Sum frequency generation vibrational spectroscopy (SFG-VS) for complex molecular surfaces and interfaces: Spectral lineshape measurement and analysis plus some controversial issues
Journal Article
·
· Progress in Surface Science
Sum-frequency generation vibrational spectroscopy (SFG-VS) was first developed in the 1980s and it has been proven a uniquely sensitive and surface/interface selective spectroscopic probe for characterization of the structure, conformation and dynamics of molecular surfaces and interfaces. In recent years, there has been significant progress in the development of methodology and instrumentation in the SFG-VS toolbox that has significantly broadened the application to complex molecular surfaces and interfaces. In this review, after presenting a unified view on the theory and methodology focusing on the SFG-VS spectral lineshape, as well as the new opportunities in SFG-VS applications with such developments, some of the controversial issues that have been puzzling the community are to be discussed. The aim of this review is to present to the researchers and students interested in molecular surfaces and interfacial sciences up-to-date perspectives complementary to the existing textbooks and reviews on SFG-VS.
- Research Organization:
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Sponsoring Organization:
- USDOE
- DOE Contract Number:
- AC05-76RL01830
- OSTI ID:
- 1339877
- Report Number(s):
- PNNL-SA--121029; 48274
- Journal Information:
- Progress in Surface Science, Journal Name: Progress in Surface Science Journal Issue: 4 Vol. 91; ISSN 0079-6816
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
Similar Records
Unified treatment and measurement of the spectral resolution and temporal effects in frequency-resolved sum-frequency generation vibrational spectroscopy (SFG-VS)
Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization and Orientation
Vibrational Spectral Signatures of Crystalline Cellulose Using High Resolution Broadband Sum Frequency Generation Vibrational Spectroscopy (HR-BB-SFG-VS)
Journal Article
·
Fri Dec 13 23:00:00 EST 2013
· Physical Chemistry Chemical Physics. PCCP, 15(46):19970-19984
·
OSTI ID:1108141
Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization and Orientation
Journal Article
·
Wed Apr 01 00:00:00 EDT 2015
· Annual Review of Physical Chemistry, 66:189-216
·
OSTI ID:1208772
Vibrational Spectral Signatures of Crystalline Cellulose Using High Resolution Broadband Sum Frequency Generation Vibrational Spectroscopy (HR-BB-SFG-VS)
Journal Article
·
Mon Mar 02 23:00:00 EST 2015
· Cellulose, 22(3):1469-1484
·
OSTI ID:1182941