells via In Situ Grain Encapsulation Liu, Tanghao; Zhou, Yuanyuan; Li, Zhen Advanced Energy Materials, Vol. 8, Issue 22 https://doi.org/10.1002/aenm.201800232	journal	May 2018
Low-Dimensional Perovskites: From Synthesis to Stability in Perovskite Solar Cells Yusoff, Abd. Rashid bin Mohd.; Nazeeruddin, Mohammad Khaja Advanced Energy Materials, Vol. 8, Issue 26 https://doi.org/10.1002/aenm.201801726	journal	September 2018
High‐Performance Perovskite Solar Cells with Enhanced Environmental Stability Based on a ( p ‐FC ₆ H ₄ C ₂ H ₄ NH ₃ ) ₂ [PbI ₄ ] Capping Layer Zhou, Qin; Liang, Lusheng; Hu, Junjie Advanced Energy Materials, Vol. 9, Issue 12 https://doi.org/10.1002/aenm.201802595	journal	January 2019
Improved Efficiency and Stability of Pb/Sn Binary Perovskite Solar Cells Fabricated by Galvanic Displacement Reaction Zhu, Zonglong; Li, Nan; Zhao, Dongbin Advanced Energy Materials, Vol. 9, Issue 7 https://doi.org/10.1002/aenm.201802774	journal	January 2019
A Review on Additives for Halide Perovskite Solar Cells Liu, Shuang; Guan, Yanjun; Sheng, Yusong Advanced Energy Materials, Vol. 10, Issue 13 https://doi.org/10.1002/aenm.201902492	journal	April 2020
Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells Kim, Min; Figueroa‐Tapia, Jetsabel M.; Prato, Mirko Advanced Energy Materials, Vol. 10, Issue 8 https://doi.org/10.1002/aenm.201903221	journal	January 2020
Chemical Approaches for Stabilizing Perovskite Solar Cells Lee, Jin‐Wook; Park, Nam‐Gyu Advanced Energy Materials, Vol. 10, Issue 1 https://doi.org/10.1002/aenm.201903249	journal	November 2019
The Second Spacer Cation Assisted Growth of a 2D Perovskite Film with Oriented Large Grain for Highly Efficient and Stable Solar Cells Lian, Xiaomei; Chen, Jiehuan; Qin, Minchao Angewandte Chemie International Edition, Vol. 58, Issue 28 https://doi.org/10.1002/anie.201902959	journal	May 2019
Effects of Self-Assembled Monolayer Modification of Nickel Oxide Nanoparticles Layer on the Performance and Application of Inverted Perovskite Solar Cells Wang, Qin; Chueh, Chu-Chen; Zhao, Ting ChemSusChem, Vol. 10, Issue 19 https://doi.org/10.1002/cssc.201701262	journal	September 2017
Two‐Dimensional Halide Perovskites in Solar Cells: 2D or not 2D? Ortiz‐Cervantes, Carmen; Carmona‐Monroy, Paulina; Solis‐Ibarra, Diego ChemSusChem, Vol. 12, Issue 8 https://doi.org/10.1002/cssc.201802992	journal	March 2019
Low‐dimensional metal halide perovskites and related optoelectronic applications Zhu, Pengchen; Zhu, Jia InfoMat, Vol. 2, Issue 2 https://doi.org/10.1002/inf2.12086	journal	February 2020
2D and Quasi‐2D Halide Perovskites: Applications and Progress Kim, Hyojung; Huynh, Kim Anh; Kim, Soo Young physica status solidi (RRL) – Rapid Research Letters, Vol. 14, Issue 2 https://doi.org/10.1002/pssr.201900435	journal	September 2019
2D and Quasi‐2D Halide Perovskites: Applications and Progress Kim, Hyojung; Huynh, Kim Anh; Kim, Soo Young physica status solidi (RRL) – Rapid Research Letters, Vol. 14, Issue 2 https://doi.org/10.1002/pssr.202070015	journal	September 2019
Formamidinium-Based Lead Halide Perovskites: Structure, Properties, and Fabrication Methodologies Li, Yang; Liu, Fang Zhou; Waqas, Muhammud Small Methods, Vol. 2, Issue 7 https://doi.org/10.1002/smtd.201700387	journal	May 2018
