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Title: Using a spherical crystallite model with vacancies to relate local atomic structure to irradiation defects in ZrC and ZrN

Journal Article · · Journal of Nuclear Materials

Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI ID:
1341166
Journal Information:
Journal of Nuclear Materials, Journal Name: Journal of Nuclear Materials Vol. 475 Journal Issue: C; ISSN 0022-3115
Publisher:
ElsevierCopyright Statement
Country of Publication:
Netherlands
Language:
English
Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

References (35)

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Nitrides as a nuclear fuel option journal January 2005
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Selection of materials as diluents for burning of plutonium fuels in nuclear reactors journal October 1999
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Transition of nc-SiC powder surface into grain boundaries during sintering by molecular dynamics simulation and neutron powder diffraction journal November 2007
Radiation damage in crystalline insulators, oxides and ceramic nuclear fuels journal January 1982
Stoichiometry effect on the irradiation response in the microstructure of zirconium carbides journal November 2014
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Comparison of extended x-ray absorption fine structure and Scherrer analysis of x-ray diffraction as methods for determining mean sizes of polydisperse nanoparticles journal December 2005
Effects of fast neutron irradiation on zirconium carbide journal April 2010
Study of irradiated mod.9Cr–1Mo steel by synchrotron extended X-ray absorption fine structure journal October 2013
Determination of crystallite size in a magnetic nanocomposite using extended x-ray absorption fine structure journal July 2003
Pertechnetate immobilization with amorphous iron sulfide journal January 2008
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Microstructure and mechanical properties of proton irradiated zirconium carbide journal September 2008
Estimating Crystallite Size in Polydispersed Samples using EXAFS journal January 2005
Improved SelfAbsorption Correction for Fluorescence Measurements of Extended XRay Absorption FineStructure journal January 2005
Research and development on HTGR fuel in the HTTR project journal October 2004
Molecular dynamics study of the milling-induced allotropic transformation in cobalt journal June 2012
Fabrication of uniform ZrC coating layer for the coated fuel particle of the very high temperature reactor journal May 2008
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Scattering-matrix formulation of curved-wave multiple-scattering theory: Application to x-ray-absorption fine structure journal April 1990
Mean coordination numbers and the non-metal–metal transition in clusters journal January 1992
Radiation stability of ZrN under 2.6MeV proton irradiation journal July 2009
Pair distribution function and structure factor of spherical particles journal March 2006

Similar Records

Using a spherical crystallite model with vacancies to relate local atomic structure to irradiation defects in ZrC and ZrN
Journal Article · Tue Nov 22 00:00:00 EST 2016 · Journal of Nuclear Materials · OSTI ID:1341166

THERMAL EXPANSION AND ATOMIC VIBRATION AMPLITUDES FOR TiC, TiN, ZrC, ZrN, AND PURE TUNGSTEN
Journal Article · Wed Apr 01 00:00:00 EST 1964 · Phys. Chem. Solids · OSTI ID:1341166

Most theoretical approaches used in nuclear astrophysics to model the nucleosynthesis of heavy elements incorporate the so-called statistical model in order to describe the excitation and decay properties of atomic nuclei. One of the basic assumptions of this model is the validity of the Brink–Axel hypothesis and the related concept of so-called photon strength functions to describe γ-ray transition probabilities. We present a novel experimental approach that allows for the first time to experimentally determine the photon strength function simultaneously in two independent ways by a unique combination of quasi-monochromatic photon beams and a newly implemented γ–γ coincidence setup. This technique does not assume a priori the validity of the Brink–Axel hypothesis and sets a benchmark in terms of the detection sensitivity for measuring decay properties of photo-excited states below the neutron separation energy. The data for the spherical off-shell nucleus 128Te were obtained for γ-ray beam-energy settings between 3 MeV and 9 MeV in steps of 130 keV for the lower beam energies and in steps of up to 280 keV for the highest beam settings. We present a quantitative analysis on the consistency of the derived photon strength function with the Brink–Axel hypothesis. The data clearly demonstrate a discrepancy of up to a factor of two between the photon strength functions extracted from the photoabsorption and photon emission process, respectively. In addition, we observe that the photon strength functions are not independent of the excitation energy, as usually assumed. Thus, we conclude, that the Brink–Axel hypothesis is not strictly fulfilled in the excitation-energy region below the neutron separation threshold (Sn = 8.78 MeV) for the studied case of 128Te.
Journal Article · Tue Jan 01 00:00:00 EST 2019 · Physics Letters B · OSTI ID:1341166

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