Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Solution-processed chalcopyrite–perovskite tandem solar cells in bandgap-matched two- and four-terminal architectures

Journal Article · · Journal of Materials Chemistry. A
DOI:https://doi.org/10.1039/C7TA00562H· OSTI ID:1343473
 [1];  [2];  [3];  [2]
  1. Univ. of Washington, Seattle, WA (United States); University of Washington
  2. Univ. of Washington, Seattle, WA (United States)
  3. Univ. of Washington, Seattle, WA (United States); City Univ. of Hong Kong (China)

Solution-processed chalcopyrite and perovskite devices of various bandgaps are combined in four- and two-terminal mechanically-stacked tandem architectures. The excellent low-light performance of Cu(In,Ga)(S,Se)2 and low-bandgap CuIn(S,Se)2 cells and the high efficiency of novel NIR-transparent inverted perovskite cells with C60/bis-C60/ITO as electron transport layers, enabled stabilized two- and four-terminal tandem efficiencies up to 18.5% and 18.8%, respectively, which represent a new record for tandem devices with solution-processed chalcopyrite and perovskite absorbers.

Research Organization:
Univ. of Washington, Seattle, WA (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Solar Energy Technologies Office; Swiss National Science Foundation (SNSF)
Grant/Contract Number:
EE0006710
OSTI ID:
1343473
Report Number(s):
DOE-UW-Uhl-2
Journal Information:
Journal of Materials Chemistry. A, Journal Name: Journal of Materials Chemistry. A Vol. 5; ISSN JMCAET; ISSN 2050-7488
Publisher:
Royal Society of ChemistryCopyright Statement
Country of Publication:
United States
Language:
English

References (58)