A Review on Reducing Grain Boundaries and Morphological Improvement of Perovskite Solar Cells from Methodology and Material‐Based Perspectives Choi, Hyuntae; Choi, Kyoungwon; Choi, Yelim Small Methods, Vol. 4, Issue 5 https://doi.org/10.1002/smtd.201900569	journal	September 2019
Lattice Modulation of Alkali Metal Cations Doped Cs _{1− x} R _x PbBr ₃ Halides for Inorganic Perovskite Solar Cells Li, Yanan; Duan, Jialong; Yuan, Haiwen Solar RRL, Vol. 2, Issue 10 https://doi.org/10.1002/solr.201800164	journal	July 2018
The Role of Diammonium Cation on the Structural and Optoelectronic Properties in 3D Cesium–Formamidinium Mixed‐Cation Perovskite Solar Cells Xu, Xiuwen; Xie, Yue-Min; Ma, Yuhui Solar RRL, Vol. 3, Issue 8 https://doi.org/10.1002/solr.201900140	journal	May 2019
Review of Stability Enhancement for Formamidinium‐Based Perovskites Fan, Yingping; Meng, Hongguang; Wang, Li Solar RRL, Vol. 3, Issue 9 https://doi.org/10.1002/solr.201900215	journal	May 2019
The Energy‐Alignment Engineering in Polytriphenylamines‐Based Hole Transport Polymers Realizes Low Energy Loss and High Efficiency for All‐Inorganic Perovskite Solar Cells Zhang, Bin; Zhou, Yingzhi; Xue, Qifan Solar RRL, Vol. 3, Issue 9 https://doi.org/10.1002/solr.201900265	journal	May 2019
Unveiling the Importance of Precursor Preparation for Highly Efficient and Stable Phenethylammonium‐Based Perovskite Solar Cells Lee, Da Seul; Kim, Jincheol; Bing, Jueming Solar RRL, Vol. 4, Issue 4 https://doi.org/10.1002/solr.201900463	journal	April 2020
Highly Efficient and Stable Planar Perovskite Solar Cells with Modulated Diffusion Passivation Toward High Power Conversion Efficiency and Ultrahigh Fill Factor Zhou, Long; Lin, Zhenhua; Ning, Zhijun Solar RRL, Vol. 3, Issue 11 https://doi.org/10.1002/solr.201970111	journal	November 2019
Unveiling the Importance of Precursor Preparation for Highly Efficient and Stable Phenethylammonium‐Based Perovskite Solar Cells Lee, Da Seul; Kim, Jincheol; Bing, Jueming Solar RRL, Vol. 4, Issue 4 https://doi.org/10.1002/solr.202070043	journal	April 2020
Material and Interface Engineering for High‐Performance Perovskite Solar Cells: A Personal Journey and Perspective Qiu, Jianhang; Yang, Shihe The Chemical Record, Vol. 20, Issue 3 https://doi.org/10.1002/tcr.201900028	journal	July 2019
Air-processed, large grain perovskite films with low trap density from perovskite crystal engineering for high-performance perovskite solar cells with improved ambient stability Ding, Manman; Sun, Leijie; Chen, Xiayan Journal of Materials Science, Vol. 54, Issue 18 https://doi.org/10.1007/s10853-019-03768-2	journal	June 2019
Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications Ma, Shuang; Cai, Molang; Cheng, Tai Science China Materials, Vol. 61, Issue 10 https://doi.org/10.1007/s40843-018-9294-5	journal	July 2018
Efficient ambient-air-stable solar cells with 2D–3D heterostructured butylammonium-caesium-formamidinium lead halide perovskites Wang, Zhiping; Lin, Qianqian; Chmiel, Francis P. Nature Energy, Vol. 2, Issue 9 https://doi.org/10.1038/nenergy.2017.135	journal	August 2017
Dimensionality engineering of hybrid halide perovskite light absorbers Gao, Peng; Bin Mohd Yusoff, Abd Rashid; Nazeeruddin, Mohammad Khaja Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-07382-9	journal	November 2018
Highly efficient Cs-based perovskite light-emitting diodes enabled by energy funnelling Ng, Yan Fong; Kulkarni, Sneha A.; Parida, Shayani Chemical Communications, Vol. 53, Issue 88 https://doi.org/10.1039/c7cc06615e	journal	January 2017
Impact of H ₂ O on organic–inorganic hybrid perovskite solar cells Huang, Jianbing; Tan, Shunquan; Lund, Peter D. Energy & Environmental Science, Vol. 10, Issue 11 https://doi.org/10.1039/c7ee01674c	journal	January 2017
Selective growth of layered perovskites for stable and efficient photovoltaics Cho, Kyung Taek; Grancini, Giulia; Lee, Yonghui Energy & Environmental Science, Vol. 11, Issue 4 https://doi.org/10.1039/c7ee03513f	journal	January 2018
Mixed cation hybrid lead halide perovskites with enhanced performance and stability Xu, Feng; Zhang, Taiyang; Li, Ge Journal of Materials Chemistry A, Vol. 5, Issue 23 https://doi.org/10.1039/c7ta00042a	journal	January 2017
Additive engineering for highly efficient organic–inorganic halide perovskite solar cells: recent advances and perspectives Li, Taotao; Pan, Yufeng; Wang, Ze Journal of Materials Chemistry A, Vol. 5, Issue 25 https://doi.org/10.1039/c7ta01798g	journal	January 2017
Gas induced conversion of hybrid perovskite single crystal to single crystal for great enhancement of their photoelectric properties Ju, Dianxing; Zhao, Tianyu; Yangyang, Dang Journal of Materials Chemistry A, Vol. 5, Issue 41 https://doi.org/10.1039/c7ta07413a	journal	January 2017
Mixed halide hybrid perovskites: a paradigm shift in photovoltaics Zarick, Holly F.; Soetan, Naiya; Erwin, William R. Journal of Materials Chemistry A, Vol. 6, Issue 14 https://doi.org/10.1039/c7ta09122b	journal	January 2018
Air-stable formamidinium/methylammonium mixed lead iodide perovskite integral microcrystals with low trap density and high photo-responsivity Wu, Guangbao; Zhou, Jiyu; Meng, Rui Physical Chemistry Chemical Physics, Vol. 21, Issue 6 https://doi.org/10.1039/c8cp07271j	journal	January 2019
Perovskite precursor solution chemistry: from fundamentals to photovoltaic applications Jung, Minsu; Ji, Sang-Geun; Kim, Gwisu Chemical Society Reviews, Vol. 48, Issue 7 https://doi.org/10.1039/c8cs00656c	journal	January 2019
An overview on enhancing the stability of lead halide perovskite quantum dots and their applications in phosphor-converted LEDs Wei, Yi; Cheng, Ziyong; Lin, Jun Chemical Society Reviews, Vol. 48, Issue 1 https://doi.org/10.1039/c8cs00740c	journal	January 2019
Imperfections and their passivation in halide perovskite solar cells Chen, Bo; Rudd, Peter N.; Yang, Shuang Chemical Society Reviews, Vol. 48, Issue 14 https://doi.org/10.1039/c8cs00853a	journal	January 2019
Improving the stability and performance of perovskite solar cells via off-the-shelf post-device ligand treatment Zhang, Hong; Ren, Xingang; Chen, Xiwen Energy & Environmental Science, Vol. 11, Issue 8 https://doi.org/10.1039/c8ee00580j	journal	January 2018
Structural features and their functions in surfactant-armoured methylammonium lead iodide perovskites for highly efficient and stable solar cells Jung, Minsu; Shin, Tae Joo; Seo, Jangwon Energy & Environmental Science, Vol. 11, Issue 8 https://doi.org/10.1039/c8ee00995c	journal	January 2018