Chalcogenide Photovoltaics book January 2011
A Low-Temperature, Solution-Processable, Cu-Doped Nickel Oxide Hole-Transporting Layer via the Combustion Method for High-Performance Thin-Film Perovskite Solar Cells journal October 2015
Thermal and Environmental Stability of Semi-Transparent Perovskite Solar Cells for Tandems Enabled by a Solution-Processed Nanoparticle Buffer Layer and Sputtered ITO Electrode journal February 2016
Tandem Architecture of Perovskite and Cu(In,Ga)(S,Se) 2 Created by Solution Processes for Solar Cells journal September 2016
Enhanced Open-Circuit Voltage in High Performance Polymer/Fullerene Bulk-Heterojunction Solar Cells by Cathode Modification with a C60 Surfactant journal December 2011
High-Performance Planar-Heterojunction Solar Cells Based on Ternary Halide Large-Band-Gap Perovskites journal August 2014
Enhanced Environmental Stability of Planar Heterojunction Perovskite Solar Cells Based on Blade-Coating journal October 2014
Monolithic Perovskite-CIGS Tandem Solar Cells via In Situ Band Gap Engineering journal September 2015
Effects of heavy alkali elements in Cu(In,Ga)Se 2 solar cells with efficiencies up to 22.6% journal July 2016
Performance of Cu(In,Ga)Se2 solar cells under low irradiance journal May 2003
Blue-photon modification of nonstandard diode barrier in CuInSe2 solar cells journal June 1998
Modelling Performance of Two- And Four-terminal Thin-film Silicon Tandem Solar Cells under Varying Spectral Conditions journal December 2015
Effects of formamidinium and bromide ion substitution in methylammonium lead triiodide toward high-performance perovskite solar cells journal April 2016
Efficiency limits for single-junction and tandem solar cells journal November 2006
Crystalline silicon cell performance at low light intensities journal September 2009
Sputtered metal oxide broken gap junctions for tandem solar cells journal January 2015
Efficiency limitations for wide-band-gap chalcopyrite solar cells journal June 2005
Optoelectronic Quality and Stability of Hybrid Perovskites from MAPbI 3 to MAPbI 2 Br Using Composition Spread Libraries journal January 2016
High-Efficiency Polycrystalline Thin Film Tandem Solar Cells journal June 2015
Efficient Monolithic Perovskite/Silicon Tandem Solar Cell with Cell Area >1 cm 2 journal December 2015
High Efficiency Tandem Thin-Perovskite/Polymer Solar Cells with a Graded Recombination Layer journal March 2016
Efficient Near-Infrared-Transparent Perovskite Solar Cells Enabling Direct Comparison of 4-Terminal and Monolithic Perovskite/Silicon Tandem Cells journal August 2016
Multilayer Transparent Top Electrode for Solution Processed Perovskite/Cu(In,Ga)(Se,S) 2 Four Terminal Tandem Solar Cells journal June 2015
Organometallic Halide Perovskites: Sharp Optical Absorption Edge and Its Relation to Photovoltaic Performance journal March 2014
Low-Temperature Solution-Processed Perovskite Solar Cells with High Efficiency and Flexibility journal January 2014
Efficient planar heterojunction perovskite solar cells by vapour deposition journal September 2013
Compositional engineering of perovskite materials for high-performance solar cells journal January 2015
Efficient organometal trihalide perovskite planar-heterojunction solar cells on flexible polymer substrates journal November 2013
Low-temperature-processed efficient semi-transparent planar perovskite solar cells for bifacial and tandem applications journal November 2015
Highly efficient Cu(In,Ga)Se2 solar cells grown on flexible polymer films journal September 2011
Photonic design principles for ultrahigh-efficiency photovoltaics journal February 2012
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells journal July 2014
The emergence of perovskite solar cells journal July 2014
Sub-150 °C processed meso-superstructured perovskite solar cells with enhanced efficiency journal January 2014
Organic–inorganic halide perovskite/crystalline silicon four-terminal tandem solar cells journal January 2015
Semi-transparent perovskite solar cells for tandems with silicon and CIGS journal January 2015
Recent progress and perspective in solution-processed Interfacial materials for efficient and stable polymer and organometal perovskite solar cells journal January 2015
Reversible photo-induced trap formation in mixed-halide hybrid perovskites for photovoltaics journal January 2015
Molecular-ink route to 13.0% efficient low-bandgap CuIn(S,Se) 2 and 14.7% efficient Cu(In,Ga)(S,Se) 2 solar cells journal January 2016
Monolithic perovskite/silicon-heterojunction tandem solar cells processed at low temperature journal January 2016
Cesium-containing triple cation perovskite solar cells: improved stability, reproducibility and high efficiency journal January 2016
Energy-yield prediction for II–VI-based thin-film tandem solar cells journal January 2016
Organic tandem solar cells: A review journal January 2009
Modeling low cost hybrid tandem photovoltaics with the potential for efficiencies exceeding 20% journal January 2012
Composition dependence of defect energies and band alignments in the Cu(In1−xGax)(Se1−ySy)2 alloy system journal February 2002
Secondary barriers in CdS–CuIn1−xGaxSe2 solar cells journal March 2005
Modeling of two‐junction, series‐connected tandem solar cells using top‐cell thickness as an adjustable parameter journal August 1990
Perovskite-kesterite monolithic tandem solar cells with high open-circuit voltage journal October 2014
Detailed balance limit of the efficiency of tandem solar cells journal May 1980
Flexible transparent conductive materials based on silver nanowire networks: a review journal October 2013
Effects of Internal Luminescence and Internal Optics on $V_{\bf oc}$ and $J_{\bf sc}$ of III--V Solar Cells journal October 2013
Interface engineering of highly efficient perovskite solar cells journal July 2014
Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts journal September 2014
Perovskite Solar Cells Keep On Surging journal May 2014
High-performance photovoltaic perovskite layers fabricated through intramolecular exchange journal May 2015
A mixed-cation lead mixed-halide perovskite absorber for tandem solar cells journal January 2016
Perovskite-perovskite tandem photovoltaics with optimized band gaps journal October 2016
High-Temperature Degradation Mechanism of Cu(In,Ga)Se 2 -Based Thin Film Solar Cells journal June 2008

Similar Records

Rapid Development of Hybrid Perovskites and Novel Tandem Architectures
Technical Report · Wed Jan 09 23:00:00 EST 2019 · OSTI ID:1494825

Exploring the Feasibility and Performance of Perovskite/Antimony Selenide Four-Terminal Tandem Solar Cells
Journal Article · Wed Apr 03 00:00:00 EDT 2024 · Solar · OSTI ID:2333040

Related Subjects