Tailored dimensionality to regulate the phase stability of inorganic cesium lead iodide perovskites Li, Faming; Pei, Yunhe; Xiao, Fei Nanoscale, Vol. 10, Issue 14 https://doi.org/10.1039/c8nr00758f	journal	January 2018
Versatile perovskite solar cell encapsulation by low-temperature ALD-Al ₂ O ₃ with long-term stability improvement Ramos, F. Javier; Maindron, Tony; Béchu, Solène Sustainable Energy & Fuels, Vol. 2, Issue 11 https://doi.org/10.1039/c8se00282g	journal	January 2018
Enhanced stability and optoelectronic properties of MAPbI ₃ films by a cationic surface-active agent for perovskite solar cells Zhao, He; Wang, Shirong; Sun, Mengna Journal of Materials Chemistry A, Vol. 6, Issue 23 https://doi.org/10.1039/c8ta00457a	journal	January 2018
Recent progress in 2D/quasi-2D layered metal halide perovskites for solar cells Yan, Jielin; Qiu, Weiming; Wu, Gang Journal of Materials Chemistry A, Vol. 6, Issue 24 https://doi.org/10.1039/c8ta02288g	journal	January 2018
Boosting the performance and stability of quasi-two-dimensional tin-based perovskite solar cells using the formamidinium thiocyanate additive Kim, Hongki; Lee, Yoon Ho; Lyu, Taecheon Journal of Materials Chemistry A, Vol. 6, Issue 37 https://doi.org/10.1039/c8ta05916k	journal	January 2018
Multi-layered hybrid perovskites templated with carbazole derivatives: optical properties, enhanced moisture stability and solar cell characteristics Herckens, Roald; Van Gompel, Wouter T. M.; Song, Wenya Journal of Materials Chemistry A, Vol. 6, Issue 45 https://doi.org/10.1039/c8ta08019d	journal	January 2018
Narrow band gap and high mobility of lead-free perovskite single crystal Sn-doped MA ₃ Sb ₂ I ₉ Ju, Dianxing; Jiang, Xiaomei; Xiao, Hang Journal of Materials Chemistry A, Vol. 6, Issue 42 https://doi.org/10.1039/c8ta08315k	journal	January 2018
Enabling room-temperature processed highly efficient and stable 2D Ruddlesden–Popper perovskite solar cells with eliminated hysteresis by synergistic exploitation of additives and solvents Yu, Shuang; Yan, Yajie; Chen, Yani Journal of Materials Chemistry A, Vol. 7, Issue 5 https://doi.org/10.1039/c8ta09146c	journal	January 2019
Stability progress of perovskite solar cells dependent on the crystalline structure: From 3D ABX ₃ to 2D Ruddlesden–Popper perovskite absorbers Arabpour Roghabadi, Farzaneh; Alidaei, Maryam; Mousavi, Seyede Maryam Journal of Materials Chemistry A, Vol. 7, Issue 11 https://doi.org/10.1039/c8ta10444a	journal	January 2019
Binary organic spacer-based quasi-two-dimensional perovskites with preferable vertical orientation and efficient charge transport for high-performance planar solar cells Chen, Shi; Shen, Nan; Zhang, Luozheng Journal of Materials Chemistry A, Vol. 7, Issue 16 https://doi.org/10.1039/c8ta12476k	journal	January 2019
Synthesis, post-synthetic modification and stability of a 2D styryl ammonium lead iodide hybrid material Peng, Yong; Albero, Josep; Garcia, Hermenegildo Dalton Transactions, Vol. 49, Issue 2 https://doi.org/10.1039/c9dt04285g	journal	January 2020
Orientationally engineered 2D/3D perovskite for high efficiency solar cells Abbas, Muhammad Sohail; Hussain, Sabir; Zhang, Jinaqi Sustainable Energy & Fuels, Vol. 4, Issue 1 https://doi.org/10.1039/c9se00817a	journal	January 2020
Self-assembled propylammonium cations at grain boundaries and the film surface to improve the efficiency and stability of perovskite solar cells Fei, Chengbin; Zhou, Meng; Ogle, Jonathan Journal of Materials Chemistry A, Vol. 7, Issue 41 https://doi.org/10.1039/c9ta01755k	journal	January 2019
Nucleation and crystal growth control for scalable solution-processed organic–inorganic hybrid perovskite solar cells Hu, Hanlin; Singh, Mriganka; Wan, Xuejuan Journal of Materials Chemistry A, Vol. 8, Issue 4 https://doi.org/10.1039/c9ta11245f	journal	January 2020
Water in hybrid perovskites: Bulk MAPbI ₃ degradation via super-hydrous state Kakekhani, Arvin; Katti, Radhika N.; Rappe, Andrew M. APL Materials, Vol. 7, Issue 4 https://doi.org/10.1063/1.5087290	journal	April 2019
Inorganic halide perovskite materials and solar cells Zhang, Cuiling; Arumugam, Gowri Manohari; Liu, Chong APL Materials, Vol. 7, Issue 12 https://doi.org/10.1063/1.5117306	journal	December 2019
Mixed Halide Perovskite Solar Cells: Progress and Challenges Hamed, Mohammed S. G.; Mola, Genene Tessema Critical Reviews in Solid State and Materials Sciences, Vol. 45, Issue 2 https://doi.org/10.1080/10408436.2018.1549976	journal	February 2019
Interfacial crosslinked quasi-2D perovskite with boosted carrier transport and enhanced stability Zhang, Taiyang; Hui, Yong; Chen, Liang Journal of Physics D: Applied Physics, Vol. 51, Issue 40 https://doi.org/10.1088/1361-6463/aad7de	journal	August 2018
An efficient implementation of two-component relativistic density functional theory with torque-free auxiliary variables Petrone, Alessio; Williams-Young, David B.; Sun, Shichao The European Physical Journal B, Vol. 91, Issue 7 https://doi.org/10.1140/epjb/e2018-90170-1	journal	July 2018
Imperfections and their passivation in halide perovskite solar cells J., Huang,; B., Chen,; P. N., Rudd, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/kzq8-3k31	text	January 2019
Attaining High Photovoltaic Efficiency and Stability with Multidimensional Perovskites. Kosasih, Felix; Ducati, Caterina Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.33139	text	January 2018
Controlling the Growth Kinetics and Optoelectronic Properties of 2D/3D Lead–Tin Perovskite Heterojunctions Ruggeri, Edoardo; Anaya, Miguel; Gałkowski, Krzysztof Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.45923	text	January 2019
Mixed 3D-2D passivation treatment for mixed-cation lead mixed-halide perovskite solar cells for higher efficiency and better stability Cho, Yongyoon; Soufiani, Arman Mahboubi; Yun, Jae Sung Proceedings of the 10th International Conference on Hybrid and Organic Photovoltaics https://doi.org/10.29363/nanoge.hopv.2018.080	conference	February 2018
Effects of Decaphenylcyclopentasilane Addition on Photovoltaic Properties of Perovskite Solar Cells Taguchi, Masaya; Suzuki, Atsushi; Oku, Takeo Coatings, Vol. 8, Issue 12 https://doi.org/10.3390/coatings8120461	journal	December 2018
Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells Kim, Min; Figueroa-Tapia, Jetsabel M.; Prato, Mirko Zenodo https://doi.org/10.5281/zenodo.3738931	text	January 2020

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